DOI QR코드

DOI QR Code

Further Electrochemical Degradation of Real Textile Effluent Using PbO2 Electrode

  • Wang, Chao (College of Mechanical and Electrical Engineering, Beijing University of Chemical Technology) ;
  • Tian, Penghao (College of Mechanical and Electrical Engineering, Beijing University of Chemical Technology)
  • Received : 2020.12.24
  • Accepted : 2021.01.20
  • Published : 2021.05.28

Abstract

A commercial PbO2 electrode was adopted as the anode for the electrochemical degradation of the real textile effluent with the initial COD of 56.0 mg L-1 and the stainless steel plate as the cathode. The effect of the initial pH, the electrolyte flow rate and the cell voltage on the COD, the current efficiency and the energy consumption were investigated without the addition of NaCl or Na2SO4. The experimental results illustrated that the PbO2 electrode can reduce the COD of the textile effluent from 56.0 mg L-1 to 26.0 mg L-1 with the current efficiency of 86.1% and the energy consumption of 17.5 kWh kg-1 (per kilogram of degraded COD) under the optimal operating conditions. Therefore PbO2 electrode as the anode was promising to further electrochemically degrade the real textile effluent.

Keywords

Acknowledgement

We thank the Major Science and Technology Program for Water Pollution Control and Treatment (2017ZX07202001) for financial support.

References

  1. J. Ding, C. Zheng, L. Wang, C. Lu, B. Zhang, Y. Chen, X. Zhuang, J. Mater. Chem. A., 2015, 87, 826-838.
  2. J. Rovira, J.L. Domingo, Environ. Res., 2019, 168, 62-69. https://doi.org/10.1016/j.envres.2018.09.027
  3. R. Kiani, F. Mirzaei, F. Ghanbari, R. Feizi, F. Mehdipour, J. Water Process Eng., 2020, 38, 101623. https://doi.org/10.1016/j.jwpe.2020.101623
  4. C.R. Holkar, A.J. Jadhav, D.V. Pinjari, N.M. Mahamuni, A.B. Pandit, J. Environ. Manag., 2016, 182, 351-366. https://doi.org/10.1016/j.jenvman.2016.07.090
  5. S. Samsami, M. Mohamadi, M.H. Sarrafzadeh, E.R. Rene, M. Firoozbahr, Process Saf. Environ. Prot., 2020, 143, 138-163. https://doi.org/10.1016/j.psep.2020.05.034
  6. N. Daneshvar, D. Salari, A.R. Khatac, Photochem. Photobiol. A Chem., 2003, 157(1), 111-116. https://doi.org/10.1016/S1010-6030(03)00015-7
  7. F.C. Moreira, R.A.R. Boaventura, E. Brillas, V.J.P. Vilar, Appl. Catal. B Environ., 2017, 202, 217-261. https://doi.org/10.1016/j.apcatb.2016.08.037
  8. C. Yang, S. Shang, X.Y. Li, Sep. Purif. Technol., 2021, 258, 118035. https://doi.org/10.1016/j.seppur.2020.118035
  9. J. Zhao, C. Zhu, J. Lu, C. Hu, S. Peng, T. Chen, Electrochim. Acta, 2014, 118, 169-175. https://doi.org/10.1016/j.electacta.2013.12.005
  10. S. Garcia-Segura, J.D. Ocon, M.N. Chong, Process Saf. Environ. Prot., 2018, 113, 48-67. https://doi.org/10.1016/j.psep.2017.09.014
  11. W.Y. Kim, D.J. Son, C.Y. Yun, D.G. Kim, D. Chang, Y. Sunwoo, K.H. Hong, J. Electrochem. Sci. Technol., 2017, 8(2), 124-132. https://doi.org/10.5229/JECST.2017.8.2.124
  12. Y. He, H. Lin, Z. Guo, W. Zhang, H. Li, W. Huang, Sep. Purif. Technol., 2019, 212, 802-821. https://doi.org/10.1016/j.seppur.2018.11.056
  13. A.F.T. Auguste, G.C. Quand-Meme, K. Ollo, B. Mohamed, S.S. placide, S. Ibrahima, O. Lassine, J. Electrochem. Sci. Technol., 2016, 7(1), 82-89. https://doi.org/10.5229/JECST.2016.7.1.82
  14. M. Xu, Z. Wang, F. Wang, P. Hong, C. Wang, X. Ouyang, C. Zhu, Y. Wei, Y. Hun, W. Fang, Electrochim. Acta, 2016, 201, 240-250. https://doi.org/10.1016/j.electacta.2016.03.168
  15. Q. Dai, J. Zhou, X. Meng, D. Feng, C. Wu, J. Chen, Chem. Eng. J., 2016, 289, 239-246.
  16. Y. Xia, Q. Dai, J. Chen, J. Electroanal. Chem., 2015, 744, 117-125. https://doi.org/10.1016/j.jelechem.2015.01.021
  17. F. Wei, D. Liao, Y. Lin, C. Hu, J. Ju, Y. Chen, D. Feng, Sep. Purif. Technol., 2021, 258, 118056. https://doi.org/10.1016/j.seppur.2020.118056
  18. M.D. Hossain, C.M. Mustafa, M.M. Islam, J. Electrochem. Sci. Technol., 2017, 8(3), 197-205. https://doi.org/10.5229/JECST.2017.8.3.197
  19. I. Elaissaoui, H. Akrout, S. Grassini, D. Fulginiti, L. Bousselmi, Chemosphere, 2019, 217, 26-34. https://doi.org/10.1016/j.chemosphere.2018.10.161
  20. Y. Xia, Q. Dai, Chemosphere, 2018, 205, 215-222. https://doi.org/10.1016/j.chemosphere.2018.04.103
  21. C. Singaravadivel, M. Vanitha, N. Balasubramanian, J. Electrochem. Sci. Technol., 2012, 3(1), 44-49. https://doi.org/10.5229/JECST.2012.3.1.44
  22. Y. Xia, G. Wang, L. Guo, Q. Dai, X. Ma, Chemosphere, 2020, 241, 125010. https://doi.org/10.1016/j.chemosphere.2019.125010
  23. K. Irikura, N. Bocchi, R.C. Rocha-Filho, S.R. Biaggio, J. Iniesta, V. Montiel, J. Environ. Manag., 2016, 183, 306-313. https://doi.org/10.1016/j.jenvman.2016.08.061
  24. X. Duan, F. Ma, Z. Yuan, L. Chang, X. Jin, J. Taiwan. Inst. Chem. Eng., 2013, 44(1), 95-102. https://doi.org/10.1016/j.jtice.2012.08.009
  25. J.M. Aquino, G.F. Pereira, R.C. Rocha-Filho, N. Bocchi, S.R. Biaggio, J. Hazard. Mater. 2011, 192(3), 1275-1282. https://doi.org/10.1016/j.jhazmat.2011.06.039
  26. G. Liu, H. Zhou, J. Teng, S. You, Chem. Eng. J., 2019, 371, 7-14. https://doi.org/10.1016/j.cej.2019.03.249
  27. M. Santhanam, R. Selvaraj, S. Annamalai, M. Sundaram, Chemosphere, 2017, 186, 1026-1032. https://doi.org/10.1016/j.chemosphere.2017.08.066
  28. J. Chen, Y. Xia, Q. Dai, Electrochim. Acta, 2015, 165, 277-287. https://doi.org/10.1016/j.electacta.2015.02.029
  29. M.R. Samarghandi, A. Dargahi, A. Shabanloo, H.Z. Nasab, Y. Vaziri, A. Ansari, Arab. J. Chem., 2020, 13(8), 6847-6864. https://doi.org/10.1016/j.arabjc.2020.06.038
  30. J.L.D.S. Duarte, L. Meili, J.I. Soletti, C.L.D.P. Zanta, J. Water Process Eng., 2019, 31, 100841. https://doi.org/10.1016/j.jwpe.2019.100841
  31. A. Mukimin, H. Vistanty, N. Zen, Chem. Eng. J., 2015, 259, 430-437. https://doi.org/10.1016/j.cej.2014.08.020
  32. D.H.S. Santos, J.L.S. Duarte, M.G.R. Tavares, M.G. Tavares, L.C. Friedrich, L. Meili, W.R.O. Pimentel, J. Tonholo, C.L.P.S. Zanta, Chem. Eng. Process. Process Intensif., 2020, 153, 107940. https://doi.org/10.1016/j.cep.2020.107940
  33. I.M.S. Pillai, A.K. Gupta, J. Environ. Manag., 2017, 193, 524-531. https://doi.org/10.1016/j.jenvman.2017.02.046
  34. Y.A. Oktem, B. Yuzer, M.I. Aydin, H.E. Okten, S. Meric, H. Selcuk, J. Environ. Manag., 2019, 247, 749-755. https://doi.org/10.1016/j.jenvman.2019.06.114