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http://dx.doi.org/10.4491/KSEE.2017.39.3.149

Capture and Ocean Storage of Carbon Dioxide Using Alkaline Wastes and Seawater  

Lee, Junghyun (Korea Electric Power Corporation Research Institute)
Park, Misun (Korea Electric Power Corporation Research Institute)
Joo, Jisun (Korea Electric Power Corporation Research Institute)
Gil, Joon-Woo (Korea Electric Power Corporation Research Institute)
Publication Information
Abstract
We investigate the availability of $CO_2$ ocean storage by means of chemical conversion of $CO_2$ to the dissolved inorganic carbon (mainly the bicarbonate ion) in seawater. The accelerated weathering of limestone (AWL) technique, which is accelerating the natural $CO_2$ uptake process through the chemical conversion using limestone and seawater, was proposed as an alternative method for reducing energy-related $CO_2$ emission. The method presented in this paper is slightly different from the AWL method. It involves reacting $CO_2$ with seawater and quicklime obtained from alkaline wastes to produce the bicarbonate-rich solution over 100 times more than seawater, which could be released and diluted into the ocean. The released dense bicarbonate-enriched water mass could subside into the deeper layer because of the density flow, and could be sequestrated stably in the ocean.
Keywords
Carbon Capture; Ocean Storage of Carbon Dioxide; Bicarbonate Ions; Alkaline Wastes; Accelerated Weathering of Limestone;
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  • Reference
1 COP 21 Paris France Sustainable Forum 2015 working with UNEP Home Page, http://www.cop21paris.org (2016).
2 Schleussner, C.-F., Rogelj, J., Schaeffer, M., Lissner, T., Licker, R., Fischer, E. M., Knutti, R., Levermann, A., Fieler, K. and Hare, W., "Science and policy characteristics of the Paris Agreement temperature goal," Nature Clim. Change, advance online publication, DOI:10.1038/NCLIMATE3096(2016).   DOI
3 Jung, Sokhee Philemon, "Practical implementation of microbial fuel cells for bioelectrochemical wastewater treatment," J. Korean Soc. Urban Environ., 13(2), 93-100(2013)
4 Intergovernmental Panel on Climate Change, IPCC Carbon dioxide capture and storage. In: Metz, B., Davidson, O., de Coninck, H. C., Loos, M., Meyer, L. A. (Eds.), IPCC Special Report. Prepared by Working Group III of the Intergovernmental Panel on Climate Change, Cambridge University Press, Cambridge and New York (2005).
5 Caldeira, K. and Rau, G. H., "Accelerating carbonate dissolution to sequester carbon dioxide in the ocean: geochemical implications," Geophys. Res. Lett., 27, 225-228(2005).
6 Rau, G. H., "$CO_2$ mitigation via capture and chemical conversion in seawater," Environ. Sci. Technol., 45, 1088-1092(2011).   DOI
7 Rau, G. H. and Caldeira, K., "Enhanced carbonate dissolution: a means of sequestering waste $CO_2$ as ocean bicarbonate," Energy Convers. Manage., 40, 1803-1813(1999).   DOI
8 Rau, G. H., Knauss, K. G., Langer, W. H. and Caldeira, K., "Reducing energy-related $CO_2$ emissions using accelerated weathering of limestone," Energy, 32, 1471-1477(2007).   DOI
9 Kheshgi, H. S., "Sequestering atmospheric carbon dioxide by increasing ocean alkalinity," Energy, 20, 915-922(1995).   DOI
10 London Protocol and Convention Home Page, http://londonprotocol.imo.org.
11 Millero, Frank J., Chemical Oceanography, CRC Press (2013).
12 Rau, G. H., McLeod, E. L. and Hoegh-Guldberg, O., "The need for new ocean conservation strategies in a high-carbon dioxide world," Nature Clim. Change, 2(10), 720-724(2012).   DOI
13 Chou, W. C., Gong, G. C., Hsieh, P. S., Chang, M. H., Chen, H. Y., Yang, C. Y. and Syu, R. W., "Potential impacts of effluent from accelerated weathering of limestone on seawater carbon chemistry: A case study for the Hoping power plant in northeastern Taiwan," Mar. Chem., 168, 27-36(2015).   DOI
14 Talley, L. D., Tishchenko, P., Luchin, V., Nedashkovskiy, A., Sagalaev, S., Kang, D. J. and Min, D. H., "Atlas of Japan (East) Sea hydrographic properties in summer," Prog. in Oceano., 61(2), 277-348(2004).   DOI
15 Haugan, P. M. and Drange, H., "Sequestration of $CO_2$ in the deep ocean by shallow injection," Nature, 357, 318-320(1992).   DOI