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http://dx.doi.org/10.5805/SFTI.2018.20.3.323

The Development of Enzymatic Mordanting Using Laccase for Phenolic Natural Dye  

Lee, Hye Bin (Dept. of Textile & Clothing, Sookmyung Women's University)
Song, Ji Eun (Dept. of Textile & Clothing, Sookmyung Women's University)
Shim, Eui Jin (Dept. of Textile & Clothing, Sookmyung Women's University)
Kim, Hye Rim (Dept. of Textile & Clothing, Sookmyung Women's University/Research Institute of ICT Convergence, Sookmyung Women's University)
Publication Information
Fashion & Textile Research Journal / v.20, no.3, 2018 , pp. 323-330 More about this Journal
Abstract
This study aim is to provide new coloration method by laccase-catalyzation on natural phenolic dyeing process. In this study, silk was dyed with black tea, which is one of polyphenolic dye, extracted in distilled water. The dyed samples were catalyzed by laccase as the eco-friendly mordanting process. To optimize the conditions of laccase-catalyzed coloration, conditions were varied by different mordanting methods (one-bath, two-bath), temperature and treatment time. The dye affinity in terms of the value of K/S, $L^*$, $a^*$, $b^*$, and H, V, C was measured by Computer Color Matching System (CCM, CM-2600d, Spectra Magic NX, Korea). The effect of laccase-catalyzed coloration on washing fastness was evaluated and compared with the synthetic mordant (Al, Cu, and Fe). As the result of color analysis of dyed silk, the optimum conditions of laccase-catalyzed coloration were determined to post-mordanting by one-bath at $50^{\circ}C$ for 3 hours. Under the optimum laccase-catalyzed conditions, the dyed silk was shown the color of yellowish-red. After laccase-catalyzed coloration on the dyed silk, the improvement of washing fastness was obtained compared with mordanted silk by synthetic mordant (Al, Cu, and Fe). Therefore, the present study was demonstrated that the effective enzymatic mordanting method by laccase for phenolic natural dyeing with vivid color and good fastness.
Keywords
enzyme mordanting; laccase; phenol; natural dye; black tea;
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Times Cited By KSCI : 4  (Citation Analysis)
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1 Jeong, C. H., Kang, S. T., Joo, O. S., Lee, S. C., Shin, Y. H., Shim, K. H., Cho, S. H., Choi, S. G., & Heo, H. J. (2009). Phenolic content, antioxidant effect and acetylcholinesterase inhibitory activity of Korean commercial green, puer, oolong, and black teas. The Korean Society of Food Preservation, 16(2), 230-237.
2 Lee, S. D. (2008). The persimmon dye with experiment of changing concentration and iron-dye process, its application possibility for textile design. Fashion & Textile Research Journal, 10(6), 822-826.
3 Manole, A., Herea, D., Chiriac, H., & Melnig, V. (2008). Laccase activity determination. Cuza University Scientific Annals Lasi, 4, 17-24.
4 Martins, S., Mussatto, S. I., Martinez-Avila, G., Montañez-Saenz, J., Aguilar, C. N., & Teixeira, J. A. (2011). Bioactive phenolic compounds: Production and extraction by solid-state fermentation. A review. Biotechnology Advances, 29(3), 365-373. doi:10.1016/j.biotechadv.2011.01.008   DOI
5 Mayer, A. M., & Staples, R. C. (2002). Laccase: new functions for an old enzyme. Phytochemistry, 60(6), 551-565. doi:10.1016/S0031-9422(02)00171-1   DOI
6 Murugesan, K., Nam, I. H., Kim, Y. M., & Chang, Y. S. (2007). Decolorization of reactive dyes by a thermostable laccase produced by ganoderma lucidum in solid state culture. Enzyme and Microbial Technology, 40(7), 1662-1672. doi:10.1016/j.enzmictec.2006.08.028   DOI
7 Riva, S. (2006). Laccases: blue enzymes for green chemistry. Trends in Biotechnology, 24(5), 219-226. doi:10.1016/j.tibtech.2006.03.006   DOI
8 Samanta, A. K., & Konar, A. (2011). Dyeing of textiles with natural dyes. IntechOpen. Retrieved November 11, 2011, from http://www.intechopen.com/books/natural-dyes/dyeing-of-textiles-withnatural-dyes
9 Seo, H. Y., Kim, H. R., & Song, H. S. (2011). Effects of chestnut hulls mordant on oenothera odorata jacguin-dyed Fabrics. Fashion & Textile Research Journal, 13(6), 983-990. doi:10.5805/KSCI.2011.13.6.983   DOI
10 Seo, M. H., & Shin, Y. S. (1998). Dyeing properties of silk with black tea colorants. Journal of the Korean Society of Clothing and Textiles, 22(5), 557-564.
11 Song, H. J., Kim, H. R., & Song, H. S. (2009). Dyeing properties and scouring of wool/polyester blend fabrics using papain from carica papaya. Journal of the Korean Society of Clothing and Textiles, 33(2), 213-221. doi:10.5850/JKSCT.2009.33.2.213   DOI
12 Sun, S. S., & Tang, R.C. (2013). Laccase-catalyzed coloration of silk with tea polyphenols. Material Sciences and Manufacturing Technology, 629, 352-357. doi:10.4028/www.scientific.net/AMR.629.352
13 Tavares, A., Rodriguez, O., & Macedo, E. (2008). Ionic liquids as alternative co-solvents for laccase: study of enzyme activity and stability. Biotechnology and Bioengineering, 101(1), 201-207. doi:10.1002/bit.21866   DOI
14 Yoon, S. H., & Lim, Y. J. (2005). 천연염료의 안정화 및 염색의 재현성 확립 [Establishment of stabilization of natural dyes and reproducibility of dyeing]. Fiber Technology and Industry, 9(2), 162-176.
15 Yuan, M., Wang, Q., Bai, R., Fan, X., Shen, J., & Smith, E. (2017). Enzymatic coloration and finishing of wool with laccase and polyethylenimine. Textile Research Journal, Advance online publication. doi:10.1177/0040517517712096
16 Camarero, S., Ibarra, D., Martinez, A. T., Romero, J., Gutierrez, A., & del Rio, J. C. (2007). Paper pulp delignification using laccase and natural mediators. Enzyme and Microbial Technology, 40(5), 1264-1271. doi:10.1016/j.enzmictec.2006.09.016   DOI
17 Bai, R., Yu, Y., Wang, Q., Yuan, J., & Fan, X. (2016). Effect of laccase on dyeing properties of polyphenol-based natural dye for wool fabric. Fibers and Polymers, 17(10), 1613-1620. doi:10.1007/s12221-016-5598-5   DOI
18 Boo, H. O., Kim, Y. H., & Song, W. S. (2010). Total phenolic componds contents and tyrosinase inhibition activities according to each kind of natural plant pigments. Proceedings of the Plant Resources Society, Fall Conference, Korea, p. 185.
19 Bourbonnais, R., & Paice, M. G. (1990). Oxidation of non-phenolic substrates: an expanded role for laccase in lignin biodegradation. FEBS Letters, 267(1), 99-102.   DOI
20 Cavaco-Paulo, A., & Gubitz, G. (2003). Textile processing with enzymes. Manchester: Woodhead publishing.
21 Cha, O. S., & Kim, S. H. (1999). A study on the dyeability and physical properties of mordanted and natural-dyed fabrics. Journal of the Korean Society of Clothing and Textiles, 23(6), 788-800.
22 Chung, Y. R., & Song, H. S. (2013). Denim decolorization using laccase. Journal of the Korean Society of Clothing and Textiles, 37(3), 348-357. doi:10.5850/JKSCT.2013.37.3.348   DOI
23 Hadzhiyska, H., Calafell, M., Gibert, J. M., Dagà, J. M., & Tzanov, T. (2006). Laccase-assisted dyeing of cotton. Biotechnology Letters, 28(10), 755-759. doi:10.1007/s10529-006-9043-5   DOI