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http://dx.doi.org/10.1016/j.jiec.2018.08.004

Catalytic effect of metal oxides on CO2 absorption in an aqueous potassium salt of lysine  

Dharmalingam, Sivanesan (Greenhouse Gas Laboratory, Korea Institute of Energy Research)
Park, Ki Tae (Greenhouse Gas Laboratory, Korea Institute of Energy Research)
Lee, Ju-Yeol (ANYTECH Co., Ltd.)
Park, Il-Gun (PYUNGHWA Engineering Consultants Ltd.)
Jeong, Soon Kwan (Greenhouse Gas Laboratory, Korea Institute of Energy Research)
Publication Information
Journal of Industrial and Engineering Chemistry / v.68, no., 2018 , pp. 335-341 More about this Journal
Abstract
We report the catalytic effects of metal oxides on the $CO_2$ absorption rate in an aqueous potassium salt of ${\text\tiny{L}}-lysine-HCl$ using the vapor liquid equilibrium method. The best $CO_2$ absorption rate obtained through testing metal oxides in a highly concentrated potassium salt of amino acids (2.0 M) was identified using CuO. The recyclability of the metal oxides was tested over three cycles. The catalyst CuO was found to enhance the absorption rate of $CO_2$ by 61%. A possible mechanism was proposed based on NMR spectroscopy studies. Further, the effect of change in liquid absorbent viscosity on $CO_2$ absorption is discussed.
Keywords
$CO_2$ absorption; Catalytic effect; Metal Oxides; Aqueous amino acid salt; ${\text\tiny{L}}-Lysine$ potassium salt; Mechanistic studies;
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