Browse > Article
http://dx.doi.org/10.11001/jksww.2015.29.6.685

Application of in situ Liquid Ferrate(VI) for 2-Bromophenol Removal  

Laksono, Fajar Budi (Dept. of Marine Convergence Design, Pukyong National University)
Kim, Il-Kyu (Dept. of Environmental Engineering, Pukyong National University)
Publication Information
Journal of Korean Society of Water and Wastewater / v.29, no.6, 2015 , pp. 685-692 More about this Journal
Abstract
The concern over the risk of environmental exposure to brominated phenols has been increased and has led the researchers to focus their attention on the study of bromophenol treatment. In this study, the effects of pH and ferrate(VI) dose on the degradation of 2-bromophenol were investigated. The results indicated that the oxidation of 2-bromophenol by liquid ferrate(VI) was found to be highly sensitive to the pH condition. Furthermore, the highest removal efficiency was observed at the neutral condition with the removal efficiency of 94.2%. In addition, experimental results showed that 2-bromophenol removal efficiency increased with increasing of ferrate dosage. Ferrate(VI) dose of 0.23 mM was sufficient to remove most of the 2-bromophenol with the efficiency of 99.73% and kapp value of $2982M^{-1}s^{-1}$. Seven compounds were identified as the intermediate products by the GC/MS analysis.
Keywords
liquid ferrate(VI); 2-bromophenol; oxidation; intermediates;
Citations & Related Records
연도 인용수 순위
  • Reference
1 Al-Abduly, A., & Sharma, V. K. (2014). Oxidation of benzothiophene, dibenzothiophene, and methyl-dibenzothiophene by ferrate(VI). Journal of Hazardous Materials, 279, 296-301. http://doi.org/10.1016/j.jhazmat.2014.06.083   DOI
2 Chengchun, J., Chen, L., & Shichao, W. (2008). Preparation of Potassium Ferrate by Wet Oxidation Method Using Waste Alkali: Purification and Reuse of Waste Alkali. In Ferrates (Vol. 985, pp. 5-94). American Chemical Society. http://doi.org/doi:10.1021/bk-2008-0985.ch005   DOI
3 Dell'Erba, A., Falsanisi, D., Liberti, L., Notarnicola, M., & Santoro, D. (2007). Disinfection by-products formation during wastewater disinfection with peracetic acid. Desalination, 215(1-3), 177-186. http://doi.org/10.1016/j.desal.2006.08.021   DOI
4 Evans, C. S., & Dellinger, B. (2005). Mechanisms of dioxin formation from the high-temperature oxidation of 2-bromophenol. Environmental Science and Technology, 39(7), 2128-2134. http://doi.org/10.1021/es048461y   DOI
5 Graham, N., Jiang, C. C., Li, X. Z., Jiang, J. Q., & Ma, J. (2004). The influence of pH on the degradation of phenol and chlorophenols by potassium ferrate. Chemosphere, 56(10), 949-956. http://doi.org/10.1016/j.chemosphere.2004.04.060   DOI
6 Huang, H., Sommerfeld, D., & Dunn…, B. C. (2001). Ferrate (VI) oxidation of aqueous phenol: kinetics and mechanism. The Journal of …, (Vi), 3536-3541. Retrieved from http://pubs.acs.org/doi/abs/10.1021/jp0039621\npapers://d1ebd311-64c1-4c1d-9832-9631d7abf4b4/Paper/p11918   DOI
7 Jeong, H. Y., & Kim, H. (2007). Transformation of Their Mackinawite ( FeS ) in the Presence, 41(22), 7736-7743.   DOI
8 Jiang, J. Q. (2007). Research progress in the use of ferrate(VI) for the environmental remediation. Journal of Hazardous Materials, 146(3), 617-623. http://doi.org/10.1016/j.jhazmat.2007.04.075   DOI
9 Jiang, J.-Q. (2014). Advances in the development and application of ferrate(VI) for water and wastewater treatment. Journal of Chemical Technology & Biotechnology, 89(2), 165-177. http://doi.org/10.1002/jctb.4214   DOI
10 Knight, V. K., Kerkhof, L. J., & Ha, M. M. (1999). Community analyses of sul¢dogenic 2-bromophenol- dehalogenating and phenol-degrading microbial consortia. FEMS Microbiology Ecology, 29, 137-147.   DOI
11 Lee, Y., Yoon, J., & Von Gunten, U. (2005). Kinetics of the oxidation of phenols and phenolic endocrine disruptors during water treatment with ferrate (Fe(VI)). Environmental Science and Technology, 39(22), 8978-8984. http://doi. org/10.1021/es051198w   DOI
12 Li, C., Li, X. Z., Graham, N., & Gao, N. Y. (2008). The aqueous degradation of bisphenol A and steroid estrogens by ferrate. Water Research, 42(1-2), 109-120. http://doi.org/10.1016/j.watres.2007.07.023   DOI
13 Sharma, V. K. (2002). Potassium ferrate(VI): An environmentally friendly oxidant. Advances in Environmental Research, 6(2), 143-156. http://doi.org/10.1016/S1093-0191(01)00119-8   DOI
14 Rhee, S. K., Fennell, D. E., Häggblom, M. M., & Kerkhof, L. J. (2003). Detection by PCR of reductive dehalogenase motifs in a sulfidogenic 2-bromophenol-degrading consortium enriched from estuarine sediment. FEMS Microbiology Ecology, 43(3), 317-324. http://doi.org/10.1016/S0168-6496(02)00435-X   DOI
15 Roberts, a L. (2000). Pathways and Kinetics of Chlorinated Ethylene and Chlorinated Acetylene Reaction with Fe (0) Particles, 34(9), 1794-1805. http://doi.org/10.1021/es990884q   DOI
16 Rush, J. D., Zhao, Z., & Bielski, B. H. J. (1996). Reaction of Ferrate (VI)/Ferrate (V) with Hydrogen Peroxide and Superoxide Anion - a Stopped-Flow and Premix Pulse Radiolysis Study. Free Radical Research, 24(3), 187-198. http://doi.org/10.3109/10715769609088016   DOI
17 Sharma, V. K. (2010). Oxidation of inorganic compounds by Ferrate (VI) and Ferrate(V): One-electron and two-electron transfer steps. Environmental Science and Technology, 44(13), 5148-5152. http://doi.org/10.1021/es1005187   DOI
18 Sharma, V. K. (2011). Oxidation of inorganic contaminants by ferrates (VI, V, and IV)-kinetics and mechanisms: A review. Journal of Environmental Management, 92(4), 1051-1073. http://doi.org/10.1016/j.jenvman.2010.11.026   DOI
19 Sharma, V. K. (2013). Ferrate(VI) and ferrate(V) oxidation of organic compounds: Kinetics and mechanism. Coordination Chemistry Reviews, 257(2), 495-510. http://doi.org/10.1016/j.ccr.2012.04.014   DOI
20 Sharma, V. K., & Bielski, B. H. J. (1991). Reactivity of ferrate(VI) and ferrate(V) with amino acids. Inorganic Chemistry, 30(23), 4306-4310. http://doi.org/10.1021/ic00023a005   DOI
21 Uhnakova, B., Petrickova, a., Biedermann, D., Homolka, L., Vejvoda, V., Bednar, P., … Martinkova, L. (2009). Biodegradation of brominated aromatics by cultures and laccase of Trametes versicolor. Chemosphere, 76(6), 826-832. http://doi.org/10.1016/j.chemosphere.2009.04.016   DOI
22 Sharma, V. K., Burnett, C. R., & Millero, F. J. (2001). Dissociation constants of the monoprotic ferrate(VI) ion in NaCl media. Physical Chemistry Chemical Physics, 3(11), 2059-2062. http://doi.org/10.1039/b101432n   DOI
23 Sharma, V. K., Rendon, R. a., Millero, F. J., & Vazquez, F. G. (2000). Oxidation of thioacetamide by ferrate(VI). Marine Chemistry, 70(1-3), 235-242. http://doi.org/10.1016/S0304-4203(00)00029-3   DOI
24 Thompson, G. W., Ockerman, L. T., & Schreyer, J. M. (1951). Preparation and Purification of Potassium Ferrate. VI. Journal of the American Chemical Society, 73(3), 1379- 1381. http://doi.org/10.1021/ja01147a536   DOI
25 Vetter, W., & Janussen, D. (2005). Halogenated natural products in five species of antarctic sponges: Compounds with POP-like properties? Environmental Science and Technology, 39(11), 3889-3895. http://doi.org/10.1021/es0484597   DOI
26 White, D. a., & Franklin, G. S. (1998). A Preliminary Investigation into the Use of Sodium Ferrate in Water Treatment. Environmental Technology, 19(11), 1157-1161. http://doi. org/10.1080/09593331908616776   DOI
27 Williams, D. H., & Riley, J. T. (1974). Preparation and alcohol oxidation studies of the ferrate(VI) ion, FeO42−. Inorganica Chimica Acta, 8(0), 177-183. http://doi. org/http://dx.doi.org/10.1016/S0020-1693(00)92612-4   DOI
28 Yang, B., Ying, G.-G., Chen, Z.-F., Zhao, J.-L., Peng, F.-Q., & Chen, X.-W. (2014). Ferrate(VI) oxidation of tetrabromobisphenol A in comparison with bisphenol A. Water Research, 62(Vi), 211-219. http://doi.org/10. 1016/j.watres.2014.05.056   DOI
29 Yang, B., Ying, G. G., Zhang, L. J., Zhou, L. J., Liu, S., & Fang, Y. X. (2011). Kinetics modeling and reaction mechanism of ferrate(VI) oxidation of benzotriazoles. Water Research, 45(6), 2261-2269. http://doi.org/10.1016/ j.watres.2011.01.022   DOI
30 Yang, B., Ying, G. G., Zhao, J. L., Liu, S., Zhou, L. J., & Chen, F. (2012). Removal of selected endocrine disrupting chemicals (EDCs) and pharmaceuticals and personal care products (PPCPs) during ferrate(VI) treatment of secondary wastewater effluents. Water Research, 46(7), 2194-2204. http://doi.org/10.1016/j.watres.2012.01.047   DOI
31 YU, M., PARK, G., & KIM, H. (n.d.). Oxidation of Nonylphenol Using Ferrate. ACS Symposium Series, 985, 389-403. Retrieved from http://cat.inist.fr/?aModele=afficheN& cpsidt=20486426