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Evaluation of the Simulated PM2.5 Concentrations using Air Quality Forecasting System according to Emission Inventories - Focused on China and South Korea

대기질 예보 시스템의 입력 배출목록에 따른 PM2.5 모의 성능 평가 - 중국 및 한국을 중심으로

  • Choi, Ki-Chul (Air Quality Forecasting Center, National Institute of Environmental Research) ;
  • Lim, Yongjae (Air Quality Forecasting Center, National Institute of Environmental Research) ;
  • Lee, Jae-Bum (Air Quality Forecasting Center, National Institute of Environmental Research) ;
  • Nam, Kipyo (Air Quality Forecasting Center, National Institute of Environmental Research) ;
  • Lee, Hansol (Air Quality Forecasting Center, National Institute of Environmental Research) ;
  • Lee, Yonghee (Air Quality Forecasting Center, National Institute of Environmental Research) ;
  • Myoung, Jisu (Air Quality Forecasting Center, National Institute of Environmental Research) ;
  • Kim, Taehee (Air Quality Forecasting Center, National Institute of Environmental Research) ;
  • Jang, Limseok (Air Quality Forecasting Center, National Institute of Environmental Research) ;
  • Kim, Jeong Soo (Air Quality Forecasting Center, National Institute of Environmental Research) ;
  • Woo, Jung-Hun (College of Global Integrated Studies, Konkuk University) ;
  • Kim, Soontae (Department of Environmental & Safety Engineering, Ajou University) ;
  • Choi, Kwang-Ho (Department of General Education, Namseoul University)
  • 최기철 (국립환경과학원 대기질통합예보센터) ;
  • 임용재 (국립환경과학원 대기질통합예보센터) ;
  • 이재범 (국립환경과학원 대기질통합예보센터) ;
  • 남기표 (국립환경과학원 대기질통합예보센터) ;
  • 이한솔 (국립환경과학원 대기질통합예보센터) ;
  • 이용희 (국립환경과학원 대기질통합예보센터) ;
  • 명지수 (국립환경과학원 대기질통합예보센터) ;
  • 김태희 (국립환경과학원 대기질통합예보센터) ;
  • 장임석 (국립환경과학원 대기질통합예보센터) ;
  • 김정수 (국립환경과학원 대기질통합예보센터) ;
  • 우정헌 (건국대학교 글로벌융합대학 융합인재학부) ;
  • 김순태 (아주대학교 환경공학과) ;
  • 최광호 (남서울대학교 교양과정부)
  • Received : 2018.02.09
  • Accepted : 2018.03.05
  • Published : 2018.04.30

Abstract

Emission inventory is the essential component for improving the performance of air quality forecasting system. This study evaluated the simulated daily mean $PM_{2.5}$ concentrations in South Korea and China for 1-year period (Sept. 2016~Aug. 2017) using air quality forecasting system which was applied by the emission inventory of E2015 (predicted CAPSS 2015 for South Korea and KORUS 2015 v1 for the other regions). To identify the impacts of emissions on the simulated $PM_{2.5}$, the emission inventory replaced by E2010 (CAPSS 2010 and MIX 2010) were also applied under the same forecasting conditions. These results showed that simulated daily mean $PM_{2.5}$ concentrations had generally suitable performance with both emission data-sets for China (IOA>0.87, R>0.87) and South Korea (IOA>0.84, R>0.76). The impacts of the changes in emission inventories on simulated daily mean $PM_{2.5}$ concentrations were quantitatively estimated. In China, normalized mean bias (NMB) showed 5.5% and 26.8% under E2010 and E2015, respectively. The tendency of overestimated concentrations was larger in North Central and Southeast China than other regions under both E2010 and E2015. Seasonal differences of NMB were higher in non-winter season (28.3% (E2010)~39.3% (E2015)) than winter season (-0.5% (E2010)~8.0% (E2015)). In South Korea, NMB showed -5.4% and 2.8% for all days, but -15.2% and -11.2% for days below $40{\mu}g/m^3$ to minimize the impacts of long-range transport under E2010 and E2015, respectively. For all days, simulated $PM_{2.5}$ concentrations were overestimated in Seoul, Incheon, Southern part of Gyeonggi and Daejeon, and underestimated in other regions such as Jeonbuk, Ulsan, Busan and Gyeongnam, regardless of what emission inventories were applied. Our results suggest that the updated emission inventory, which reflects current status of emission amounts and spatio-temporal allocations, is needed for improving the performance of air quality forecasting.

Keywords

References

  1. Bae, C.H., Kim, H.C., Kim, B.U., Kim, S. (2015) Improvement of PM forecast using PSAT based customized emission inventory over Northeast Asia, 14th Annual CMAS Models-3 Users' Conference, October 5-7, Chapel Hill, NC.
  2. Byun, D.W., Ching, J.K.S. (1999) Science algorithms of the EPA Models-3 community multi-scale air quality (CMAQ) modeling system, NERL, Research Triangle Park, NC.
  3. Chen, F., Dudhia, J. (2001) Coupling an advanced land surface-hydrology model with the Penn State-NCAR MM5 modeling system. Part I: Model implementation and sensitivity, Monthly Weather Review, 129(4), 569-585. https://doi.org/10.1175/1520-0493(2001)129<0569:CAALSH>2.0.CO;2
  4. Davies, T., Cullen, M.J.P., Malcolm, A.J., Mawson, M.H., Staniforth, A., White, A.A., Wood, N. (2005) A new dynamical core for the Met Office's global and regional modelling of the atmosphere, Quarterly Journal of the Royal Meteorological Society, 131(608), 1759-1782. https://doi.org/10.1256/qj.04.101
  5. Emery, C., Liu, Z., Russell, A.G., Odman, M.T., Yarwood, G., Kumar, N. (2016) Recommendations on statistics and benchmarks to assess photochemical model performance, Journal of the Air and Waste Management Association, 67(5), 582-598.
  6. Ghim, Y.S., Choi, Y., Kim, S., Bae, C.H., Park, J., Shin, H.J. (2017) Evaluation of model performance for forecasting fne particle concentrations in Korea, Aerosol and Air Quality Research, 17(7), 1856-1864. https://doi.org/10.4209/aaqr.2016.10.0446
  7. Guenther, A., Karl, T., Harley, P., Wiedinmyer, C., Palmer, P.I., Geron, C. (2006) Estimates of global terrestrial isoprene emissions using MEGAN (Model of Emissions of Gases and Aerosols from Nature), Atmospheric Chemistry and Physics, 6(11), 3181-3210. https://doi.org/10.5194/acp-6-3181-2006
  8. Hong, S., Noh, Y., Dudhia, J. (2006) A New Vertical Diffusion Package with an Explicit Treatment of Entrainment Processes, Monthly Weather Review, 134(9), 2318-2341. https://doi.org/10.1175/MWR3199.1
  9. Huang, X., Song, Y., Li, M., Li, J., Huo, Q., Cai, X., Zhu, T., Hu, M., Zhang, H. (2012) A high-resolution ammonia emission inventory in China, Global Biogeochemical Cycles, 26(1), 1-14.
  10. Hurley, P.J., Blockley, A., Rayner, K. (2001) Verifcation of a prognostic meteorological and air pollution model for year-long predictions in the Kwinana industrial region of Western Australia, Atmospheric Environment, 35(10), 1871-1880. https://doi.org/10.1016/S1352-2310(00)00486-6
  11. Kanaya, Y., Matsui, H., Taketani, F., Pan, X., Komazaki, Y., Wang, Z., Chang, L., Kang, D., Choi, M., Kim, S.Y., Kang, C.H., Takami, A., Tanimoto, H., Ikeda, K., Yamaji, K. (2017) Observed and modeled mass concentrations of organic aerosols and $PM_{2.5}$ at three remote sites around the East China Sea: Roles of chemical aging, Aerosol and Air Quality Research, 17(12), 3091-3105. https://doi.org/10.4209/aaqr.2016.12.0573
  12. Kim, H.C., Kim, E., Bae, C., Cho, J.H., Kim, B.-U., Kim, S. (2017) Regional contributions to particulate matter concentration in the Seoul metropolitan area, South Korea: seasonal variation and sensitivity to meteorology and emissions inventory, Atmospheric Chemistry and Physics, 17(17), 10315-10332. https://doi.org/10.5194/acp-17-10315-2017
  13. Kim, J.-H., Choi, D.-R., Koo, Y.-S., Lee, J.-B., Park, H.-J. (2016) Analysis of Domestic and Foreign Contributions using DDM in CMAQ during Particulate Matter Episode Period of February 2014 in Seoul, Journal of Korean Society for Atmospheric Environment, 32(1), 82-99. (in Korean with English abstract) https://doi.org/10.5572/KOSAE.2016.32.1.082
  14. Kim, S., Moon, N., Byun, D.W. (2008) Korea Emissions Inventory Processing Using the US EPA 's SMOKE System, Asian Journal of Atmospheric Environment, 2(1), 34-46. https://doi.org/10.5572/ajae.2008.2.1.034
  15. Lee, D., Kim, S., Kim, H., Ngan, F. (2014) Retrospective Air Quality Simulations of the TexAQS-II: Focused on Emissions Uncertainty, Asian Journal of Atmospheric Environment, 8(4), 212-224. https://doi.org/10.5572/ajae.2014.8.4.212
  16. Li, M., Zhang, Q., Kurokawa, J.I., Woo, J.H., He, K., Lu, Z., Ohara, T., Song, Y., Streets, D.G., Carmichael, G.R., Cheng, Y., Hong, C., Huo, H., Jiang, X., Kang, S., Liu, F., Su, H., Zheng, B. (2017) MIX: A mosaic Asian anthropogenic emission inventory under the international collaboration framework of the MICS-Asia and HTAP, Atmospheric Chemistry and Physics, 17(2), 935-963. https://doi.org/10.5194/acp-17-935-2017
  17. National Institute of Environmental Research (NIER) (2014) National air pollutants emission 2012.
  18. National Institute of Environmental Research (NIER) (2016a) An international measurement campaign on megacity air pollution study (II) - Modeling study for investigation of source of urban air pollution and emission inventory verifcation.
  19. National Institute of Environmental Research (NIER) (2016b) Improvement of Ozone Forecast Accuracy and Emission Preparation Model (III).
  20. National Institute of Environmental Research (NIER) (2017) the status of particulate matter and current measures for China 2017.
  21. Park, R.S., Han, K.M., Song, C.H., Park, M.E., Lee, S.J., Hong, S.Y., Kim, J., Woo, J.-H. (2013) Current Status and Development of Modeling Techniques for Forecasting and Monitoring of Air Quality over East Asia, Journal of Korean Society for Atmospheric Environment, 29(4), 407-438. (in Korean with English abstract) https://doi.org/10.5572/KOSAE.2013.29.4.407
  22. Skamarock, W.C., Klemp, J.B. (2008) A time-split nonhydrostatic atmospheric model for weather research and forecasting applications, Journal of Computational Physics, 227(7), 3465-3485. https://doi.org/10.1016/j.jcp.2007.01.037
  23. U.S. Environmental Protection Agency (US EPA) (2008) Technical Support Document: Preparation of Emissions Inventories for the 2002-based Platform, Version 3, Criteria Air Pollutants.
  24. Willmott, C.J., Ackleson, S.G., Davis, R.E., Feddema, J.J., Klink, K.M., Legates, D.R., O'Donnell, J., Rowe, C.M. (1985) Statistics for the evaluation and comparisons of models, Journal of Geophysical Research, 90(C5), 8995-9005. https://doi.org/10.1029/JC090iC05p08995
  25. Woo, J.-H., Choi, K.-C., Kim, H.K., Baek, B.H., Jang, M., Eum, J.-H., Song, C.H., Ma, Y.-I., Sunwoo, Y., Chang, L.-S., Yoo, S.H. (2012) Development of an anthropogenic emissions processing system for Asia using SMOKE, Atmospheric Environment, 58, 5-13. https://doi.org/10.1016/j.atmosenv.2011.10.042
  26. Zhang, Q., Streets, D.G., Carmichael, G.R., He, K.B., Huo, H., Kannari, A., Klimont, Z., Park, I.S., Reddy, S., Fu, J.S., Chen, D., Duan, L., Lei, Y., Wang, L.T., Yao, Z.L. (2009) Asian emissions in 2006 for the NASA INTEX-B mission, Atmospheric Chemistry and Physics, 9(14), 5131-5153. https://doi.org/10.5194/acp-9-5131-2009
  27. Zhang, X., Wu, Y., Liu, X., Reis, S., Jin, J., Dragosits, U., Van Damme, M., Clarisse, L., Whitburn, S., Coheur, P.-F., Gu, B. (2017) Ammonia Emissions May Be Substantially Underestimated in China, Environmental Science & Technology, 51(21), 12089-12096. https://doi.org/10.1021/acs.est.7b02171