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http://dx.doi.org/10.4491/KSEE.2014.36.5.342

Mineral Carbonation of High Carbon Dioxide Composition Gases Using Wollastonite-distilled Water Suspension  

Song, Haejung (Department of Environmental Engineering, The Catholic University of Korea)
Han, Sang-Jun (Department of Environmental Engineering, The Catholic University of Korea)
Wee, Jung-Ho (Department of Environmental Engineering, The Catholic University of Korea)
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Abstract
The present paper investigates the performance of direct wet mineral carbonation technology to fix carbon dioxide ($CO_2$) from relatively high $CO_2$ concentration feeding gas using wollastonite ($CaSiO_3$)-water (and 0.46 M acetic acid) suspension solution. To minimize the energy consumed on the process, the carbonation in this work is carried out at atmospheric pressure and slightly higher room temperature. As a result, carbon fixation is confirmed on the surface of $CaSiO_3$ after carbonation with wollastonite-water suspension solution and its amount is increased according to the $CO_2$ composition in the feeding gas. The leaching and carbonation ratio of wollastonite-water suspension system obtained from the carbonation with 50% of $CO_2$ composition feeding gas is 13.2% and 10.4%, respectively. On the other hand, the performance of wollastonite-acetic acid in the same condition is 63% for leaching and 1.39% for carbonation.
Keywords
Mineral Carbonation; Wollastonite; Carbon Capture and Storage; Calcium Carbonate; Leaching; Climate Change;
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