[KSCI] Korea Science Citation Index Service

http://dx.doi.org/10.5857/RCP.2014.3.4.67

DNA Length Dependent Photocurrent of Diketopyrrolopyrrole Aggregates Constructed with DNA

Nakamura, Mitsunobu (Department of Materials Science and Chemistry, University of Hyogo)
Tsuto, Koji (Department of Materials Science and Chemistry, University of Hyogo)
Takada, Tadao (Department of Materials Science and Chemistry, University of Hyogo)
Yamana, Kazushige (Department of Materials Science and Chemistry, University of Hyogo)

Publication Information

Rapid Communication in Photoscience / v.3, no.4, 2014 , pp. 67-69 More about this Journal

Abstract

Bis(2-thienyl)-diketopyrrolopyrrole having two $Zn^{II}$ -cylcens (DPPCy) was synthesized. DPP-aggregates were constructed by self-organization of DPPCy and $dT_n$ -DNAs. In the presence of L-ascorbic acid as an electron sacrifice reagent, the DPP aggregates immobilized on a gold electrode exhibit good anodic photocurrent responses as well as cathodic photocurrent responses in the presence of methyl viologen. The anodic photocurrent responses depend on the DNA lengths because of the formation of uniform DPP-aggregates corresponding to the DNA lengths. The present results show that photocurrent responses of the DPP-aggregates can be controlled by DNA lengths and electron sacrifice reagents.

Keywords

Diketopyrrolopyrrole; DNA; Self-organization; Dye aggregates; Photocurrent;

Citations & Related Records

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