Journal of Industrial and Engineering Chemistry

  • Volume 68
  • /
  • Pages.406-415
  • /
  • 2018
  • /
  • 1226-086X(pISSN)
  • /
  • 1876-794X(eISSN)
The Korean Society of Industrial and Engineering Chemistry (한국공업화학회)
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Implementation of magnetic Fe3O4@ZIF-8 nanocomposite to activate sodium percarbonate for highly effective degradation of organic compound in aqueous solution

  • Sajjadi, Saeed (Research Laboratory of Advanced Water and Wastewater Treatment Processes, Department of Applied Chemistry, Faculty of Chemistry, University of Tabriz) ;
  • Khataee, Alireza (Research Laboratory of Advanced Water and Wastewater Treatment Processes, Department of Applied Chemistry, Faculty of Chemistry, University of Tabriz) ;
  • Soltani, Reza Darvishi Cheshmeh (Department of Environmental Health Engineering, School of Health, Arak University of Medical Sciences) ;
  • Bagheri, Nafiseh (Research Laboratory of Advanced Water and Wastewater Treatment Processes, Department of Applied Chemistry, Faculty of Chemistry, University of Tabriz) ;
  • Karimi, Afzal (Faculty of Advanced Technologies in Medicine, Iran University of Medical Sciences) ;
  • Azar, Amirali Ebadi Fard (Faculty of Medicine, Iran University of Medical Sciences)
  • Received : 2018.05.23
  • Accepted : 2018.08.27
  • Published : 2018.12.25
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Abstract

Here, as-synthesized $Fe_3O_4$ nanoparticles were incorporated into the zeolitic imidazolate framework (ZIF-8) lattice to activate sodium percarbonate (SPC) for degradation of methylene blue (MB). The reaction rate constant of $Fe_3O_4@ZIF-8/SPC$ process ($0.0632min^{-1}$) at acidic conditions (pH = 3) was more than six times that of the $Fe_3O_4/SPC$ system ($0.009min^{-1}$). Decreasing the solute concentration, along with increasing SPC concentration and $Fe_3O_4@ZIF-8$ nanocomposite (NC) dosage, favored the catalytic degradation of MB. The $Fe_3O_4@ZIF-8$ NC after fifteen consecutive treatment processes showed the excellent stability with a negligible drop in the efficiency of the system (<10%). The reaction pathway was obtained via GC-MS analysis.

Keywords

Acknowledgement

Supported by : University of Tabriz, Arak University of Medical Sciences

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