DOI QR코드

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An Improved Movable 3 photomultiplier (3PM)-γ Coincidence Counter Using Logical Sum of Double Coincidences in β-Channel for Activity Standardization

  • Hwang, Han Yull (Department of Fire Protection & Safety Management, Mokwon University) ;
  • Lee, Jong Man (Center for Ionizing Radiation, Korea Research Institute of Standards and Science)
  • 투고 : 2020.01.08
  • 심사 : 2020.04.16
  • 발행 : 2020.06.30

초록

Background: To improve the measurement accuracy of liquid-scintillation counting for activity standardization, it is necessary to significantly reduce the background caused by thermal noise or after-pulses. We have therefore improved a movable 3 photomultiplier (3PM)-γ coincidence-counting method using the logical sum of three double coincidences for β events. Materials and Methods: We designed a new data-acquisition system in which β events are obtained by counting the logical sum of three double coincidences. The change in β-detection efficiency can be derived by moving three photomultiplier tubes sequentially from the liquid-scintillation vial. The validity of the method was investigated by activity measurement of 134Cs calibrated at the Korea Research Institute of Standards and Science (KRISS) with 4π(PC)β-γ(NaI(Tl)) coincidence counting using a proportional counter (PC) for the β detector. Results and Discussion: Measurements were taken over 14 counting intervals for each liquidscintillation sample by displacing three photomultiplier tubes up to 45 mm from the sample. The dead time in each β- and γ-counting channel was adjusted to be a non-extending type of 20 ㎲. The background ranged about 1.2-3.3 s-1, such that the contributions of thermal noise or after-pulses were negligible. As the β-detection unit was moved away from the sample, the β-detection efficiencies varied between 0.54 and 0.81. The result obtained by the method at the reference date was 396.3 ± 1.7 kBq/g. This is consistent with the KRISS-certified value of 396.0 ± 2.0 kBq/g within the uncertainty range. Conclusion: The movable 3PM-γ method developed in the present work not only succeeded in reducing background counts to negligible levels but enabled β-detection efficiency to be varied by a geometrical method to apply the efficiency extrapolation method. Compared with our earlier work shown in the study of Hwang et al. [2], the measurement accuracy has much improved. Consequently, the method developed in this study is an improved method suitable for activity standardization of β-γ emitters.

키워드

참고문헌

  1. Hwang HY, Kwak SI, Lee HY, Lee JM, Lee KB, Park TS. Development of 3-PM liquid scintillation counting system with geometrical efficiency variation. Appl Radiat Isot. 2004;60:469-473. https://doi.org/10.1016/j.apradiso.2003.11.061
  2. Hwang HY, Sung KS, Lee KB, Lee JM, Park TS. Standardization of radionuclide by ${\beta}(LS)-{\gamma}$ coincidence counting using the geometry-efficiency variation method. Appl Radiat Isot. 2006;64:1119-1123. https://doi.org/10.1016/j.apradiso.2006.02.079
  3. Pochwalski K, Broda R, Radoszewski T. Standardization of pure beta emitters by liquid-scintillation counting. Int J Rad Appl Instrum A. 1988;39:165-172. https://doi.org/10.1016/0883-2889(88)90162-1
  4. Cassette P, Bouchard J. The design of a liquid scintillation counter based on the triple to double coincidence ratio method. Nucl Instrum Methods Phys Res A. 2003;505:72-75. https://doi.org/10.1016/S0168-9002(03)01023-4
  5. Broda R, Cassette P, Kossert K. Radionuclide metrology using liquid scintillation counting. Metrologia. 2007;44:S36-S52. https://doi.org/10.1088/0026-1394/44/4/S06
  6. Bobin Ch, Bouchard J. A $4{\pi}(LS){\beta}-{\gamma}$ coincidence system using a TDCR apparatus in the beta-channel. Appl Radiat Isot. 2006;64:124-130. https://doi.org/10.1016/j.apradiso.2005.06.008
  7. Johansson LC, Sephton JP. Validation of a new TDCR system at NPL. Appl Radiat Isot. 2010;68:1537-1539. https://doi.org/10.1016/j.apradiso.2009.11.058
  8. Ziemek T, Jeczmieniowski A, Cacko D, Broda R, Lech E. A new $4{\pi}(LS)-{\gamma}$ coincidence counter at NCBJ RC POLATOM with TDCR detector in the beta channel. Appl Radiat Isot. 2016;109:290-295. https://doi.org/10.1016/j.apradiso.2015.12.017
  9. Sochorova J, Auerbach P. Activity standardization of $^{134}Cs$ and $^(137}Cs$. Appl Radiat Isot. 2014;87:207-210. https://doi.org/10.1016/j.apradiso.2013.11.127
  10. da Silva CJ, da Cruz PA, Iwahara A, Loureiro JD, Gomes RD, Dos Santos AR, et al. $^{134}Cs$ activity standardization by $4{\pi}{\beta}(LS)-{\gamma}(NaITl)$ anticoincidence counting and submission to international reference system. Appl Radiat Isot. 2018;134:316-320. https://doi.org/10.1016/j.apradiso.2017.10.025
  11. Be MM, Chiste V, Dulieu C, Browne E, Chechev V, Kuzmenko N, et al. Table of Radionuclides [Internet]. Sevres, France: Bureau International des Poids et Mesures; c2017 [cited 2020 May 31]. Available from: https://www.bipm.org/en/publications/scientific-output/monographie-ri-5.html
  12. Cox DR, Isham V. A bivariate point process connected with electronic counters. Proc R Soc Lond A Math Phys Sci. 1977;356:149-160.
  13. Smith D. Improved correction formulae for coincidence counting. Nucl Instrum Methods. 1978;152:505-519. https://doi.org/10.1016/0029-554X(78)90052-6