한국환경과학회지 (Journal of Environmental Science International)

  • 제21권2호
  • /
  • Pages.165-179
  • /
  • 2012
  • /
  • 1225-4517(pISSN)
  • /
  • 2287-3503(eISSN)
한국환경과학회 (The Korean Environmental Sciences Society)
권호 표지
DOI QR코드

DOI QR Code

비메탄계 휘발성유기화합물에 의한 간접 온실효과의 산출

Estimation of Indirect Greenhouse Effect by Non-methane Volatile Organic Compounds

  • 최은화 (한국환경공단 기후변화대응처)
  • Choi, Eun-Hwa (Department of Climate Change Action, Korea Environmental Corporation)
  • 투고 : 2011.09.16
  • 심사 : 2012.01.03
  • 발행 : 2012.02.29
PDF 다운로드
⟨ 이전 논문 다음 논문 ⟩

초록

Indirect $CO_2$ effect due to non-methane volatile organic compound (NMVOC) emissions from solvent and product use and fugitive NMVOC emissions from fuels in the Republic of Korea and 13 Annex I countries under United Nations Framework on Climate Change were estimated and the proportions of them to total greenhouse gas (GHG) emissions ranged from 0.092% to 0.45% in 2006. Indirect greenhouse effect ($CO_2$, $CH_4$, and $O_3$) were estimated at 13 photochemical assessment monitoring sites in the Republic of Korea using concentrations of 8 NMVOCs of which indirect global warming potential (GWP) were available. The contribution of toluene to mixing ratio was highest at 11 sites and however, the contribution of toluene to indirect greenhouse effect was highest at nine sites. In contrast to toluene, the contributions of ethane, butane, and ethylene were enhanced. The indirect greenhouse effects of ethane and propane, of which ozone formation potentials are the lowest and the third lowest respectively among targeted 10 NMVOCs, ranked first and fourth highest respectively. Acetaldehyde has relatively higher maximum incremental reactivity and is classified as probable human carcinogen however, its indirect GWP ranked second lowest.

키워드

참고문헌

  1. 에너지경제연구원, 2011, 온실가스배출통계, http://www.kesis.net/flexapp/KesisFlexApp.jsp.
  2. 환경부, 2005, 대기환경연보(2004), 부록 7.
  3. 환경부, 2006, 대기환경연보(2005), 부록 7.
  4. 환경부, 2007, 대기환경연보(2006), 부록 7.
  5. 환경부, 2008, 대기환경연보(2007), 부록 7.
  6. 환경부, 2009, 대기환경연보(2008)., 부록 7과 부록 13.
  7. Choi, E., Heo, J. B., Yi, S. M., 2010, Apportioning and locating non-methane hydrocarbon sources to a background site in Korea,. Environ Sci Technol, 44(15), 5849-5854. https://doi.org/10.1021/es903634e
  8. Choi, E., Heo, J. B., Hopke, P. K., Jin, B. B., Yi, S. M., 2011, Identification, apportionment, and photochemical reactivity of non-methane hydrocarbon sources in Busan, Korea, Water Air Soil Poll, 215(1-4), 67-82. https://doi.org/10.1007/s11270-010-0459-0
  9. Carter, W. P. L, 2010, Development of the SAPRC-07 chemical mechanism and updated ozone reactivity scales, Report to the California Air Resources Board, Contracts No. 03-318, 06-408, and 07-730
  10. Collins, W. J., Derwent, R. G., Johnson, C. E., Stevenson, D. S., 2002, The oxidation of organic compounds in the troposphere and their global warming potentials, Climatic Change, 52(4), 453-479. https://doi.org/10.1023/A:1014221225434
  11. Gillenwater, M., 2008, Forgotten carbon: indirect $CO_{2}$ in greenhouse gas emission inventories, Environ Sci Policy, 11(3), 195-203. https://doi.org/10.1016/j.envsci.2007.09.001
  12. IEA, 2009, $CO_{2}$ emissions from fuel combustion, OECD/IEA, Paris, France, III.44-III.47
  13. IPCC, 1990, Climate change : The IPCC scientific assessment, Cambridge University Press, Cambridge, United Kingdom and New York, NY, USA, 58-61.
  14. IPCC, 1997, Revised 1996 IPCC guidelines for national greenhouse inventories, IPCC/OECD/IEA, Paris, France.
  15. IPCC, 2000, Emissions scenarios, Cambridge University Press, UK, 570.
  16. IPCC, 2006, 2006 IPCC guidelines for national greenhouse gas inventories, IGES, Japan.
  17. IPCC, 2007, Climate change 2007 : The physical science basis, Cambridge University Press, Cambridge, United Kingdom and New York, NY, USA, 214
  18. UNFCCC, 2006, Updated UNFCCC reporting guidelines on annual inventories following incorporation of the provisions of decision 14/CP.11. FCCC/SBSTA/2006/9.
  19. UNFCCC, 2009, Annex I party GHG inventory submissions, http://unfccc.int/national_reports/annex_i_ghg_inventories/national_inventories_submissions/ items/4771.php.
  20. UNFCCC, 2011, Greenhouse gas inventory data - Detailed data by party, http://unfccc.int/di/DetailedByParty.do.
  21. US Environmental Protection Agency, 1989, Risk assessment guidance for superfund (RAGS), Volume I, Part A, Office of Emergency and Remedial Response, Washington, D.C.
  22. US Environmental Protection Agency, 2011, Integrated risk information system, http://www.epa.gov/IRIS.
  23. Watson, J. G., Chow, J. C., Fujita, E. M., 2001, Review of volatile organic compound source apportionment by chemical mass balance, Atmos Environ., 35(9), 1567-1584. https://doi.org/10.1016/S1352-2310(00)00461-1