Browse > Article
http://dx.doi.org/10.5916/jkosme.2009.33.3.378

Experimental Study on Characteristics of Synergistic Effect of Fuel Mixing on Number Density and Size of Soot in Ethylene-base Counterflow Diffusion Flames by Laser Techniques  

Choi, Jae-Hyuk (Korean Register of Shipping)
Abstract
The effect of fuel mixing on soot structure with methane, ethane, and propane to ethylene-base counterflow diffusion flames has been investigated by measuring the volume fraction, number density, and particle size of soot by adopting the light extinction/scattering techniques. The experimental result showed that the mixing of ethane and propane in ethylene diffusion flame increased soot volume fraction while the mixing of methane decreased. As compare to the ethylene-base flame, the diameters of soot particles for mixture flames are slightly smaller. While the soot number densities for the mixture flames are much higher. Thus, the increase in the soot volume fraction can be attributed to the appreciably increased soot number density by the fuel mixing.
Keywords
Counterflow; Soot; Laser extinction; Laser scattering; Volume fraction; Number density;
Citations & Related Records
연도 인용수 순위
  • Reference
1 K.C. Oh and H, D. Shin, "The effect of oxygen and carbon dioxide concentration on soot formation in non-premixed flames", Fuel, Vol. 85, pp. 615-624, 2006   DOI   ScienceOn
2 KT. Kang, JY. Hwang, SH. Chung, W. Lee, "Soot zone structure and sooting limit in diffusion flames: comparison of counterflow and Co-flow flames", Combust.Flame, Vol. 109, pp. 266-281, 1997   DOI   ScienceOn
3 S. S. Yoon, S. M. Lee, S. H. Chung, "Effect of mixing methane, ethane, propane, and propene on the synergistic effect of PAH and soot formation in ethylene-base counterflow diffusion flames", Proc. Combust.Inst., Vol. 30, pp. 1417-1424, 2005   DOI   ScienceOn
4 RA. Dobbins, RJ. Santoro, HG. Semerjian ,"Interpretation of optical measurement of soot in flames", Prog. Astronaut. Aeronaut., Vol. 92, pp. 208-237, 1984
5 MP. Bogaard, AD. Buckingham, RK. Pierens, AH. White, "Rayleigh scattering depolarization ratio and molecular polarizability anisotropy for gases." J. Chem. Society, Faraday Transactions, Vol. 74, pp. 3008-3015, 1978   DOI
6 D. Lack, B. Lerner, C. Granier, T. Baynard, E. Lovejoy, P. Massoli, A. R. Ravishankara, and E. Williams, "Light absorbing carbon emissions from commercial shipping", Geophysical. Res. Lett., 35, L13815, doi : 10. 1029 /2008 GL033906, 2008   DOI   ScienceOn
7 RR. Rudder, DR. Bach, "Rayleigh scattering of ruby-laser light bym neutral gases." J The Optical Society of America, Vol. 58, pp. 1260-1266, 1968   DOI
8 JA. Miller and CF. Melius, "Kinetic and thermodynamic issues in the formation of aromatic compounds in flames of aliphatic fuels", Combust. Flame, Vol. 91, pp. 21-39, 1992   DOI   ScienceOn
9 A. D'Anna, A. Violi, A. D'Alessio, "Modeling the rich combustion of aliphatic hydrocarbons", Combust. Flame, Vol. 121, pp. 418-429, 2000   DOI   ScienceOn
10 M.D. Smooke , C.S. Mcenally , LD. Pfefferle , RJ. Hall , MB Colket, "Computational and experimental study of soot formation in a coflow laminar diffusion flame", Combust. Flame, Vol. 117, pp. 117-139, 1999   DOI   ScienceOn
11 B. Zhao, Z. Yang, Z. Li, M.V. Johnston, H. Wang, "Particle size distribution function of incipient soot in laminar premixed ethylene flames: effect of flame temperature", Proc. Combust. Inst., Vol. 30: pp. 1441-1448, 2005   DOI   ScienceOn
12 I. Glassman, "Soot formation in combustion processes", Combust. Inst. Vol. 22, pp. 295-311, 1988   DOI   ScienceOn
13 Y. Hidaka, K. Sato, H. Hoshikawa, T. Nishimori, R. Takahashi, H. Tanaka, K. Inami, N. Ito, "Shock-tube and modeling study of ethane pyrolysis and oxidation", Combust. Flame, Vol. 120, pp. 245-264, 2000   DOI   ScienceOn
14 RA. Dobbins, RJ. Santoro, HG. Semerjian, "Analysis of light scattering form soot using optical cross sections for aggregates." 23rd Proc. Combust. Inst., pp. 1525-1532, 1990
15 CF. Bohren, DR. Huffman, "Absorption and scattering of light by small particles", John Willey & Sons New York, 1983
16 CS. McEnally and LD. Pfefferle "The effects of dimethyl ether and ethanol on benzene and soot formation in ethylene nonpremixed flames", Proc. Combust. Inst., Vol. 31, pp. 603-610, 2007   DOI   ScienceOn
17 NM. Marinov, WJ. Pitz, CK. Westbrook, MJ. Castaldi,SM. Senkan, "Modeling of aromatic and polycyclic aromatic hydrocarbon formation in premixed methane and ethane flames." Combust. Sci. Tech., Vol. 116/117, pp. 211-287, 1996   DOI
18 M. Frenklach, D. W. Clary, C. William, J. R. Gardiner, and E. S. Stephen, "Detailed kinetic modeling of soot formation in shock-tube pyrolysis of acetylene", 20th Proc. Combust. Inst., pp. 887-901, 1984
19 NM. Marinov, MJ. Castaldi, CF. Melius , W. Tsang, "Aromatic and polycyckic aromatic hydrocarbon formation in a premixed propane flame", Combust. Sci. Tech., Vol. 128, pp. 295-342, 1997   DOI   ScienceOn