Browse > Article
http://dx.doi.org/10.5012/bkcs.2009.30.1.097

New Calculation of Charge Generation Efficiency and Photocurrent in Organic Photoconducting Device  

Lee, Choong-Kun (Department of Chemistry, Hanyang University)
Oh, Jin-Woo (Department of Chemistry, Hanyang University)
Choi, Chil-Sung (Department of Chemistry, Hanyang University)
Lee, Nam-Soo (Department of Chemistry, Chungbuk National University)
Kim, Nak-Joong (Department of Chemistry, Hanyang University)
Publication Information
Abstract
A new approach was applied to examine the charge generation and transport in organic photoconductive devices by Monte‐Carlo simulation utilizing multiple site interactions of carriers with all other charges within Coulomb radius. Stepwise generation frame was considered first by a charge separation process that was counted in two separate transactions, i.e., hopping against physical decay and dissociation against recombination. Thereafter, diffusion/ drifting process of free carriers was counted to follow. This method enables to examine readily the photocurrent generated alongside the charge generation efficiency. The field and temperature dependences of the efficiency and photocurrent were obtained comparable to Onsager’s and experimental data.
Keywords
Monte Carlo simulation; Photo charge generation; Photocurrent; Multiple site interaction;
Citations & Related Records
Times Cited By KSCI : 2  (Citation Analysis)
Times Cited By Web Of Science : 2  (Related Records In Web of Science)
Times Cited By SCOPUS : 2
연도 인용수 순위
1 Melz, P. J. J. Chem. Phys. 1972, 57, 1694   DOI
2 Offermans, T.; Meskers, S. C. J.; Janssen, R. A. J. J. Chem. Phys. 2003, 119, 10924   DOI   ScienceOn
3 Borsenberger, P. M.; Weiss, D. S. Organic Photoreceptors for Imaging Systems; Marcel Dekker Inc.: New York, 1993
4 Schildkraut, J. S. Appl. Phys. Lett. 1991, 58, 340   DOI
5 Borsenberger, P. M.; Ateya, A. I. J. Appl. Phys. 1978, 49, 4035   DOI   ScienceOn
6 Braun, C. L. J. Chem. Phys. 1984, 80, 4157   DOI
7 Goliber, T. E.; Perlstein, J. H. J. Chem. Phys. 1984, 80, 4162   DOI
8 Cimrova V.; Nespurek, A. Chem. Phys. 1994, 184, 283   DOI   ScienceOn
9 Lin, L..B.; Jenekhe, S. A.; Borsenberger, P. M. J. Chem. Phys. 1996, 105, 8490   DOI   ScienceOn
10 Miyasaka, H.; Moriyama, T.; Ide, T.; Itaya, A. Chem. Phys. Lett. 1988, 292, 339   DOI   ScienceOn
11 Jung, J.; Glowacki, I.; Ulanki, J. J. Chem. Phys. 1999, 110, 7000   DOI   ScienceOn
12 Albrecht, U.; Bassler, H. Chem. Phys. Lett. 1995, 235, 389   DOI   ScienceOn
13 Glowacki, I.; Jung, J.; Ulanski, J. Synth. Met. 2000, 109, 143.   DOI   ScienceOn
14 Onsager, L. J. Chem. Phys. 1934, 2, 599   DOI
15 Onsager, L. Phys. Rev. 1938, 54, 554   DOI
16 Barth, S.; Herter, D.; Tak, Y.-H.; Bassler, H.; Horhold, H. H. Chem. Phys. Lett. 1997, 274, 165   DOI   ScienceOn
17 Pasveer, W. F.; Cottaar, J.; Tanase, C.; Coehoom, R.; Bobbert, P. A.; Blom, P. W. M.; Leeuw, D. M. de; Michels, M. A. J. Phys. Rev. Lett. 2005, 94, 206601   DOI   ScienceOn
18 Baranovskii, S. D.; Rubel, O.; Thomas, P. Thin Solid Films 2005, 487, 2   DOI   ScienceOn
19 Offermans, T.; Meskers, S. C. J.; Janssen, R. A. J. Chem. Phys. 2005, 308, 125   DOI   ScienceOn
20 Lee, C. J. Bull. Korean Chem. Soc. 2006, 27, 1186   DOI   ScienceOn
21 Lee, C.; Yang, M.; Lee, N..S.; Kim, N. Chem. Phys. Lett. 2006, 418, 54   DOI   ScienceOn
22 Lee, C.; Park, S..K.; Yang, M.; Lee, N..S.; Kim, N. Chem. Phys. Lett. 2006, 422, 106   DOI   ScienceOn
23 Miller, A.; Abrahams, E. Phys. Rev. 1960, 120, 745   DOI
24 Lee, C.; Park, S..K.; Yang, M.; Lee, N..S.; Kim, N. Bull. Korean Chem. Soc. 2007, 28, 447   DOI   ScienceOn
25 Novikov, S. V.; Vannikov, A. V. Synth. Met. 1997, 85, 1167   DOI   ScienceOn
26 Novikov, S. V.; Dunlap, D. H.; Kenkre, V. M.; Pattis, P. E.; Vannikov, A. V. Phys. Rev. Lett. 1998, 81, 4472   DOI
27 Schonherr, G.; Bassler, H.; Silver, M. Phil. Mag. B 1981, 44, 47   DOI
28 Samoc, M.; Willams, D. F. J. Chem. Phys. 1983, 78, 1924   DOI
29 Ito, C.; Kigoshi, S. Phys. Stat. Sol. A 2006, 203, 3774   DOI   ScienceOn
30 Gommans, H. H. P.; Kemerink, M.; Kramer, J. M.; Janssen, R. A. J. Appl. Phys. Lett. 2005, 87, 122104   DOI   ScienceOn
31 Mihailetchi, V. D.; Koster, L. J. A.; Hummelen, J. C.; Blom, P. W. M. Phys. Rev. Lett. 2004, 93, 216601   DOI   ScienceOn
32 Steenwinckel, D. V.; Hendrickx, E.; Persoons, A. J. Chem. Phys. 2001, 114, 9557   DOI   ScienceOn