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http://dx.doi.org/10.1016/j.jiec.2018.03.017

Improved photoelectric performance via fabricated heterojunction g-C3N4/TiO2/HNTs loaded photocatalysts for photodegradation of ciprofloxacin  

Wu, Dongyao (Institute of Green Chemistry and Chemical Technology, School of Chemistry & Chemical Engineering, Jiangsu University)
Li, Jinze (Institute of Green Chemistry and Chemical Technology, School of Chemistry & Chemical Engineering, Jiangsu University)
Guan, Jingru (Institute of Green Chemistry and Chemical Technology, School of Chemistry & Chemical Engineering, Jiangsu University)
Liu, Chongyang (Institute of Green Chemistry and Chemical Technology, School of Chemistry & Chemical Engineering, Jiangsu University)
Zhao, Xiaoxu (Institute of Green Chemistry and Chemical Technology, School of Chemistry & Chemical Engineering, Jiangsu University)
Zhu, Zhi (Institute of Green Chemistry and Chemical Technology, School of Chemistry & Chemical Engineering, Jiangsu University)
Ma, Changchang (School of Environment, Jiangsu University)
Huo, Pengwei (Institute of Green Chemistry and Chemical Technology, School of Chemistry & Chemical Engineering, Jiangsu University)
Li, Chunxiang (Institute of Green Chemistry and Chemical Technology, School of Chemistry & Chemical Engineering, Jiangsu University)
Yan, Yongsheng (Institute of Green Chemistry and Chemical Technology, School of Chemistry & Chemical Engineering, Jiangsu University)
Publication Information
Journal of Industrial and Engineering Chemistry / v.64, no., 2018 , pp. 206-218 More about this Journal
Abstract
An Intercalated heterostructural $g-C_3N_4/TiO_2/HNTs$ supported photocatalyst was successfully prepared via sol-gel and calcination methods. The introduction of HNTs and the $g-C_3N_4-TiO_2$ heterojunction effectively enhanced the charge transfer and separation efficiency of photogenerated electron-hole pairs, which endued the $g-C_3N_4/TiO_2/HNTs$ hybrid material with an outstanding photoelectric performance and good stability. And an obviously enhanced photocatalytic activity was exhibited by photodegrading ciprofloxacin compared with pure $TiO_2$. Furthermore, the main active species were detected through trapping experiment and ESR spin-trap technique with DMPO, which confirmed that the $^{\bullet}O_2{^-}$ and the $h^+$ were the main active species in the photocatalytic system.
Keywords
$TiO_2$; $g-C_3N_4$; Halloysite nanotubes; Heterojunction; Photocatalytic;
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