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http://dx.doi.org/10.1016/j.jiec.2018.07.019

Carbon bead-supported copper-dispersed carbon nanofibers: An efficient catalyst for wet air oxidation of industrial wastewater in a recycle flow reactor  

Yadav, Ashish (Department of Chemical Engineering, Indian Institute of Technology Kanpur)
Verma, Nishith (Department of Chemical Engineering, Indian Institute of Technology Kanpur)
Publication Information
Journal of Industrial and Engineering Chemistry / v.67, no., 2018 , pp. 448-460 More about this Journal
Abstract
Copper nanoparticle-doped and graphitic carbon nanofibers-covered porous carbon beads were used as an efficient catalyst for treating synthetic phenolic water by catalytic wet air oxidation (CWAO) in a packed bed reactor over 10-30 bar and $180-230^{\circ}C$, with air and water flowing co-currently. A mathematical model based on reaction kinetics assuming degradation in both heterogeneous and homogeneous phases was developed to predict reduction in chemical oxygen demand (COD) under a continuous operation with recycle. The catalyst and process also showed complete COD reduction (>99%) without leaching of Cu against a high COD (~120,000 mg/L) containing industrial wastewater.
Keywords
Catalytic wet air oxidation; Kinetic model; Recycle reactor; Carbon nanofibers; Copper nanoparticle;
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1 S. Hocevar, U.O. Krasovec, B. Orel, A.S. Arico, H. Kim, Appl. Catal. B: Environ. 28 (2000) 113.   DOI
2 F. Arena, C. Italiano, A. Raneri, C. Saja, Appl. Catal. B: Environ. 99 (2010) 321.   DOI
3 T.D. Burchell, Carbon Materials for Advanced Technologies, Pergamon, Elsevier Science Ltd., Oxford, UK, 1999.
4 R.S. Ruoff, D.C. Lorents, in: M.E.I.S. Dresselhaus (Ed.), Carbon Nanotubes, Pergamon, Oxford, UK, 1996.
5 C. Wang, M. Zhao, J. Li, J. Yu, S. Sun, S. Ge, X. Guo, F. Xie, B. Jiang, E.K. Wujcik, Y. Huang, N. Wang, Z. Guo, Polymer 131 (2017) 263.   DOI
6 Y. He, S. Yang, H. Liu, Q. Shao, Q. Chen, C. Lu, Y. Jiang, C. Liu, Z. Guo, J. Colloid Interface Sci. 517 (2018) 40.   DOI
7 L. Zhang, W. Yu, C. Han, J. Guo, Q. Zhang, H. Xie, Q. Shao, Z. Sun, Z. Guo, J. Electrochem. Soc. 164 (2017) H651.   DOI
8 B. Song, T. Wang, H. Sun, Q. Shao, J. Zhao, K. Song, L. Hao, L. Wang, Z. Guo, Dalton Trans. 46 (2017) 15769.   DOI
9 Y. Li, B. Zhou, G. Zheng, X. Liu, T. Li, C. Yan, C. Cheng, K. Dai, C. Liu, C. Shen, Z. Guo, J. Mater. Chem. C 6 (2018) 2258.   DOI
10 H. Liu, Y. Li, K. Dai, G. Zheng, C. Liu, C. Shen, X. Yan, J. Guo, Z. Guo, J. Mater. Chem. C 4 (2016) 157.   DOI
11 F. Arena, E. Alongi, P. Famulari, A. Parmaliana, G. Trunfio, Catal. Lett.107 (2006) 39.   DOI
12 H. Liu, W. Huang, X. Yang, K. Dai, G. Zheng, C. Liu, C. Shen, X. Yan, J. Guo, Z. Guo, J. Mater. Chem. C 4 (2016) 4459.   DOI
13 Q. Luo, H. Ma, F. Hao, Q. Hou, J. Ren, L. Wu, Z. Yao, Y. Zhou, N. Wang, K. Jiang, H. Lin, Z. Guo, Adv. Funct. Mater. 27 (2017) 1703068.   DOI
14 F. Stuber, I. Polaert, H. Delmas, J. Font, A. Fortuny, A. Fabregat, J. Chem. Technol. Biotechnol. 76 (2001) 743.   DOI
15 B. Erjavec, R. Kaplan, P. Djinovic, A. Pintar, Appl. Catal. B: Environ. 132-133 (2013) 342.   DOI
16 D.F.M. Santos, O.S.G.P. Soares, A.M.T. Silva, J.L. Figueiredo, M.F.R. Pereira, Appl. Catal. B: Environ. 199 (2016) 361.   DOI
17 A. Fortuny, C. Bengoa, J. Font, F. Castells, A. Fabregat, Catal. Today 53 (1999) 107.   DOI
18 A. Pintar, M. Besson, P. Gallezot, Appl. Catal. B: Environ. 31 (2001) 275.   DOI
19 A. Vallet, G. Ovejeroa, A. Rodrigueza, J.A. Peres, J. Garciaa, J. Hazard. Mater. 244-245 (2013) 46.   DOI
20 P.M. Alvarez, D. McLurgh, P. Plucinski, Ind. Eng. Chem. Res. 41 (2002) 2147.   DOI
21 R.R. Zapico, P. Marin, F.V. Diez, S. Ordonez, Chem. Eng. J. 270 (2015) 122.   DOI
22 A. Santos, P. Yustos, B. Durban, F. Garcia-Ochoa, Ind. Eng. Chem. Res. 40 (2001) 2773.   DOI
23 J. Guo, M. Al-Dahhan, Ind. Eng. Chem. Res. 42 (2003) 5473.   DOI
24 S. Yang, W. Zhu, J. Wang, Z. Chen, J. Hazard. Mater. 153 (2008) 1248.   DOI
25 A. Pintar, J. Levec, Ind. Eng. Chem. Res. 33 (1994) 3070.   DOI
26 Y. Oshima, K. Tomita, S. Koda, Ind. Eng. Chem. Res. 38 (1999) 4183.   DOI
27 S. Nousir, S. Keav, J. Barbier, M. Bensitel, R. Brahmi, D. Duprez, Appl. Catal. B: Environ. 84 (2008) 723.   DOI
28 F. Stuber, K.M. Smith, M.B. Mendoza, R.R.N. Marques, A. Fabregat, C. Bengoa, J. Font, A. Fortuny, S. Pullket, G.D. Fowler, N.J.D. Graham, Appl. Catal. B: Environ. 110 (2011) 81.   DOI
29 F. Arena, R.D. Chio, B. Gumina, L. Spadaro, G. Trunfio, Inorg. Chim. Acta 431 (2015) 101.   DOI
30 S. Keav, A. Martin, J. Barbier, D. Duprez, Catal. Today 151 (2010) 143.   DOI
31 E. Castillejos-Lopez, A. Maroto-Valiente, D.M. Nevskaia, V. Munoz, I. Rodriguez-Ramos, A. Guerrero-Ruiz, Catal. Today 143 (2009) 355.   DOI
32 P.D. Vaidya, V.V. Mahajani, Chem. Eng. J. 87 (2002) 403.   DOI
33 L. Oliviero, J. Barbier, D. Duprez, A. Guerrero-Ruiz, B. Bachiller-Baeza, I. Rodriguez-Ramos, Appl. Catal. B: Environ. 25 (2000) 267.   DOI
34 E. Szabados, D.F. Sranko, F. Somodi, B. Maroti, S. Kemeny, A. Tungler, J. Ind. Eng. Chem. 34 (2016) 405.   DOI
35 S. Chaliha, K.G. Bhattacharyya, Chem. Eng. J. 139 (2008) 575.   DOI
36 B.L. Yadav, A. Garg, Chem. Eng. J. 252 (2014) 185.   DOI
37 G. Ovejero, A. Rodriguez, A. Vallet, J. Garcia, Chem. Eng. J. 215-216 (2013) 168.   DOI
38 S.K. Kim, S.K. Ihm, Ind. Eng. Chem. Res. 41 (2002) 1967.   DOI
39 S.K. Kim, S.K. Ihm, Top. Catal. 33 (2005) 171.   DOI
40 F. Arena, R. Giovenco, T. Torre, A. Venuto, A. Parmaliana, Appl. Catal. B: Environ. 45 (2003) 51.   DOI
41 S. Hocevar, U.O. Krasovec, B. Orel, A.S. Arico, H. Kim, Appl. Catal. B: Environ. 28 (2000) 113.   DOI
42 D. Posada, P. Betancourt, F. Liendo, J.L. Brito, Catal. Lett. 106 (2006) 81.   DOI
43 H. Zhao, W. Deng, Y. Li, Adv. Compos. Hybrid Mater. 1 (2018) 404.   DOI
44 K. Srinivasarao, P. Mohanbabu, P.K. Mukhopadhyay, Adv. Compos. Hybrid Mater. 1 (2018) 364.   DOI
45 J. Barbier, L. Oliviero, B. Renard, D. Duprez, Top. Catal. 33 (2005) 77.   DOI
46 K.-H. Kim, S.-K. Ihm, J. Hazard. Mater. 186 (2011) 16.   DOI
47 A. Pintar, J. Batista, T. Tisler, Appl. Catal. B: Environ. 84 (2008) 30.   DOI
48 J. Guo, M. Al-Dahhan, Chem. Eng. Sci. 60 (2005) 735.   DOI
49 Z.P.G. Masende, B.F.M. Kuster, K.J. Ptasinski, F. Janssen, J.H.Y. Katima, J.C. Schouten, Top. Catal. 33 (2005) 87.   DOI
50 E. Szabados, G. Sagi, F. Somodi, B. Maroti, D. Sranko, A. Tungler, J. Ind. Eng. Chem. 46 (2017) 364.   DOI
51 APHA, Standard Methods for the Examination of Water and Wastewater, American Public Health Association, Washington DC, 2005.
52 Y. Guo, G. Xu, X. Yang, K. Ruan, T. Ma, Q. Zhang, J. Gu, Y. Wu, H. Liu, Z. Guo, J. Mater. Chem. C 6 (2018) 3004.   DOI
53 A. Yadav, A.K. Teja, N. Verma, J. Environ. Chem. Eng. 4 (2016) 1504.   DOI
54 S. Mishra, N. Verma, J. Ind. Eng. Chem. 36 (2016) 346.   DOI
55 C. Kaweeteerawat, A. Ivask, R. Liu, H. Zhang, C.H. Chang, C. Low-Kam, et al., Environ. Sci. Technol. 49 (2015) 1105.   DOI
56 B. Bhaduri, N. Verma, J. Colloid Interface Sci. 457 (2015) 62.   DOI
57 S. Lim, S.H. Yoon, Y. Shimizu, H. Jung, I. Mochida, Langmuir 20 (2004) 5559.   DOI
58 Y.N. Prajapati, B. Bhaduri, H.C. Joshi, A. Srivastava, N. Verma, Chemosphere 155 (2016) 62.   DOI
59 A.F.J. Santiago, J.F. Sousa, R.C. Guedes, C.E.M. Jeronimo, M. Benachour, J. Hazard. Mater. B 38 (2006) 325.
60 S. Yang, X. Li, W. Zhu, J. Wang, C. Descorme, Carbon 46 (2008) 445.   DOI
61 R.M. Singhal, A. Sharma, N. Verma, Ind. Eng. Chem. Res. 47 (2008) 3700.   DOI
62 M. Abecassis-Wolfovich, M.V. Landau, A. Brenner, M. Herskowitz, Ind. Eng. Chem. Res. 43 (2004) 5089.   DOI
63 S. Keav, A. Martin, J. Barbier, D. Duprez, C. R. Chim. 13 (2010) 508.   DOI
64 A. Pintar, J. Levec, J. Catal. 135 (1992) 345.   DOI
65 Z.P.G. Masende, B.F.M. Kuster, K.J. Ptasinski, F. Janssen, J.H.Y. Katima, J.C. Schouten, Catal. Today 79-80 (2003) 357.   DOI