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Heavy Metals in Road Deposited Sediments and Control of Them in Urban Areas: A Review

문헌고찰에 의한 도시 지역 도로퇴적물의 중금속 특성 및 적정 관리방안

  • 김도군 (국립순천대학교 환경공학과)
  • Received : 2022.10.03
  • Accepted : 2022.10.16
  • Published : 2022.10.30

Abstract

Road Deposited Sediment (RDS) is the solids formed from the wear of road, wear of vehicles, exhausts, and the input of the emissions from various sources out of the roads. RDS is seriously polluted by organic matter, nutrients, and metals. RDS plays an important role as the sink and the transport medium of the associated pollutants because RDS can be carried to the adjacent water system via stormwater runoff. In this regard, the heavy metals in RDS were investigated based on the publications. The contents of the metals in RDS were highly variable. The concentration of Cr, Ni, Cu, Fe, Zn, As, Cd, and Pb in urban RDS in various regions was in a range of 3.16-3,410, 1.15-1,382, 20.2-9,069, 2,980-124,853, 81-2,550, 2.3-214, 0.19-21.3, and 15.21-1,125 mg/kg, respectively. The anthropogenic enrichment of the metals in RDS was confirmed by the high concentration of Cu, Zn, Cd, and Pb. The contents of the metals were higher in industrial and traffic areas than in residential areas, while they were generally increased with decreasing particle size. It is believed that this study's results would contribute to quantifying the metals' load via RDS and establishing control strategies.

도로퇴적물(Road Deposited Sediments, RDS)은 도로, 도로 시설물, 자동차 마모와 배가스, 그리고 도로 외부에서의 유입에 의해 형성되어 도로에 축적되는 입자 물질이다. RDS는 유기물, 휘발성 고형물, 영양염류, 각종 금속류 등 다양한 오염물에 고농도로 오염되어 있고, 강우유출수와 함께 주변 수계로 유출되므로, 도시 지역 비점오염물질의 축적과 이동에 중요한 역할을 한다. 이에, 본 연구는 RDS의 중금속 농도를 문헌에 의해 검토하여, 관련 부하저감 대책수립에 도움이 되고자 하였다. 도시지역 RDS의 중금속 농도는 매우 편차가 컸다. Norway, Spain, Australia, UK, Jordan, Turkey, Iran, Angola, Canada, USA, China, Taiwan, Malaysia, Thailand 그리고 India의 도시 지역 RDS의 Cr, Ni, Cu, Fe, Zn, As, Cd, 그리고 Pb 농도는 각각 3.16-3,410, 1.15-1,382, 20.2-9,069, 2980-124,853, 81-2,550, 2.3-214, 0.19-21.3, 그리고 15.21-1,125mg/kg 이었다. 특히, Cu, Fe, Mn, Zn, Cd, 그리고 Pb의 농도가 높아, 인위적 요인에 의한 RDS의 중금속 오염이 확인되었다. RDS의 Cr, Ni, Cu, Zn, Cd, 그리고 Pb 농도는 주거지역이나 공원 등에 비해, 교통지역이나 산업지역에서 높았으며, 입도가 감소함에 따라 중금속 농도가 높아졌다. 본 연구결과는 RDS에 의한 수계의 중금속 부하의 산정과, RDS 제어에 의한 비점오염 저감대책의 수립에 도움이 될 것으로 생각된다.

Keywords

Acknowledgement

순천대학교 교연비 사업에 의하여 연구되었음.

References

  1. 서울특별시(2021), 「2021년 도로 청소 종합계획」, 서울.
  2. Agarwal, A. K., T. Gupta, J. Lukose and A. P. Singh (2015), "Particulate Characterization and Size Distribution in the Exhaust of a Gasoline Homogeneous Charge Compression Ignition Engine", Aerosol and Air Quality Research, 15: 504~516. https://doi.org/10.4209/aaqr.2014.01.0021
  3. Ahmed, F., M. H. Bibi and H. I. Ahmed (2007), "Environmental Assessment of Dhaka City (Bangladesh) based on Trace Metal Contents in Road Dusts", Environmental Geology, 51: 975~985. https://doi.org/10.1007/s00254-006-0367-1
  4. Al-Khashman, O. A. (2007), "The Investigation of Metal Concentrations in Street Dust Samples in Aqaba City", Jordan Environmental Geochemistry Health, 29: 197~207. https://doi.org/10.1007/s10653-006-9065-x
  5. Apeayei E., M. S. Bank and J. D. Spengler (2011), "Distribution of Heavy Metals in Road Dust along an Urban-Rural Gradient in Massachusetts", Atmospheric Environment, 45: 2310~2323. https://doi.org/10.1016/j.atmosenv.2010.11.015
  6. Baum, P., B. Kuch and U. Dittmer (2021), "Adsorption of Metals to Particles in Urban Stormwater Runoff-Does Size Really Matter?", Water (Basel), 13: 309.
  7. Birch, G. F. and A. Scollen (2003), "Heavy Metals in Road Dust, Gully Pots and Park land Soils in a Highly Urbanised Sub-Catchment of Port Jackson, Australia", Australian Journal of Soil Research, 41: 1329~1342. https://doi.org/10.1071/SR02147
  8. Cai, K. and C. Li (2019), "Street Dust Heavy Metal Pollution Source Apportionment and Sustainable Management in a Typical City-Shijiazhuang, China", International Journal of Environmental Research and Public Health, 16: 2625~2639. https://doi.org/10.3390/ijerph16142625
  9. Charlesworth, S. M. and J. A. Lees (1999), "The Distribution of Heavy Metals in Deposited Urban Dusts and Sediments, Coventry, England", Environmental Geochemistry and Health, 21: 97~115. https://doi.org/10.1023/A:1006694400288
  10. Charlesworth, S., M. Everett, R. McCarthy, A. Ordonez and E. De Miguel (2003), "A Comparative Study of Heavy Metal Concentration and Distribution in Deposited Street Dusts in a Large and a Small Urban Area: Birmingham and Coventry, West Midlands, UK", Environment International, 29: 563~573. https://doi.org/10.1016/S0160-4120(03)00015-1
  11. Calvillo, S. J., E. S. Williams and B. W. Brooks, (2015), "Street Dust: Implications for Stormwater and Air Quality, and Environmental Management through Street Sweeping", In Reviews of Environmental Contamination and Toxicology, (ed.) Whitacre, D. M., 233 (71~128), Berlin: Springer.
  12. Crosby, C. J., M. A. Fullen, C. A. Booth and D. E. Searle (2014), "A Dynamic Approach to Urban Road Deposited Sediment Pollution Monitoring (Marylebone Road, London, UK)", Journal of Applied Geophysics, 105: 10~20. https://doi.org/10.1016/j.jappgeo.2014.03.006
  13. De Miguel, E., J. F. Llamas, E. Chacon, T. Berg, S. Larssen, O. Royset and M. Vadset (1997), "Origin and Patterns of Distribution of Trace Elements in Street Dust: Unleaded Petrol and Urban Lead", Atmospheric Environment, 31: 2733~2740. https://doi.org/10.1016/S1352-2310(97)00101-5
  14. Ferreira-Baptista, L. F. and E. De Miguel (2005), "Geochemistry and Risk Assessment of Street Dust in Luanda, Angola: A Tropical Urban Environment", Atmospheric Environment, 39: 4501~4512. https://doi.org/10.1016/j.atmosenv.2005.03.026
  15. Gao, S., X. Wang, H. Li, Y. Kong, J. Chen and Z. Chen (2021), "Heavy Metals in Road-Deposited Sediment and Runoff in Urban and Intercity Expressways", Transportation Safety and Environment, 4: tdab030.
  16. Gunawardana, C., A. Goonetilleke, P. Egodawatta, L. Dawes and S. Kokot (2012), "Source Characterisation of Road Dust based on Chemical and Mineralogical Composition", Chemosphere, 87: 163~170. https://doi.org/10.1016/j.chemosphere.2011.12.012
  17. Herath, D., A, Pitawala and J. Gunatilake (2016), "Heavy Metals in Road Deposited Sediments and Road Dusts of Colombo Capital, Sri Lanka", Journal of the National Science Foundation of Sri Lanka, 44: 193~202. https://doi.org/10.4038/jnsfsr.v44i2.8000
  18. Hwang, C.-C. and C.-H. Weng (2015), "Effects of Rainfall Patterns on Highway Runoff Pollution and Its Control", Water and Environment Journal, 29: 214~220. https://doi.org/10.1111/wej.12109
  19. Jiries, A. (2003), "Vehicular Contamination of Dust in Amman, Jordan", The Environmentalist, 23: 205~210. https://doi.org/10.1023/B:ENVR.0000017390.93161.99
  20. Jeong, H., J. Y. Choi and K. Ra (2020a), "Characteristics of Heavy Metal Pollution in Road Dust from Urban Areas: Comparison by Land Use Types", Journal of Environmental Analysis, Health and Toxicology, 23: 101~111 (in Korean). https://doi.org/10.36278/jeaht.23.2.101
  21. Jeong, H., J. Y. Choi and K. Ra (2020b), "Assessment of Metal Pollution of Road-Deposited Sediments and Marine Sediments Around Gwangyang Bay, Korea", Journal of Korean Society of Oceanography, 25: 42~53 (in Korean).
  22. Joshi, U. M., K. Vijayaraghavan and R. Balasubramanian (2009), "Elemental Composition of Urban Street Dusts and their Dissolution Characteristics in Various Aqueous Media", Chemosphere, 77: 526~533. https://doi.org/10.1016/j.chemosphere.2009.07.043
  23. Kim, D-G., H-M. Kang and S-O Ko (2019), "Reduction of Non-Point Source Contaminants Associated with Road-Deposited Sediments by Sweeping", Environmental Science and Pollution Research, 26: 1192~1207. https://doi.org/10.1007/s11356-017-0192-y
  24. Kim, D. G., K. Jeong and S. O. Ko (2014), "Removal of Road Deposited Sediments by Sweeping and its Contribution to Highway Runoff Quality in Korea", Environmental Technology, 35: 2546-55. https://doi.org/10.1080/09593330.2014.911777
  25. Kim, D. G. and S. O. Ko (2021), "Road-Deposited Sediments Mediating the Transfer of Anthropogenic Organic Matter to Stormwater Runoff", Environmental Geochemistry and Health, 43: 3287~3301. https://doi.org/10.1007/s10653-020-00703-2
  26. Kayhanian, M., A. Singh, C. Suverkropp and S. Borroum (2003), "Impact of Annual Average Daily Traffic on Highway Runoff Pollutant Concentrations", Journal of Environmental Engineering, 129: 975~990. https://doi.org/10.1061/(ASCE)0733-9372(2003)129:11(975)
  27. Kayhanian, M., B. D. Fruchtman, J. S. Gulliver, C., Montanaro, E. Ranieri and S. Wuertz (2012), "Review of Highway Runoff Characteristics: Comparative Analysis and Universal Implications", Water Research, 46: 6609~6624. https://doi.org/10.1016/j.watres.2012.07.026
  28. Kreider, M. L., J. M. Panko, B. L. McAtee, L. I. Sweet and B. L. Finley (2010), "Physical and Chemical Characterization of Tire-Related Particles: Comparison of Particles Generated Using Different Methodologies", Science of the Total Environment, 408: 652~659. https://doi.org/10.1016/j.scitotenv.2009.10.016
  29. Kuo, C. Y., J. Y. Wang, S. H. Chang and M. C. Chen (2009), "Study of Metal Concentrations in the Environment Near Diesel Transport Routes", Atmospheric Environment, 43: 3070~3076. https://doi.org/10.1016/j.atmosenv.2009.03.028
  30. Lau, S. L. and M. K. Stenstrom (2005), "Metals and PAHs Adsorbed to Street Particles", Water Research, 39: 4083~4092. https://doi.org/10.1016/j.watres.2005.08.002
  31. Lee, J., H. Jeong, K. Ra and J. Y. Choi (2020), "Assessment of Particle Size Distribution and Pollution Impact of Heavy Metals in Road-deposited Sediments (RDS) from Shihwa Industrial Complex", Journal of Environmental Impact Assessment, 29: 8~25 (in Korean). https://doi.org/10.14249/EIA.2020.29.1.8
  32. Li, X. D., C. S. Poon and P. S. Liu (2001), "Heavy Metals Contamination of Urban Soils and Street Dusts in Hongkong", Applied Geochemistry, 16: 1361~1368. https://doi.org/10.1016/S0883-2927(01)00045-2
  33. Lu. Xl, L. Wang, K. Lei, J. Huang and Y. Zhai (2009), "Contamination Assessment of Copper, Lead, Zinc, Manganese and Nickel in Street Dust of Baoji, NW China", Journal of Hazardous Materials, 161: 1058~1062. https://doi.org/10.1016/j.jhazmat.2008.04.052
  34. Martinelli, T. J., R. Waschbusch, R. Bannerman and A. Wisner (2002), Pollutant Loadings to Stormwater Run-Off from Expressways: The Impact of a Freeway Sweeping Program, Madison: WISCONSIN DOT.
  35. Ma, Y., McGree, A. Liu, K. Deilami, P. Egodawatta and A. Goonetilleke (2017), "Catchment Scale Assessment of Risk Posed by Traffic Generated Heavy Metals and Polycyclic Aromatic Hydrocarbons", Ecotoxicology and Environmental Safety, 144: 593~600. https://doi.org/10.1016/j.ecoenv.2017.06.073
  36. Mohammed, T., P. Loganathan, A. Kinsela, S. Vigneswaran and J. Kandasamy (2012), "Enrichment, Inter-Relationship, and Fractionation of Heavy Metals in Road-Deposited Sediments of Sydney, Australia", Australian Journal of Soil Research, 50: 229~238. https://doi.org/10.1071/SR12010
  37. Nawrot, N., E, Wojciechowska, S. Rezania, J. Walkusz-Miotk and K. Pazdro (2020), "The Effects of Urban Vehicle Traffic on Heavy Metal Contamination in Road Sweeping Waste and Bottom Sediments of Retention Tanks", Science of The Total Environment, 749: 141511. https://doi.org/10.1016/j.scitotenv.2020.141511
  38. Nguyen, T. C., P. Loganathan, T. V. Nguyen, T. T. N. Pham, J. Kandasamy, M. Wu, R. Naidu and S. Vigneswaran (2015), "Trace Elements in Road-deposited and Waterbed Sediments in Kogarah Bay, Sydney: Enrichment, Sources and Fractionation", Soil Research, 53: 401-411. https://doi.org/10.1071/SR14163
  39. Ordonez, A., J. Loredo, E. De Miguel and S. Charlesworth (2003), "Distribution of Heavy Metals in the Street Dusts and Soils of an Industrial City in Northern Spain", Archives of Environmental Contamination and Toxicology, 44: 160~170. https://doi.org/10.1007/s00244-002-2005-6
  40. Rasmussen, P. E., K. S. Subramanian and B. J. Jessiman (2001), "A Multi-Element Profile of Housedust in Relation to Exterior Dust and Soils in the City of Ottawa, Canada", The Science of the Total Environment, 267: 125~140. https://doi.org/10.1016/S0048-9697(00)00775-0
  41. Robertson, D. J., K. G. Taylor and S. R. Hoon (2003), "Geochemical and Mineral Magnetic Characterization of Urban Sediment Particulates, Manchester, UK", Applied Geochemistry, 18: 269~282. https://doi.org/10.1016/S0883-2927(02)00125-7
  42. Rudnick, R. L. and S. Gao (2003), "Composition of the Continental Crust", In The crust. Treatise on Geochemistry, vol 3, (ed) Rudnick R. L., Elsevier-Pergamon, Oxford, pp. 1~64.
  43. Saeedi, M., Y. L. Loretta and M. Salmanzadeh (2012), "Heavy Metals and Polycyclic Aromatic Hydrocarbons: Pollution and Ecological Risk Assessment in Street Dust of Tehran", Journal of Hazardous Materials, 227, 228: 9~17.
  44. Seattle Public Utilities and Herrera Environmental Consultants (2009), "Seattle Street Sweeping Pilot Study: Monitoring Report".
  45. Sezgin, N., H. K. Ozcan, G. Demir, S. Nemlioglu and C. Bayat (2004), "Determination of Heavy Metal Concentrations in Street Dusts in Istanbul E-5 Highway", Environment International, 29: 979~985. https://doi.org/10.1016/S0160-4120(03)00075-8
  46. Shabanda, I. S., I. B. Koki, K. H. Low, S. M. Zain, S. M. Khor and N. K. A. Bakar (2019), "Daily Exposure to Toxic Metals through Urban Road Dust from Industrial, Commercial, Heavy Traffic and Residential Areas in Petaling Jaya, Malaysia: A Health Risk Assessment", Environmental Science and Pollution Research, 26: 37193~37211. https://doi.org/10.1007/s11356-019-06718-2
  47. Shabbaj, I. I., M. A. Alghmdi, M. Shamy, S. K. Hassan, M. M. Alsharif and M. I. Khoder (2018), "Risk Assessment and Implication of Human Exposure to Road Dust Heavy Metals in Jeddah, Saudi Arabia", International Journal of Environmental Research and Public Health, 15: 36~57.
  48. Shi, G., Z. Chen, C. Bi, L. Wang, J. Teng, Y. Li and S. Xu (2011), "A Comprehensive Study of Health Risk of Potentially Toxic Metals in Urban and Suburban Road Dust in the Most Populated City of China", Atmospheric Environment, 43: 764~771.
  49. Siriwardene, N. R., A. Deletic and T. D. Fletcher (2007), "Clogging of Stormwater Gravel Infiltration Systems and Filters: Insights from a Laboratory Study", Water Research, 41: 1433~1440. https://doi.org/10.1016/j.watres.2006.12.040
  50. Srithawirat, T. and M. T. Latif (2015), "Concentration of Selected Heavy Metals in the Surface Dust of Residential Building in Phitsanulok, Thailand", Environmental Earth Science, 74: 2701~2706. https://doi.org/10.1007/s12665-015-4291-0
  51. Sutherland, R. A. and C. A. Tolosa (2000), "Multi-Element Analysis of Road-Deposited Sediment in an Urban Drainage Basin, Honolulu, Hawaii", Environmental Pollution, 110: 483~495. https://doi.org/10.1016/S0269-7491(99)00311-5
  52. Surayawanshi, P. V., B. S. Rajaram, A. D. Bhanakar and C. V. Charapatirao (2016), "Determining Heavy Metal Contamination of Road Dust in Delhi, India", Atmosfera, 29: 221~234.
  53. Tuzen, M. (2003), "Investigation of Heavy Metal Levels in Street Dust Samples in Tokat, Turkey", Journal of Trace and Microprobe Techniques, 21: 513~521. https://doi.org/10.1081/TMA-120023067
  54. United States Department of Transportation (USDOT) and Federal Highway Administration (FHWA), Eisenhower Interstate Highway System Website. Accessed June 20, 2017. http://www.Fhwa.Dot.Gov/Interstate/Homepage.Cfm.
  55. Wei, B. and L. Yang (2010), "A Review of Heavy Metal Contaminations in Urban Soils, Urban Road Dusts and Agricultural Soils from China", Microchemical Journal, 94: 99~107. https://doi.org/10.1016/j.microc.2009.09.014
  56. Wei, B., F. Jiang, X. Li and S. Mu (2010), "Heavy Metal Induced Ecological Risk in the City of Urumqi, NW China", Environmental Monitoring and Assessment, 160: 33~45. https://doi.org/10.1007/s10661-008-0655-1
  57. Wijeyawardana, P., N. Nanayakkara, C. Gunasekara, A. Karunarathna, D. Law and B. K. Pramanik (2022), "Removal of Cu, Pb and Zn from Stormwater Using an Industrially Manufactured Sawdust and Paddy Husk Derived Biochar", Environmental Technology and Innovation, 28: 102640. https://doi.org/10.1016/j.eti.2022.102640
  58. Yang, J., Y. Teng, L. Song and R. Zuo (2016), "Tracing Sources and Contamination Assessments of Heavy Metals in Road and Foliar Dusts in a Typical Mining City, China", PLOS One, 11: e0168528. https://doi.org/10.1371/journal.pone.0168528
  59. Yuen, J. Q., P. H. Olin, H. S. Lim, S. G. Benner, R. A. Sutherland and A. D. Ziegler (2012), "Accumulation of Potentially Toxic Elements in Road Deposited Sediments in Residential and Light Industrial Neighborhoods of Singapore", Journal of Environmental Management, 101: 151~163.
  60. Zafra, C. A., J. Temprano and I. Tejero (2011), "Distribution of the Concentration of Heavy Metals Associated with the Sediment Particles Accumulated on Road Surface", Environmental Technology, 32: 997~1008. https://doi.org/10.1080/09593330.2010.523436
  61. Zhang, M. K. and H. Wang (2009), "Concentrations and Chemical Forms of Potentially Toxic Metals in Road-Deposited Sediments from Different Zones of Hangzhou, China", Journal of Environmental Sciences, 21: 625~631. https://doi.org/10.1016/S1001-0742(08)62317-7