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http://dx.doi.org/10.5322/JES.2012.21.1.11

Characterization of Volatile Organic Compounds in New Residential Buildings Before Moving-in  

Shin, Seung-Ho (Department of Environmental Engineering, Kyungpook National University)
Jo, Wan-Kuen (Department of Environmental Engineering, Kyungpook National University)
Publication Information
Journal of Environmental Science International / v.21, no.1, 2012 , pp. 11-21 More about this Journal
Abstract
This study investigated the characteristics of selected volatile organic compounds(VOCs) in newly-finished residential buildings, before the occupants moved in. This investigation was carried out by measuring the indoor and outdoor concentrations of selected VOCs before the occupants moved in and by utilizing an indoor mass balance model. Among 25 target VOCs, five aromatics(benzene, ethyl benzene, toluene, m,p-xylene, and o-xylene) were detected in all samples of both indoor and outdoor air. Toluene was most abundant VOC in the indoor air of new apartments, with a median value of 168 mg $m^{-3}$. Unlike other VOCs, halogenated compounds would not be significantly emitted from building materials. The indoor air concentrations of all selected VOCs, except for 1,3,5-trimethyl benzene, exhibited significant correlations each other, while for outdoor air concentrations, five aromatics only were significantly correlated between them. The emission rate of toluene was higher for the current study(median value, 76.8 mg $m^{-2}\;h^{-1}$) than for a previous study, while the emission rates of limonene, a-pinene and b-pinene(geometric means of 2.4, 13.8 and 9.6 mg $m^{-2}\;h^{-1}$, respectively) were lower and the emission rates of m,p-xylene and 2-butanone(geometric means of 10.9 and 21.3 mg $m^{-2}\;h^{-1}$, respectively) were similar. Although there were a few exceptions, the emission strengths are likely proportional to indoor temperature, and appear to reversely proportional to air exchange rate.
Keywords
Emission characterization; Building materials; Indoor model; New apartment; Air exchange rate;
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1 Nielsen, G. D., Larsen, S. T., Olsen, O., Lovik, M., Poulsen, L. K., Glue, C., Wolkoff, P., 2007, Do indoor chemicals promote development of airway allergy?, Indoor Air, 17, 236-255.   DOI   ScienceOn
2 OEHHA (Office of Environmental Health Hazard Assessment), 2005, Proposition 65 Status Report Safe Harbor Levels: No Significant Risk Levels for Carcinogens and Maximum Allowable Dose Levels for Chemicals Causing Reproductive Toxicity, California Environmental Protection Agency, Office of Environmental Health Hazard Assessment, California EPA, August 2005.
3 Ohura, T., Amagai, T., Senga, Y., Fusaya, M., 2006, Organic air pollutants inside and outside residences in Shimizu, Japan: levels, sources and risks, Sci. Total Environ., 366, 485-499.   DOI
4 Ohura, T., Amagai, T., Shen, X., Li, S., Zhang, P., Zhu, L., 2009, Comparative study on indoor air quality in Japan and China: characteristics of residential indoor and outdoor VOCs, Atmos. Environ., 43, 6352-6359.   DOI   ScienceOn
5 Park, J. S., Ikeda, K., 2006, Variations of formaldehyde and VOC levels during 3 years in new and older homes, Indoor Air, 16, 129-135.   DOI   ScienceOn
6 Edwards, R. D., Schweizer, C., Jantunen, M., Lai, H. K., Bayer-Oglesby, L., Katsouyanni, K., Nieuwenhuijsen, M., Saarela, K., Sram, R., Kunzli, N., 2005, Personal exposures to VOC in the upper end of the distribution-relationships to indoor, outdoor and workplace concentrations, Atmos. Environ., 39, 2299-2307.   DOI   ScienceOn
7 Geiss, O., Giannopoulos, G., Tirendi, S., Barrero- Moreno, J., Larsen, B. R., Kotzias, D., 2011, The AIRMEX study - VOC measurements in public buildings and schools/kindergartens in eleven European cities: statistical analysis of the data, Atmos. Environ., 45, 3676-3684.   DOI   ScienceOn
8 Gokhale, S., Kohajda, T., Schlink, U., 2008, Source apportionment of human personal exposure to volatile organic compounds in homes, offices and outdoors by chemical mass balance and genetic algorithm receptor models, Sci. Total Environ., 407, 122-138.   DOI   ScienceOn
9 Parra, M. A., Elustondo, D., Bermejo, R., Santamaria, J. M., 2008, Exposure to volatile organic compounds (VOC) in public buses of Pamplona, Northern Spain, Sci. Total Environ., 404, 18-25.   DOI   ScienceOn
10 Peng, C. -Y., Lan, C. -H., Wu, T. -J., 2009, Investigation of indoor chemical pollutants and perceived odor in an area with complaints of unpleasant odors, Build. Environ., 44, 2106-2113.   DOI   ScienceOn
11 Roukos, J., Riffault, V., Locoge, N., Plaisance, H., 2009, VOC in an urban and industrial harbor on the French North Sea coast during two contrasted meteorological situations, Environ. Poll., 157, 3001-3009.   DOI   ScienceOn
12 Sarigiannis, D. A., Karakitsios, S. P., Gotti, A., Liakos, I. L., Katsoyiannis, D., 2011, Exposure to major volatile organic compounds and carbonyls in European environments and associated health risk, Environ. Int., 37, 743-765.   DOI   ScienceOn
13 Schlink, U., Rehwagen, M., Damm, M., Richter, M., Borte, M., Herbarth, O., 2004, Seasonal cycle of indoor-VOCs: comparsion of apartments and cities, Atmos. Environ., 38, 1181-1190.   DOI   ScienceOn
14 Jia, C., Batterman, S., Godwin, C., 2008, VOCs in industrial, urban and suburban neighborhoods-Part 2: Factors affecting indoor and outdoor concentrations, Atmos. Environ., 42, 2101-2116.   DOI   ScienceOn
15 Han, K. H., Zhang, J. S., Knudsen, H. N., Wargocki, P., Chen, H., Varshney, P. K., Guo, B., 2011, Development of a novel methodology for indoor emission source identification, Atmos. Environ., 45, 3034-3045.   DOI   ScienceOn
16 Hodgson, A. T., Rudd, A. F., Beal, D., Chandra, S., 2000, Volatile organic compound concentrations and emission rates in new manufactured and site-built houses, Indoor Air, 10, 178-192.   DOI   ScienceOn
17 Jarnstrom, H., Saarela, K., Kalliokoski, P., Pasanen, A. -L., 2006, Reference values for indoor air pollution concentrations in new residential buildings in Finland, Atmos. Environ., 40, 7178-7191.   DOI   ScienceOn
18 Jia, C., Batterman, S., Godwin, C., Charles, S., Chin, J. Y., 2010, Sources and migration of volatile organic compounds in mixed-use buildings, Indoor Air, 20, 357-369.   DOI   ScienceOn
19 Kwon, K. D., Jo, W. K., Lim, H. J., Jeong, W. S., 2008, Volatile Pollutants Emitted From Selected Liquid Household Products, Environ. Sci. Poll. Res., 15, 521-526.   DOI   ScienceOn
20 Schlink, U., Thiem, A., Kohajda, T., Richter, M., Strebel, K., 2010, Quantile regression of indoor air concentrations of volatile organic compounds (VOC), Sci. Total Environ., 408, 3840-3851.   DOI   ScienceOn
21 Su, F. -C., Mukherjee, B., Batterman, S., 2011, Trends of VOC exposures among a nationally representative sample: analysis of the NHANES 1988 through 2004 data sets, Atmos. Environ., 45, 4858-4867.   DOI   ScienceOn
22 Takigawa, T., Wang, B. L., Sakano, N., Wang, D. H., Ogino, K., Kishi, R., 2009, A longitudinal study of environmental risk factors for subjective symptoms associated with sick building syndrome in new dwellings, Sci. Total Environ., 407, 5223-5228.   DOI   ScienceOn
23 Tuomainen, M., Tuomainen, A., Liesvuori, J., Pasanen, A. -P., 2001, The 3-year follow-up study in a block of flats - experiences in the use of the Finnish indoor climate classification, Indoor Air, 13, 136-147.   DOI
24 Weisel, C. P., Nicholas, N. J., Lioy, P. J., 1992, Exposure to emissions from gasoline within automobile cabins, J. Expos. Anal. Environ. Epidemiol., 2, 79-96.
25 Leuchner, M., Rappengluck, B., 2010, VOC sourcereceptor relationships in Houston during TexAQS-II, Atmos. Environ., 44, 4056-4067.   DOI   ScienceOn
26 Lim, S., Lee, K., seo, S., Jang, S., 2011, Impact of regulation on indoor volatile organic compounds in new unoccupied apartment in Korea, Atmos. Environ, 45, 1994-2000.   DOI   ScienceOn
27 Loh, M. M., Houseman, E. A., Gray, G. M., Levy, J. I., Spengler, J. D., Bennett, D. H., 2006, Measured concentrations of VOCs in several non-residential microenvoronments in the United States, Enviro. Sci. Technol., 40, 6903-6911.   DOI   ScienceOn
28 Na, K., Kim, Y. P., 2007, Chemical mass balance receptor model applied to ambient $C_2$-$C_9$ VOC concentration in Seoul, Korea : effect of chemical reaction losses, Atmos. Environ., 41, 6715-6728.   DOI   ScienceOn
29 Deng, Q., Yang, X., Zhang, J. S., 2012, Key factor analysis of VOC sorption and its impact on indoor concentrations: the role of ventilation, Build. Environ., 47, 182-187.   DOI
30 Delfino, R. J., Gong, H., Linn, W. S., Hu, Y., Pellizzari, E. D., 2003, Respiratory symptoms and peak expiratory flow in children with asthma in relation to volatile organic compounds in exhaled breath and ambient air, J. Expo. Anal. Environ. Epidemiol., 13, 348-363.   DOI   ScienceOn