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Sonolysis of Trichloroethylene in the Multi Ultrasound Irradiation Reactor  

Lee, Min-Ju (Department of civil & Environmental Engineering, Chung-Ang University)
Oh, Je-Ill (Department of civil & Environmental Engineering, Chung-Ang University)
Publication Information
Journal of Korean Society of Environmental Engineers / v.31, no.10, 2009 , pp. 873-882 More about this Journal
Abstract
Sonolysis of TCE (Trichloroethylene) was performed in 584 kHz rectangular reactor. At first, the effect of acoustic power and aqueous temperature which are both important factors to operate ultrasound system on sonolysis of TCE were examined under one side irradiation condition. First degradation rate constants of TCE and chloride yields were increased with increasing acoustic power from 100 to 300 W. And increasing the aqeuous temperature resulted in the increase of first degradation rate constants of TCE and the decrease of chloride yield. Sonolysis of TCE was performed under multi ultrasound irradiation conditions that total acoustic power of 300 W was distributed according to the number of irradiation sides. First degradation rate constants of TCE followed the order 4 sides > 3 sides > 1 side > 2 sides (parallel) > 2 sides (orthogonal). When comparing the experimental results under parallel and orthogonal irradiation conditions of 2 sides with 300 and 450 W, first degradation rate constants of TCE were similar, while production rate constants of hydrogen peroxide were more higher at parallel conditions compared to orthogonal conditions.
Keywords
Sonolysis; Multi-irradiation; Ultrasound; Pyrolysis; Trichloroethylene;
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1 U. S. Environmental Protection Agency, Technical Background Document to Support 308 Rulemaking Pursuant to the Clean Air ActCSection 112 (g). Ranking of Pollutants with 309 Respect to Hazard to Human Health, EPAB450/3-92-010, Emissions Standards Division, 310 Office of Air Quality Planning and Standards, Research Triangle Park, NC, (1994)
2 Shemer, H., and Narkis, N., 'Trihalomethanes aqueous solutions sono-oxidation,' Water Res. 39, 2704-2710(2005)   DOI   ScienceOn
3 Maezawa, A., Nakadoi, H., Suzuki, K., Furusawa, T., Suzuki, Y., and Uchida, S., 'Treatment of dye wastewater by using photo-catalytic oxidation with sonication,' Ultrason. Sonochem. 14, 615-620(2007)   DOI   ScienceOn
4 Aarthi, T., M. S. Shaama, et al. 'Degradation of Water Soluble Polymers under Combined Ultrasonic and Ultraviolet Radiation,' Ind. Eng. Chem. Res., 46(19): 6204-6210(2007)   DOI   ScienceOn
5 Feng, R., Zhao, Y., Zhu, C., and Mason, T. J., 'Enhancement of ultrasonic cavitation yield by multi-frequency sonication,' Ultrason. Sonochem., 9, 231-236(2002)   DOI   ScienceOn
6 Gogate, P., Mujumdar, S., and Pandit, A. B., 'Sonochemical reactors for waste water treatment: comparison using formic acid degradation as a model reaction,' Adv. Env. Res., 7, 283-299(2003)   DOI   ScienceOn
7 Kormann, C., Bahnemann, D. W., and Hoffman, M. R., 'Photocatalytic production of hydrogen peroxides and organic peroxides in aqueous suspensions of titanium dioxide, zinc oxide, and desert sand,' Environ. Sci. Tech., 22, 798-806(1988)   DOI   ScienceOn
8 F${\i}$nd ${\i}$k, S., $G{\ddot{u}}nd{\ddot{u}}z$, G., and $G{\ddot{u}}nd{\ddot{u}}z$, E., 'Direct sonication of acetic acid in aqueous solutions,' Ultrason. Sonochem., 13, 203-207(2006)   DOI   ScienceOn
9 Neppolian, B., Jung, H., Choi, H., Lee, J. H., and Kang, J., 'Sonolytic degradation of methyl tert-butyl ether: the role of coupled fenton process and persulphate ion,' Water Res., 36, 4699-4708(2002)   DOI   ScienceOn
10 Jiang, Y., Petrier, C., and Waite, T. D., 'Kinetics and mechanisms of ultrasonic degradation of volatile chlorinated aromatics in aqueous solutions,' Ultrason. Sonochem., 9, 317-323(2002)   DOI   ScienceOn
11 Vassilakis, C., Pantidou, A., Psillakis, E., Kalogerakis, N., and Mantzavinos, D., 'Sonolysis of natural phenolic compounds in aqueous solutions: degradation pathways and biodegradability,' Water Res., 38, 3110-3118(2004)   DOI   ScienceOn
12 Jiang, Y., Petrier, C., and Waite, T. D., 'Sonolysis of 4-chlorophenol in aqueous solution: Effects of substrate concentration, aqueous temperature and ultrasonic frequency,' Ultrason. Sonochem., 13, 415-422(2006)   DOI   ScienceOn
13 Emery, R. J., Papadaki, M., Freitas dos Santos, L. M., and Mantzavinos, D., 'Extent of sonochemical degradation and change of toxicity of a pharmaceutical precursor (triphenylphosphine oxide) in water as a function of treatment conditions,' Environ. Int., 31, 207-211(2005)   DOI   ScienceOn
14 Manousaki, E., Psillakis, E., Kalogerakis, N., and Mantzavinos, D., 'Degradation of sodium dodecylbenzene sulfonate in water by ultrasonic irradiation,' Water Res., 38, 3751-3759(2004)   DOI   ScienceOn
15 Suslick, K. S., 'Sonochemistry and Sonoluminescence in Encyclopedia of Physical Science and Technology,' 17, Academic Press, San Diego(2001)
16 Mason, T. J., and Lorimer, J. P., Applied sonochemistry, Wiley-VCH Weinheim.(2002)
17 Destaillats, H., Li, T. W. A., and Hoffman, M. R., 'Applications of ultrasound in NAPL remediation: sonochemical degradation of TCE in aqueous surfactant solutions,' Environ. Sci. Technol., 35, 3019-3024(2001)   DOI   ScienceOn
18 Fischer, C. H., Hart, E. J., and Henglein, A., 'Ultrasonic irradiation of water in the presence of 18, $18O_{2}$: isotope exchange and isotopic distribution of $H_{2}O_{2}$,' J. Phys. Chem., 90, 1954-1956(1986)   DOI
19 Peller, J., Wiest, O., and Kamat, P. V., 'Synergy of combining sonolysis and photocatalysis in the degradation and mineralization of chlorinated aromatic compounds,' Environ. Sci. Technol, 37, 1926-1932(2003)   DOI   ScienceOn
20 Wang, S., Huang, B., Wang, Y., and Liao, L., 'Comparison of enhancement of pentachlorophenol sonolysis at 20kHz by dualfrequency sonication,' Ultrason. Sonochem., 13, 506-510(2006)   DOI   ScienceOn
21 Naddeo, V., Belgiorno, V., and Napoli, R. M. A., 'Behaviour of natural organic mater during ultrasonic irradiation,' Desalination, 210, 175-182(2007)   DOI   ScienceOn
22 Naffrechoux, E., and Chanoux, S., 'Sonochemical and photochemical oxidation of organic matter,' Ultrason. Sonochem., 7, 255-259(2000)   DOI   ScienceOn
23 환경부, '2007년 지하수 측정망 운영 결과 보고', (2008)
24 Liu, H.-L. and Hsieh, C. M., 'Single-transducer dual-frequency ultrasound generation to enhance acoustic cavitation,' Ultrason. Sonochem., 16, 431-438(2009)   DOI   ScienceOn
25 Adewuyi, Y. G., 'Sonochemistry: environmental science and engineering applications,' Ind. Eng. Chem. Res., 40, 4681-4715(2001)   DOI   ScienceOn
26 Kang, J. W., Hung, H. M., Liin, A., and Hoffman, M. R., 'Sonolytic destruction of methyl tert-butyl ether by ultrasonic irradiation: the role of $O_{3},\;H_{2}O_{2}$, frequency, and power density,' Environ. Sci. Technol., 33, 3199-3205(1999)   DOI   ScienceOn
27 Appaw, C., and Adewuyi, Y. G., 'Destruction of carbon disulfide in aqueous solutions by sonochemical oxidation,' J. Hazard. Mater., 90, 237-249(2002)   DOI   ScienceOn
28 Lim, M. H., Kim, S. H., Kim, Y. U., and Khim, J., 'Sonolysis of chlorinated compounds in aqueous solution,' Ultrason. Sonochem., 14, 93-98(2007)   DOI   ScienceOn
29 Kubo, M., Onodera, R., Shibasaki-Kitakawa, N., Tsumoto, K., and Yonemoto, T., 'Kinetics of ultrasonic disinfection of Escherichia coli in the presence of titanium dioxide particles,' Biochem. Prog., 21, 897-901(2005)
30 Neppolian, B., Park, J. S., and Choi, H., 'Effect of Fenton-like oxidation on enhanced oxidative degradation of parachlorobenzoic acid by ultrasonic irradiation,' Ultrason. Sonochem., 11, 273-279(2004)   DOI   ScienceOn
31 Sivakumar, M., Tatake, P. A., and Pandit, A. B., 'Kinetics of pnitrophenol degradation: effect of reaction conditions and cavitational parameters for a multiple frequency system, 'Chem. Eng. J., 85, 327-338(2002)   DOI   ScienceOn