Observations related to the along-wind dispersion of puffs were collected from 12 field sites and from a wind tunnel experiment and used to test simple similarity relations. Because most of the date made use of concentration time series observation from fixed monitors, the basic observation was t, the standard deviation of the concentration time series. This data also allowed the travel time, t, from the source to the receptor to be estimated, from which the puff advective speed ue, could be determined. The along-wind dispersion coefficient, x, was then assumed to equal tue. The data, which extended over four orders of magnitude, supported the similarity relations t=0.1 t and x=1.8 $u^*$t, where t is the travel time and $u^*$ is the friction velocity. About 50% of the observations were within a factor of two of the predictions based on the similarity relations.