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http://dx.doi.org/10.4491/eer.2013.18.3.169

Temporal Characteristics of Volatile Organic Compounds in Newly-Constructed Residential Buildings: Concentration and Source  

Shin, Seung-Ho (Department of Environmental Engineering, Kyungpook National University)
Jo, Wan-Kuen (Department of Environmental Engineering, Kyungpook National University)
Publication Information
Environmental Engineering Research / v.18, no.3, 2013 , pp. 169-176 More about this Journal
Abstract
The present study was designed to examine the concentrations, emission rates, and source characteristics of a variety of volatile organic compounds (VOCs) in 30 newly-constructed apartment buildings by measuring indoor and outdoor VOC concentrations over a 2-year period. For comparison, seven villa-type houses were also surveyed for indoor and outdoor VOC concentrations over a 3-month period. Indoor and outdoor air samples were collected on Tenax-TA adsorbent and analyzed using a gas chromatograph (GC)/mass spectrometer system or a GC/flame ionization detector system coupled to a thermal desorption system. The long-term change in indoor VOC concentrations depended on the type of VOCs. Generally, aromatic (except for naphthalene), aliphatic, and terpene compounds exhibited a gradual deceasing trend over the 2-year follow-up period. However, the indoor concentrations of the six halogenated VOCs did not significantly vary with time changes. Similar to these halogenated VOCs, the indoor naphthalene concentrations did not vary significantly with time changes over the 2-year period. Unlike the halogenated VOCs, the indoor naphthalene concentrations were much higher than the outdoor concentrations. The indoor concentrations of aliphatic and aromatic compounds were higher for the villa-type houses when compared to those of apartment buildings. In addition, four source groups (floor coverings and interior painting, household products, wood paneling and furniture, moth repellents) and three source groups (floor coverings and interior painting, household products, and moth repellents) were considered as potential VOC sources inside apartment buildings for the first- and second-year post-occupancy stages, respectively.
Keywords
Apartment building; Follow-up period; Source characteristic; Villa-type house;
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1 Li A, Schoonover TM, Zou Q, et al. Polycyclic aromatic hydrocarbons in residential air of ten Chicago area homes: concentrations and influencing factors. Atmos. Environ. 2005;39:3491-3501.   DOI   ScienceOn
2 Lu R, Wu J, Turco RP, et al. Naphthalene distributions and human exposure in Southern California. Atmos. Environ. 2005;39:489-507.   DOI   ScienceOn
3 Zuraimi MS, Tham KW, Sekhar SC. A study on the identification and quantification of sources of VOCs in 5 airconditioned Singapore office buildings. Build. Environ. 2004;39:165-177.   DOI   ScienceOn
4 Zhu J, Cao XL, Beauchamp R. Determination of 2-butoxyethanol emissions from selected consumer products and its application in assessment of inhalation exposure associated with cleaning tasks. Environ. Int. 2001;26:589-597.   DOI   ScienceOn
5 Kwon KD, Jo WK, Lim HJ, Jeong WS. Characterization of emissions composition for selected household products available in Korea. J. Hazard. Mater. 2007;148:192-198.   DOI   ScienceOn
6 Theloke J, Friedrich R. Compilation of a database on the composition of anthropogenic VOC emissions for atmospheric modeling in Europe. Atmos. Environ. 2007;41:4148-4160.   DOI   ScienceOn
7 Wilke O, Jann O, Brodner D. VOC- and SVOC-emissions from adhesives, floor coverings and complete floor structures. Indoor Air 2004;14 Suppl 8:98-107.   DOI   ScienceOn
8 Yuan B, Shao M, Lu S, Wang B. Source profiles of volatile organic compounds associated with solvent use in Beijing, China. Atmos. Environ. 2010;44:1919-1926.   DOI   ScienceOn
9 Guo H. Source apportionment of volatile organic compounds in Hong Kong homes. Build. Environ. 2011;46:2280-2286.   DOI   ScienceOn
10 Hutter HP, Moshammer H, Wallner P, Damberger B, Tappler P, Kundi M. Health complaints and annoyances after moving into a new office building: a multidisciplinary approach including analysis of questionnaires, air and house dust samples. Int. J. Hyg. Environ. Health 2006;209:65-68.   DOI   ScienceOn
11 Mendell MJ. Indoor residential chemical emissions as risk factors for respiratory and allergic effects in children: a review. Indoor Air 2007;17:259-277.   DOI   ScienceOn
12 Rumchev K, Brown H, Spickett J. Volatile organic compounds: do they present a risk to our health? Rev. Environ. Health 2007;22:39-55.
13 Brinkman GL, Milford JB, Schauer JJ, Shafer MM, Hannigan MP. Source identification of personal exposure to fine particulate matter using organic tracers. Atmos. Environ. 2009;43:1972-1981.   DOI   ScienceOn
14 Leuchner M, Rappengluck B. VOC source-receptor relationships in Houston during TexAQS-II. Atmos. Environ. 2010;44:4056-4067.   DOI   ScienceOn
15 Perez-Rial D, Lopez-Mahia P, Tauler R. Investigation of the source composition and temporal distribution of volatile organic compounds (VOCs) in a suburban area of the northwest of Spain using chemometric methods. Atmos. Environ. 2010;44:5122-5132.   DOI   ScienceOn
16 Chiriac R, De Araujos Morais J, Carre J, Bayard R, Chovelon JM, Gourdon R. Study of the VOC emissions from a municipal solid waste storage pilot-scale cell: comparison with biogases from municipal waste landfill site. Waste Manag. 2011;31:2294-2301.   DOI   ScienceOn
17 Vega E, Sanchez-Reyna G, Mora-Perdomo V, et al. Air quality assessment in a highly industrialized area of Mexico: concentrations and sources of volatile organic compounds. Fuel 2011;90:3509-3520.   DOI   ScienceOn
18 Jo WK, Chun HH, Lee SO. Evaluation of atmospheric volatile organic compound characteristics in specific areas in Korea using long-term monitoring data. Environ. Eng. Res. 2012;17:103-110.   DOI   ScienceOn
19 California Environmental Protection Agency, Office of Environmental Health Hazard Assessment. Air toxics hot spots program risk assessment guidelines. Part II: Technical support document for describing available cancer potency factors. Sacramento: California Environmental Protection Agency, Office of Environmental Health Hazard Assessment; 2005.
20 Wang J, Jin L, Gao J, et al. Investigation of speciated VOC in gasoline vehicular exhaust under ECE and EUDC test cycles. Sci. Total Environ. 2013;445-446:110-116.   DOI   ScienceOn
21 US Environmental Protection Agency. Integrated Risk Information System (IRIS) [Internet]. Washington: US Environmental Protection Agency; c2013 [cited 2013 Jul 15]. Available from: http://www.epa.gov/IRIS/index.html.
22 Hodgson AT, Rudd AF, Beal D, Chandra S. Volatile organic compound concentrations and emission rates in new manufactured and site-built houses. Indoor Air 2000;10:178-192.   DOI   ScienceOn
23 Jarnstrom H, Saarela K, Kalliokoski P, Pasanen AL. Reference values for indoor air pollutant concentrations in new, residential buildings in Finland. Atmos. Environ. 2006;40:7178-7191.   DOI   ScienceOn
24 Park JS, Ikeda K. Variations of formaldehyde and VOC levels during 3 years in new and older homes. Indoor Air 2006;16:129-135.   DOI   ScienceOn
25 Lim S, Lee K, Seo S, Jang S. Impact of regulation on indoor volatile organic compounds in new unoccupied apartment in Korea. Atmos. Environ. 2011;45:1994-2000.   DOI   ScienceOn
26 Smith GB, Aguilar JL, Gentle AR, Chen D. Multi-parameter sensitivity analysis: a design methodology applied to energy efficiency in temperate climate houses. Energy Build. 2012;55:668-673.   DOI   ScienceOn
27 Chino S, Kato S, Seo J, Ataka Y. Study on emission of decomposed chemicals of esters contained in PVC flooring and adhesive. Build. Environ. 2009;44:1337-1342.   DOI   ScienceOn
28 Sarigiannis DA, Karakitsios SP, Gotti A, Liakos IL, Katsoyiannis A. Exposure to major volatile organic compounds and carbonyls in European indoor environments and associated health risk. Environ. Int. 2011;37:743-765.   DOI   ScienceOn
29 Nicolle J, Desauziers V, Mocho P, Ramalho O. Optimization of FLEC-SPME for field passive sampling of VOCs emitted from solid building materials. Talanta 2009;80:730-737.   DOI   ScienceOn
30 Shinohara N, Kai Y, Mizukoshi A, et al. On-site passive flux sampler measurement of emission rates of carbonyls and VOCs from multiple indoor sources. Build. Environ. 2009;44:859-863.   DOI   ScienceOn
31 World Health Organization, Regional Office for Europe. Air quality guidelines for Europe. Copenhagen: World Health Organization; 2000.
32 International Agency for Research on Cancer. Agents classified by the IARC monographs, volumes 1-108 [Internet]. Lyon: International Agency for Research on Cancer; c2013 [cited 2013 Jul 15]. Available from: http://monographs.iarc. fr/ENG/Classification/ClassificationsAlphaOrder.pdf.
33 Ramirez N, Cuadras A, Rovira E, Borrull F, Marce RM. Chronic risk assessment of exposure to volatile organic compounds in the atmosphere near the largest Mediterranean industrial site. Environ. Int. 2012;39:200-209.   DOI   ScienceOn
34 Su FC, Jia C, Batterman S. Extreme value analyses of VOC exposures and risks: a comparison of RIOPA and NHANES datasets. Atmos. Environ. 2012;62:97-106.   DOI   ScienceOn
35 Jia C, D'Souza J, Batterman S. Distributions of personal VOC exposures: a population-based analysis. Environ. Int. 2008;34:922-931.   DOI   ScienceOn
36 Han KH, Zhang JS, Wargocki P, Knudsen HN, Varshney PK, Guo B. Model-based approach to account for the variation of primary VOC emissions over time in the identification of indoor VOC sources. Build. Environ. 2012;57:403-416.   DOI   ScienceOn
37 Brown SK. Volatile organic pollutants in new and established buildings in Melbourne, Australia. Indoor Air 2002;12:55-63.   DOI   ScienceOn
38 Jarnstrom H, Saarela K, Kalliokoski P, Pasanen AL. Reference values for structure emissions measured on site in new residential buildings in Finland. Atmos. Environ. 2007;41:2290-2302.   DOI   ScienceOn