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http://dx.doi.org/10.5012/bkcs.2003.24.8.1075

Femtosecond Coherent Spectroscopic Study of Zn(II)porphyrin Using Chirped Ultrashort Pulses  

Yoon, Min-Chul (National Creative Research Initiatives Center for Ultrafast Optical Characteristics Control andDepartment of Chemistry, Yonsei University)
Song, Jae-Kyu (National Creative Research Initiatives Center for Ultrafast Optical Characteristics Control andDepartment of Chemistry, Yonsei University)
Cho, Sung (National Creative Research Initiatives Center for Ultrafast Optical Characteristics Control andDepartment of Chemistry, Yonsei University)
Kim, Dong-Ho (National Creative Research Initiatives Center for Ultrafast Optical Characteristics Control andDepartment of Chemistry, Yonsei University)
Publication Information
Bulletin of the Korean Chemical Society / v.24, no.8, 2003 , pp. 1075-1080 More about this Journal
Abstract
We have investigated femtosecond coherent vibrational motions of Zn(II)-5,15-diphenylporphyrin in toluene using chirp-controlled ultrashort pulses. The oscillatory features superimposed on the temporal profiles of the pump-probe transient absorption signal are affected by the chirping and energy of excitation pulses. Using chirp- and excitation energy-controlled femtosecond pulses, we are able to obtain information on the structural changes between the electronic ground and excited states based on a comparative analysis of the Fouriertransformed frequency-domain spectra retrieved from the oscillatory components with the ground state resonance Raman spectra and normal mode calculations.
Keywords
Chirped pulse; Wave packet; Zn(II)porphyrin;
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1 Schere, N. F.; Carlson, R. J.; Matro, A.; Du, M.; Ruggerio, A. J.;Romero-Rochin, V.; Cina, J. A.; Fleming, G. R.; Rice, S. A. J.Chem. Phys. 1991, 95, 1487.   DOI
2 Kobayashi, H.; Kaizu, Y. In Porphyrins: Excited States andDynamics; Gouterman, M.; Rentzepis, P.; Straub, K. D.; ACSSymposium Series 321; American Chemical Socienty: WashingtonDC, 1986; p 105.
3 Rosca, F.; Kumar, A. T. N.; Ye, X.; Sjodin, T.; Demidov, A. A.;Champion, P. M. J. Phys. Chem. A 2000, 104, 4280.   DOI   ScienceOn
4 Saito, T.; Kobayashi, T. J. Phys. Chem. A 2002, 106, 9436.   DOI   ScienceOn
5 Pollard, W. T.; Dexheimer, S. L.; Wang, Q.; Peteanu, L. A.; Shank,C. V.; Mathies, R. A. J. Phys. Chem. 1992, 96, 6147.   DOI
6 Krause, J. L.; Whitnell, R. M.; Wilson, K. R.; Yan, Y. J.;Mukamel, S. J. Chem. Phys. 1993, 99, 6562.   DOI   ScienceOn
7 Lin, V. S.-Y.; DiMagno, S. G.; Therien, M. J. Science 1994, 264,1105.   DOI
8 Bardeen, C. J.; Wang, Q.; Shank, C. J. J. Phys. Chem. A 1998,102, 2759.   DOI   ScienceOn
9 Bardeen, C. J.; Wang, Q.; Shank, C. J. Phys. Rev. Lett. 1995, 75,3410.   DOI   ScienceOn
10 Wasielewski, M. R. Chem. Rev. 1992, 92, 435.   DOI
11 Gouterman, M. In The Porphyrins; Dolphin, D., Ed.; AcademicPress: New York, 1978; Vol. I.
12 Aratani, N.; Osuka, A.; Cho, H. S.; Kim, D. J. Photochem.Photobiol. C 2002, 3, 25.   DOI   ScienceOn
13 Bardeen, C. J.; Che, J.; Wilson, K. R.; Yakovlev, V. V.; Apkarian,V. A.; Martens, C. C.; Zadoyan, R.; Kohler, B.; Messina, M. J.Chem. Phys. 1997, 106, 8486.   DOI   ScienceOn
14 Ye, X.; Demidov, A.; Champion, P. M. J. Am. Chem. Soc. 2002, 124, 5914.   DOI   ScienceOn
15 Yoon, M.-C.; Jeong, D. H.; Cho, S.; Kim, D.; Rhee, H.; Joo, T. J.Chem. Phys. 2003, 118, 164.   DOI   ScienceOn
16 Cho, H. S.; Song, N. W.; Kim, Y. H.; Jeoung, S. C.; Hahn, S.;Kim, D.; Kim, S. K.; Yoshida, N.; Osuka, A. J. Phys. Chem. A2000, 104, 3287.   DOI   ScienceOn
17 Barkhuijsen, H.; de Beer, R.; Bovee, W. M. M. J.; van Ormondt,D. J. Magn. Reson. 1985, 61, 465.
18 Jeong, D. H.; Yoon, M.-C.; Jang, S. M.; Kim, D.; Cho, D. W.;Yoshida, N.; Aratani, N.; Osuka, A. J. Phys. Chem. A 2002, 106,2359.   DOI   ScienceOn
19 Kim, Y. H.; Jeong, D. H.; Kim, D.; Jeoung, S. C.; Cho, H. S.;Kim, S. K.; Aratani, N.; Osuka, A. J. Am. Chem. Soc. 2001, 123,76.   DOI   ScienceOn
20 Averbukh, I.; Shapiro, M. Phys. Rev. A 1993, 47, 5086.   DOI   ScienceOn
21 Misawa, K.; Kobayashi, T. J. Chem. Phys. 2000, 113, 7546.   DOI   ScienceOn
22 Li, X.-Y.; Czernuszewicz, R. S.; Kincaid, J. R.; Su, Y. O.; Spiro, T.G. J. Phys. Chem. 1990, 94, 31.   DOI
23 Mataga, N.; Shibata, Y.; Chosrowjan, H.; Yshida, N.; Osuka, A. J.Phys. Chem. B 2000, 104, 4001.   DOI   ScienceOn
24 Min, C.-K.; Joo, T.; Yoon, M.-C.; Kim, C. M.; Hwang, Y. N.; Kim,D.; Aratani, N.; Yoshida, N.; Osuka, A. J. Chem. Phys. 2001, 114,6750.   DOI   ScienceOn
25 Martin, R. E.; Diederich, F. Angew. Chem. Int. Ed. Engl. 1999, 38,1350.   DOI   ScienceOn
26 Wagner, R. W.; Lindsey, J. S. J. Am. Chem. Soc. 1994, 116, 9759.   DOI   ScienceOn
27 Aratani, N.; Osuka, A.; Kim, Y. H.; Jeong, D. H.; Kim, D. Angew.Chem. Int. Ed. Engl. 2000, 39, 1458.   DOI   ScienceOn
28 Albrecht, A. C. J. Chem. Phys. 1961, 34, 1476.   DOI
29 Szintay, G.; Horvth, A. Inorg. Chim. Acta 2000, 310, 175.   DOI   ScienceOn