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대기 라돈 및 기체상 오염물질의 기류 이동경로별 농도변화: 2010~2015년 측정

Concentration Variation of Atmospheric Radon and Gaseous Pollutants Related to the Airflow Transport Pathways during 2010~2015

  • 송정민 (제주대학교 화학.코스메틱스학과) ;
  • 김기주 (제주대학교 화학.코스메틱스학과) ;
  • 부준오 (제주대학교 화학.코스메틱스학과) ;
  • 김원형 (제주대학교 화학.코스메틱스학과) ;
  • 강창희 (제주대학교 화학.코스메틱스학과) ;
  • Song, Jung-Min (Department of Chemistry and Cosmetics, Jeju National University) ;
  • Kim, Ki-Ju (Department of Chemistry and Cosmetics, Jeju National University) ;
  • Bu, Jun-Oh (Department of Chemistry and Cosmetics, Jeju National University) ;
  • Kim, Won-Hyung (Department of Chemistry and Cosmetics, Jeju National University) ;
  • Kang, Chang-Hee (Department of Chemistry and Cosmetics, Jeju National University) ;
  • Chambers, S. (Australian Nuclear Science and Technology Organisation)
  • 투고 : 2018.03.05
  • 심사 : 2018.03.22
  • 발행 : 2018.04.30

초록

Concentrations of the atmospheric radon and gaseous pollutants were measured at the Gosan site on Jeju Island from 2010 to 2015, in order to observe their time-series variation characteristics and examine the concentration change related to the airflow transport pathways. Based on the realtime monitoring of the atmospheric radon and gaseous pollutants, the daily mean concentrations of radon ($^{222}Rn$) and gaseous pollutants($SO_2$, CO, $O_3$, $NO_x$) were $2,400mBq\;m^{-3}$ and 1.3, 377.6, 41.1, 3.9 ppb, respectively. On monthly variations of radon, the mean concentration in October was the highest as $3,033mBq\;m^{-3}$, almost twice as that in July ($1,452mBq\;m^{-3}$). The diurnal variation of radon concentration shows bimodal curves at early morning (around 7 a.m.) and near midnight, whereas its lowest concentration was recorded at around 3 p.m. Several gaseous pollutants($SO_2$, CO, $NO_x$) showed a similar seasonal variation with radon concentration as high in winter and low in summer, whereas the $O_3$ concentrations had a bit different seasonal trend. According to the cluster back trajectory analysis, the frequencies of airflow pathways moving from continental North China, East China, Japan and the East Sea, the Korean Peninsula, and North Pacific Ocean routes were 36, 37, 10, 13, and 4%, respectively. When the airflow were moved to Jeju Island from continental China, the concentrations of radon and gaseous pollutants were relatively high. On the other hand, when the airflows were moved from North Pacific Ocean and East Sea, their concentrations were much lower than those from continental China.

키워드

참고문헌

  1. Almeida, R.M., Lauria, D.C., Ferreira, A.C., Sracek, O. (2004) Groundwater radon, radium and uranium concentrations in Região dos Lagos, Rio de Janeiro State, Bra­zil, Journal of Environmental Radioactivity, 73(3), 323-334. https://doi.org/10.1016/j.jenvrad.2003.10.006
  2. Chambers, S., Zahorowski, W., Matsumoto, K. Uematsu, M. (2009) Seasonal variability of radon-derived fetch regions for Sado Island, Japan, based on 3 years of observations: 2002-2004, Atmospheric Environment, 43(2), 271-279. https://doi.org/10.1016/j.atmosenv.2008.09.075
  3. Chambers, S.D., Kang, C.H., Williams, A.G., Crawford, J., Griffths, A.D., Kim, K.H., Kim, W.H. (2016) Improving the representation of cross-boundary transport of anthropogenic pollution in Southeast Asia using Radon-222, Aerosol and Air Quality Research, 16(4), 958-­976, doi: 10.4209/aaqr.2015.08.0522.
  4. Chan, S.W., Lee, C.W., Tsui, K.C. (2010) Atmospheric radon in Hong Kong, Journal of Environmental Radioactivity, 101(6), 494-503. https://doi.org/10.1016/j.jenvrad.2010.02.007
  5. Choi, I.C., Shin, S.H., Jo, W.K. (2009) Evaluation of radon levels in various public-acess buildings or underground facilities, and their temporal variation in underground facilities, Journal of Environmental Toxicology, 24(3), 203-211. (in Korean with English abstract)
  6. Draxler, R.R., Rolph, G.D. (2013) HYSPLIT (HYbrid Single-Particle Lagrangian Integrated Trajectory) Model access via NOAA ARL READY Website, (http://ready.arl.noaa.gov/HYSPLIT_traj.php).
  7. Duckworth, F.A., Sandberg, J.S. (1954) The effect on cities upon horizontal and vertical temperature gradients, Bulletin of the American Meteorological Society, 35, 198-207.
  8. Kang, C.H., Kim, W.H., Hu, C.G., Kang, D.H. (2012) Real-time monitoring of radon background level at Gosan site, Jeju Island, Journal of Analytical Science & Technology, 25(1), 7-13. (in Korean with English abstract) https://doi.org/10.5806/AST.2012.25.1.007
  9. Kim, E.H., Kim, P.S., Kim, C.Y., Lee, K.S., Kwon, K.D. (1985) Determination of the mixing height in Seoul by the radioactivity measurement of radon in air, Bulletin of Environmental Sciences (Research Institute for Environmental Sciences Hanyang University), 6(2), 129-136.
  10. Kim, Y.S., Lee, C.M., Kim, K.Y., Jeon, H.J., Kim, J.C., Iida, T. (2007) Time series observations of atmospheric radon concentration in Seoul, Korea for an analysis of long-range transportation of air pollutants in the North-East Asia, Korean Journal of Environmental Health Sciences, 33(4), 283-292. (in Korean with English abstract) https://doi.org/10.5668/JEHS.2007.33.4.283
  11. Lee, K., Seo, S., Yoo, J., Oh, S., Kwon, M., Lee, W. (2016) Factors infuencing indoor radon concentration in detached house, Journal of Odor Indoor Environment, 15(2), 93-99. (in Korean with English abstract) https://doi.org/10.15250/joie.2016.15.2.93
  12. Miles, J. (1988) Development of maps of radon-prone areas using radon measurements in houses, Journal of Hazardous Materials, 61, 53-58.
  13. Ministry of Environment (MOE) (2007) Comprehensive Countermeasures for Indoor Radon Control (2007-2012); Safe Maintenance of Indoor Environment from Radon (accessed on Aug., 2007).
  14. Ministry of Science & Technology (MST) (2007) Assessment of Radiation Risk for the Korean Population, KINS/GR-355, 185 pp. (accessed on Feb., 2007).
  15. Moon, K.H., Kim, J.S., Ahn, J.K., Kim, H.C., Lee, H.M. (2009) Long-term variation of radon in granitic residual soil at Mt. Guemjeong in Busan, Korea, The Journal of the Petrological Society of Korea, 18(4), 279-291.
  16. National Institute of Environmental Research (NIER) (2009) Investigation for Nationwide Actual Indoor Radon: Research Report of Public Facilities (accessed on Feb., 2009).
  17. National Institute of Environmental Research (NIER) (2016) Annual Report of Air Quality in Korea, 2015. NIER-GP2016-122.
  18. National Research Council (NRC) (2000) Health risk of radon and other internally deposited alpha emitters, report of the Committee on UNSCEAR. Sources and Effects of Ionizing Radiation. UNSCEAR 2000 Report.
  19. Pitari, G., Coppari, E., De Luca, N., Di Carlo, P. (2014) Observations and box model analysis of radon-222 in the atmospheric surface layer at L'Aquila, Italy: March 2009 case study, Environmental Earth Sciences, 71(5), 2353-2359. https://doi.org/10.1007/s12665-013-2635-1
  20. Song, J.M., Bu, J.O., Kim, W.H., Kang, C.H., Ko, H.J., Cham­bers, S. (2017) Background level and time series variation of atmospheric radon concentrations at Gosan site in Jeju Island, Journal of Korean Society for Atmospheric Environment, 33(2), 174-183. (in Korean with English abstract) https://doi.org/10.5572/KOSAE.2017.33.2.174
  21. U.S. Environmental Protection Agency (US EPA) (2003) EPA Assessment of Risks from Radon in Homes, EPA 402-R-03-003.
  22. Whittlestone, S., Zahorowski, W. (1998) Baseline radon detec­tors for shipboard use: Development and deployment in the First Aerosol Characterization Experiment (ACE 1), Journal of Geophysical Research, 103(D13), 16,743-16,751. https://doi.org/10.1029/98JD00687
  23. World Meteorological Organization/Global Atmospheric Watch (WMO/GAW) (2001) Global Atmosphere Watch Measurements Guide (No. 143), WMO TD No. 1073.
  24. World Meteorological Organization/Global Atmospheric Watch (WMO/GAW) (2004) 1st International Expert Meeting on Sources and Measurements of Natural Radio nuclides Applied to Climate and Air Quality Studies (No. 155), WMO TD No. 1201.
  25. Zahorowski, W., Chambers, S.D., Henderson-Sellers, A. (2004) Ground based radon-222 observations and their application to atmospheric studies, Journal of Environmental Radioactivity, 76(1-2), 3-33. https://doi.org/10.1016/j.jenvrad.2004.03.033
  26. Zahorowski, W., Chambers, S., Wang, T., Kang, C.H., Uno, I., Poon, S., Oh, S.N., Wercqynski, S., Kim, J., Hender­son-Sellers, A. (2005) Radon-222 in boundary layer and free tropospheric continental outfow events at three ACE-Asia sites, Tellus, 57(2), 124-140. https://doi.org/10.3402/tellusb.v57i2.16776
  27. Zoran, M.A., Dida, M.R., Zoran, A.T., Zoran, L.F., Dida, A. (2013) Outdoor $^{222}Radon$ concentrations monitoring in relation with particulate matter levels and possible health effects, Journal of Radioanalytical Nuclear Chemistry, 296(3), 1179-1192. https://doi.org/10.1007/s10967-012-2259-z