DOI QR코드

DOI QR Code

Coincidence Summing Corrections in HPGe Gamma Ray Spectrometry in Marinelli-beakers with Efficiency

효율을 적용한 마리넬리 비이커에서 HPGe 감마선 분광분석법의 동시합성보정

  • Jang, Eun-Sung (Department of Radiation Oncology Kosin University Gospel Hospital) ;
  • Lee, Hyo-Yeong (Department of Radiological Science, Dongeui University)
  • 장은성 (고신대학교 복음병원 방사선종양학과) ;
  • 이효영 (동의대학교 방사선학과)
  • Received : 2018.07.18
  • Accepted : 2018.10.31
  • Published : 2018.10.31

Abstract

Coincidence summing correction effects are known to be greater as the efficiency of the detector increases and as the distance between the source and the detector increases. A point source($^{60}Co$) was used to vary the distance in the direction of the detector's center axis and in the radial direction to obtain the P/T ratio for Coincidence summing correction calibration. In this study, values for coincidence summing corrected calibration of the values in the central and radial directions were applied to the mixed volume source(450 ml CRM source) to compare the overall peak efficiency change according to P/T with Geant4. In addition, the efficiency obtained from the mapping method is applied to the seaweed, a marine sample, and the compatibility of the P/T ratio with the detector and sample very dose together. The efficiency corrected to 1,836 keV was applied to the energy zone affected by the efficiency of 500 keV and the relative error of the measured and corrected values was well matcched by the 3.2 % peak efficiency correction. As with 450 mL CRM source, the larger the volume, the lower the P/T ratio was by ${\pm}5%$. This is due to the increased scattering of gamma-rays emitted as the source becomes farther away from the detector, and this change in P/T has been confirmed to affect the Coincidence summing corrected peak efficiency.

동시 합성 보정 효과는 검출기의 효율이 향상할 때 그리고 선원과 검출기 사이의 거리가 가까울수록 크게 나타나는 것으로 알려져 있다. 점 선원($^{60}Co$)을 사용하여 검출기 중심축 방향 및 방사상 방향에서 거리에 따른 변화를 주어 P/T 비를 구하여 동시합성 보정을 하였다. 따라서 본 연구에서는 중심축 및 방사상 방향에서 동시합성 보정한 값들을 혼합부피선원(450 mL CRM source)에 적용하여 P/T에 따른 전체 피크효율 변화를 Geant4과 비교하였다. 또한 검출기와 시료가 아주 밀착된 상태에서 맵핑법에서 구한 효율을 환경시료 중에서 해양 시료인 미역에 적용하여 P/T 비의 적합성을 평가하고자 한다. 500 keV 이상의 효율의 영향을 받는 에너지 영역에 1,836 keV로 보정한 효율을 적용한 결과 측정값과 보정값의 상대오차는 3.2 % peak 효율이 보정되어 잘 일치하였다. 450 mL CRM source처럼 부피가 커질수록 P/T 비는 ${\pm}5%$까지 감소하였다. 이것은 검출기로부터 선원이 멀어짐에 따라 방출된 감마선의 산란이 많아지기 때문이며, 이처럼 P/T 변화는 동시합성 보정 피크 효율에 영향을 줌을 확인하였다.

Keywords

References

  1. Keyser, Ronald MRonald M., Susan E. Haywood, and Daniel L. Upp., "Performance of the True Coincidence Correction Method in Gamma Vision," Journal of Radioanalical and Nuclear Chemistry, Vol. 245, No. 4, pp. 185-188, 2000. https://doi.org/10.1023/A:1006722512885
  2. McFarland, R. C. "Coincidence Summing Considerations When Using Marinelli-Beaker Geometries in Germanium Gamma-Ray Spectrometry," Radioactivity and Radiochemistry, Vol. 2, No. 3, pp. 72-74, 1991.
  3. De Felice, Pierino, et al. "Fast Procedures for coincidence summing correction in Gamma-Ray Spectrometry," Applied Radiation and Isotopes, Vol. 52. No. 3, pp. 745-752, 2000. https://doi.org/10.1016/S0969-8043(99)00239-0
  4. Blaauw, Menno, Sjoerd J. Gelsema. "Cascade summing in gamma-ray spectrometry in marinelli-beaker geometries: the third efficiency curve," Nuclear Instruments and Methods in Physicis Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 505, No. 1-2, pp. 311-315, 2003.
  5. Garcia-Torano, Eduardo, Milagros Pozuelo, and Francesc Salvat, "Monte Carlo calculations of coincidence summing corrections for volume sources in gamma-ray spectrometry with Ge detectors," Nuclear Instruments and Methods in Physicis Research Section A: Acclerators, Spectrometers, Detectors and Associated Equipment, Vol. 554, No. 3, pp. 577-583, 2005.
  6. Garcia-Talavera, M., et al. "Coincidence summing corrections for the natural decay series in gamma-ray dpectrometry." Applied Radiation anf Isotopes Vol. 54, No. 5, pp. 769-776, 2001. https://doi.org/10.1016/S0969-8043(00)00318-3
  7. S. H. Kim, "Evaluation of The Cascade Summing effect for HPGe Detector by Using The Cross Analysis Sample," Journal of Radiation Protection and Research. Vol. 30, No. 2, pp. 103-112, 2005.
  8. M. S. Lee, "Study on the cascade summing correction for high efficiency HPGe detector," Journal of Radiation Protection and Research. Vol. 30, No. 3, pp. 107-112, 2005.
  9. Giubrone, G., et al. "Calculation of Coincidence Summing Correction Factors for an HPGe detector using GEANT4," Journal of environmental radioactivity, Vol. 158-159, pp. 114-118, 2016. https://doi.org/10.1016/j.jenvrad.2016.04.008
  10. M. Lee, T. S. Park, J. K. Woo, "Coincidence summing effects in gamma ray spectrometry using a Marinelli beaker," Applied Radiation and Isotopes, Vol. 66, No. 6-7, pp. 799-803. 2008. https://doi.org/10.1016/j.apradiso.2008.02.017
  11. M. C. Lepy. "Total efficiency calibration for coincidence summing corrections," Nuclear Instruments and. Methods in Physics Research, Vol. 579, No. 1, pp 284-287, 2007. https://doi.org/10.1016/j.nima.2007.04.081
  12. C. C. Conti, I. C .P. Salinas, H. Zylberberg, "A detailed procedure to simualte an HPGe detector with MCNP5," Progress in Nuclear Energy, Vol, 66, pp. 35-40, 2013. https://doi.org/10.1016/j.pnucene.2013.03.003
  13. C. S. Chaudhury, A. Goswami, et al., "Full energy peak efficiency calibration of HPGe detector for point and extended sources using Monte Carlo code," Journal of Radioanalitical and Nuclear Chemistry, Vol. 287, No. 3, pp. 701-708, 2010.
  14. E, Tomarchio, "Coincidence summing correction equations in gamma-ray spectrometry with p-type HPGe detectors," Radiation Physics and Chemistry, Vol. 80, No. 3, pp. 318-323, 2011. https://doi.org/10.1016/j.radphyschem.2010.09.014
  15. G. Haase, D. Tait, A. Wiechen, "Monte Carlo simulation of several gamma-emitting source and detector arrangments for determining corrections of self-attenuation and coincidence summation in gamma-spectrometry," Nuclear Instruments and. Methods in Physics Research, Vol. A239, No. 3, pp. 483-492, 1993.
  16. M.Decombaz, J. J. Gostely, J. P. Lawdermann, "Coincidence summing corrections for extended sources in gamma-ray spectrometry using Monte Carlo simulation," Nuclear Instruments and. Methods in Physics Research, Vol. A312, No. 1-2, pp. 152-159, 1992.
  17. R. G. Helmer, R. J. Cek, "Calculation of coincidence summing corrections for a specific small soil sample geometry," Radioactivity Radiochemistry, Vol. 8, No. 1, pp. 18-29, 1997.
  18. B. S. Zoran Milosevic, "Coincidence summing correction for point and volume 152Eu sources," Applied Radiation and Isotopes, Vol.107, pp 138-144, 2016. https://doi.org/10.1016/j.apradiso.2015.10.015
  19. Laslo J. Nadderd, Dragana J. Jordanov, Molos D. Davidovic, "A new matrix method for calculating coincidence summing effects for gamma spectroscopy," Nuclear Instruments and Method in Physics Research, Vol. 662, No. 1, pp 21-25, 2012. https://doi.org/10.1016/j.nima.2011.10.002
  20. Yosimune Ogata, Hiroshi Miyahara, Ishiqure Nobuhito, Masashi Ishihara., "Development of the modified sum-peak method and its application," Applied Radiation and Isotopes, Vol. 109, pp. 354-357, 2015.
  21. M. J. Safari, H. A. Heidari, "Method for developing HPGe detector model in Monte Carlo simuilation codes," Radiation Measurements, Vol. 88, 2016.
  22. Y. D. Qingbin, W. Z. Ma, "HPGe detector application on monitoring environmental samples around the accelerator," IPAC, 2016.