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PRELIMINARY STUDY ON THE ALPHA TRACK ANALYSIS OF SPHERICAL URANIUM METAL PARTICLES  

Pyo Hyung-Yeol (Korea Atomic Energy Research Institute)
Kim Jong-Yun (Korea Atomic Energy Research Institute)
Lee Myung-Ho (Korea Atomic Energy Research Institute)
Park Yong-Jun (Korea Atomic Energy Research Institute)
Jee Kwang-Yong (Korea Atomic Energy Research Institute)
Kim Won-Ho (Korea Atomic Energy Research Institute)
Publication Information
Nuclear Engineering and Technology / v.38, no.4, 2006 , pp. 353-358 More about this Journal
Abstract
Alpha track analysis for the determination of the trace amount of alpha emitting nuclides in a very small particle was performed as an efficient and powerful technique during safeguard inspection. Metal particles with well-defined spherical shape, size and isotopic compositions as a reference material were used to correlate the number of tracks or track diameter with an isotopic composition eventually to identify the uranium enrichment in the environmental swipe samples. Slopes in the number of tracks versus the exposure time curve provide a simple insight into the uranium enrichment of an unknown particle. Low enriched uranium metal particles result in slopes still steeper than the depleted or natural uranium metal particles. In addition, a linear relationship between track diameter and particle size Is thought to be a useful first stage analytical tool as an efficient and convenient inspection guide. The significance of the simple linear model was also judged using the usual statistical tests.
Keywords
Solid-state Nuclear Track Detector; Alpha Track Analysis; Swipe Sample; Uranium Micro-particles; Uranium Content; Enrichment; Number of Track; Track Diameter;
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  • Reference
1 Y. J. Park, M. H. Lee, H. Y. Pyo, H. A. Kim, S. C. Sohn, K. Y. Jee and W. H. Kim, 'The Preparation of Uranium-Adsorbed Silica Particles as a Reference Material for the Fission Track Analysis', Nucl. Instrum. Meth. A, 545, 493 (2005)   DOI   ScienceOn
2 K. Y. Jee, M. H. Lee, H. Y. Pyo, Y. J. Park and W. H. Kim, 'A Study on Fission Track Analysis Technique for Uraniumadsorbed Silica Reference Particles', Proceedings of the International Symposium on Research Reactor and Neutron Science (HANARO 2005), Daejeon, Korea, April, 11?13, 2005
3 J. Jernstrom, M. Eriksson, J. Osan, G. Tamborini, S. Torok, R. Simon, G. Falkenberg, A. Alsecz and M. Betti, 'Nondestructive Characterisation of Low Radioactive Particles from Irish Sea Sediment by Micro X-ray Synchrotron Radiation Techniques: Micro X-ray Fluorescence (l-XRF) and Micro X-ray Absorption Near Edge Structure (l-XANES) Spectroscopy' J. Anal. At. Spectrom., 19, 1428 (2004)   DOI   ScienceOn
4 O. Stetzer, M. Betti, J. van Geelb, N. Erdmann,.J.-V. Kratza, R. Schenkel and N. Trautmann, 'Determination of the 235U Content in Uranium Oxide Particles by Fission Track Analysis', Nucl. Instrum. Meth. A, 525, 582 (2004)   DOI   ScienceOn
5 D. A. Young, 'Etching of Radiation Damage in Lithium Fluoride', Nature, 182, 375 (1958)   DOI   ScienceOn
6 R. L. Fleischer, P. B. Price and R. M. Walker, Nuclear Tracks in Solids: Principles and Applications, University of California Press, Berkeley, California (1975)
7 D. Nikezic and K. N. Yu, 'Formation and Growth of Tracks in Nuclear Track Materials', Mater. Sci. Eng., R46, 51 (2004)
8 M. Betti, G. Tamborini and L. Koch, 'Use of Secondary Ion Mass Spectrometry in Nuclear Forensic Analysis for the Characterization of Plutonium and Highly Enriched Uranium Particles', Anal. Chem., 71(14), 2616 (1999)   DOI   ScienceOn
9 B. Center and F. H. Ruddy, 'Detection and Characterization of Aerosols Containing Transuranic Elements with the Nuclear Track Technique', Anal. Chem., 48(14), 2135 (1976)   DOI
10 D. L. Donohue, 'Strengthen IAEA Safeguards Through Environmental Sampling and Analysis', J. Alloy. Compd., 271-273, 11 (1998)   DOI   ScienceOn