DOI QR코드

DOI QR Code

Distribution and Source of Atmospheric Polycyclic Aromatic Hydrocarbons and Nitropolycyclic Aromatic Hydrocarbons in Tieling City, Liaoning Province, a Typical Local City in Northeast China

  • Tang, Ning (Graduate School of Natural Science and Technology, and Institute of Medical, Pharmaceutical and Health Sciences, Kanazawa University) ;
  • Araki, Yuki (National Institute for Environmental Studies) ;
  • Tamura, Kenji (Shenyang Center for Disease Control and Prevention) ;
  • Dong, Lijun (Shenyang Center for Disease Control and Prevention) ;
  • Zhang, Xuemei (Shenyang Center for Disease Control and Prevention) ;
  • Liu, Qiuhua (Shenyang Center for Disease Control and Prevention) ;
  • Ji, Ruonan (Shenyang Center for Disease Control and Prevention) ;
  • Kameda, Takayuki (Graduate School of Natural Science and Technology, and Institute of Medical, Pharmaceutical and Health Sciences, Kanazawa University) ;
  • Toriba, Akira (Graduate School of Natural Science and Technology, and Institute of Medical, Pharmaceutical and Health Sciences, Kanazawa University) ;
  • Hayakawa, Kazuichi (Graduate School of Natural Science and Technology, and Institute of Medical, Pharmaceutical and Health Sciences, Kanazawa University)
  • 투고 : 2009.03.09
  • 심사 : 2009.06.17
  • 발행 : 2009.06.30

초록

Airborne particulates were collected in three different size fractions (>7 ${\mu}m$; 2.1-7 ${\mu}m$; < 2.1 ${\mu}m$) by using Andersen low-volume air samplers at three sites in Tieling city, Liaoning Province, a typical local city in northeast China, in every season during the period from July 2003 to May 2004. Nine polycyclic aromatic hydrocarbons (PAHs) and seven nitropolycyclic aromatic hydrocarbons (NPAHs) in the airborne particulates were determined by HPLC with fluorescence and chemiluminescence detection, respectively. The mean total concentrations of the nine PAHs and seven NPAHs were highest at The mixed residential and light industrial site, and lowest at the residential site near the suburbs. At all sites, more than 70% of the total PAHs and more than 60% of the total NPAHs were found in the finest particulate (< 2.1 ${\mu}m$) fraction. Both cluster analysis and several diagnostic ratios showed that the major contributors of PAHs and NPAHs in airborne particulates were coal combustion systems such as domestic stoves and coal boilers in all seasons in Tieling city.

키워드

참고문헌

  1. Arey J., B. Zielinska, R. Atkinson, A.M. Winer, T. Ramdahl, and J.N. Pitts (1986) The formation of nitro-PAH from the gas-phase reactions of fluoranthene and pyrene with the OH radical in the presence of $NO_{x}$. Atmos. Environ., 20(12), 2339-2345. https://doi.org/10.1016/0004-6981(86)90064-8
  2. Bamford H.A. and J.E. Baker (2003) Nitro-polycyclic aromatic hydrocarbon concentrations and sources in urban and suburban atmospheres of the Mid-Atlantic region. Atmos. Environ., 37(15), 2077-2091. https://doi.org/10.1016/S1352-2310(03)00102-X
  3. Benson J.M., A.L. Brooks, Y.S. Cheng, T.R. Henderson, and J.E. White (1985) Environmental transformation of 1-nitropyrene on glass surfaces. Atmos. Environ., 19(7), 1169-1174. https://doi.org/10.1016/0004-6981(85)90200-8
  4. Harner T. and T.F. Bidleman (1998) Octanol-air partition coefficient for describing particle/gas partitioning of aromatic compounds in urban air. Environ. Sci. Technol., 32(10), 1494-1502. https://doi.org/10.1021/es970890r
  5. Hayakawa K., K. Noji, N. Tang, A. Toriba, R. Kizu, S. Sakai, and Y. Matsumoto (2001) A high-performance liquid chromatographic system equipped with on-line reducer, clean-up and concentrator columns for determination of trace levels of nitropolycyclic aromatic hydrocarbons in airborne particulates. Anal. Chim. Acta, 445(2), 205-212. https://doi.org/10.1016/S0003-2670(01)01279-X
  6. Hayakawa K., R. Kitamura, M. Butoh, N. Imaizumi, and M. Miyazaki (1991) Determination of diamino- and aminopyrenes by high performance liquid chromatography with chemiluminescence detection. Anal. Sci., 7(4), 573-577. https://doi.org/10.2116/analsci.7.573
  7. Hayakawa K., T. Murahashi, K. Akutsu, T. Kanda, N. Tang, H. Kakimoto, A. Toriba, and R. Kizu (2000) Comparison of polycyclic aromatic hydrocarbons and nitropolycyclic aromatic hydrocarbons in airborne and automobile exhaust particulates. Polycycl. Aromat. Comp., 20, 179-190. https://doi.org/10.1080/10406630008034784
  8. Hayakawa K., T. Murahashi, M. Butoh, and M. Miyazaki (1995) Determination of 1,3-, 1,6-, and 1,8-dinitropyrenes and 1-nitropyrene in urban air by high-performance liquid chromatography using chemiluminescence detection. Environ. Sci. Technol., 29(4), 928-932. https://doi.org/10.1021/es00004a012
  9. International Agency for Research on Cancer (2006) IARC Monographs on the evaluation of the carcinogenic risk humans, http://monographs.iarc.fr/index.php.
  10. Kakimoto H., M. Kitamura, Y. Matsumoto, S. Sakai, F. Kanoh, T. Murahashi, K. Akutsu, R. Kizu, and K. Hayakawa (2000) Comparison of atmospheric polycyclic aromatic hydrocarbons and nitropolycyclic aromatic hydrocarbons in Kanazawa, Sapporo and Tokyo. J. Health Sci., 46(1), 5-15. https://doi.org/10.1248/jhs.46.5
  11. Kakimoto H., Y. Matsumoto, S. Sakai, F. Kanoh, K. Arashidani, N. Tang, K. Akutsu, A. Nakajima, Y. Awata, A. Toriba, R. Kizu, and K. Hayakawa (2002) Comparison of atmospheric polycyclic aromatic hydrocarbons and nitropolycyclic aromatic hydrocarbons in an industrialized city (Kitakyushu) and two commercial cities (Sapporo and Tokyo). J. Health Sci., 48(4), 370-375. https://doi.org/10.1248/jhs.48.370
  12. Khalili N.R., P.A. Scheff, and T.M. Holsen (1995) PAH source fingerprints for coke ovens, diesel and, gasoline engines, highway tunnels, and wood combustion emissions. Atmos. Environ., 29(4), 533-542. https://doi.org/10.1016/1352-2310(94)00275-P
  13. Kizu R., K. Ishii, J. Kobayashi, T. Hashimoto, E. Koh, M. Namiki, and K. Hayakawa (2000) Antiandrogenic effect of crude extract of C-heavy oil. Mater. Sci. Eng.: C, 12, 97-102. https://doi.org/10.1016/S0928-4931(00)00165-X
  14. Lighty J.A., J.M. Veranth, and A.F. Sarofim (2000) Combustion aerosols: factors governing their size and composition and implication to human health. J. Air & Waste Manage. Assoc., 50(9), 1565-1618. https://doi.org/10.1080/10473289.2000.10464197
  15. Lin G., G. Sun, K. Tamura, N. Tang, L. Song, and W. Zhai (2005) Analysis on concentrations of atmospheric particles and PAHs/NPAHs in Fushun, P. R. China. Chin. J. Public Health, 21, 604-606.
  16. Matsumoto Y., S. Sakai, T. Kato, T. Nakajima, and H. Satoh (1998) Long-term trends of particulate mutagenic activity in the atmosphere of Sapporo. 1. Determination of mutagenic activity by the conventional tester strains TA98 and TA100 during an 18-year period (1974-1992). Environ. Sci. Technol., 32(18), 2665- 2671. https://doi.org/10.1021/es9801036
  17. Matsumoto Y., T. Nakajima, S. Sakai, I. Noguchi, and M. Akiyama (1991) Seasonal variation of the mutagenic activity of airborne particulate matter in the city of cold district. Nippon Kagaku Kaishi, 6, 837-844.
  18. Park S.S., Y.J. Kim, and C.H. Kang (2002) Atmospheric polycyclic aromatic hydrocarbons in Seoul, Korea. Atmos. Environ., 36(17), 2917-2924. https://doi.org/10.1016/S1352-2310(02)00206-6
  19. Rogge W.F., L.M. Hildemann, M.A. Mazurek, G.R. Cass, and B.R.T. Simoneit (1993) Sources of fine organic aerosol. 2. Noncatalyst and catalyst-equipped automobiles and heavy-duty diesel trucks. Environ. Sci. Technol., 27(4), 636-651. https://doi.org/10.1021/es00041a007
  20. Sicre M.A., J.C. Marty, A. Saliot, X. Aparicio, J. Grimalt, and J. Albaiges (1987) Aliphatic and aromatic hydrocarbons in different sized aerosols over the Mediterranean Sea: Occurrence and origin. Atmos. Environ., 21(10), 2247-2259. https://doi.org/10.1016/0004-6981(87)90356-8
  21. Simcik M.F., S.J. Eisenreich, and P.J. Lioy (1999) Source apportionment and source/sink relationships of PAHs in the coastal atmosphere of Chicago and Lake Michigan. Atmos. Environ., 33(30), 5071-5079. https://doi.org/10.1016/S1352-2310(99)00233-2
  22. Tang N., A. Toriba, R. Kizu, and K. Hayakawa (2003) Improvement of an automatic HPLC system for nitropolycyclic aromatic hydrocarbons: Removal of an interfering peak and increase in the number of analystes. Anal. Sci., 19, 249-253. https://doi.org/10.2116/analsci.19.249
  23. Tang N., M. Oguri, Y. Watanabe, M. Tabata, V.F. Mishukov, V. Sergienko, A. Toriba, R. Kizu, and K. Hayakawa (2002a) Comparison of atmospheric polycyclic aromatic hydrocarbons in Vladivostok, Toyama and Kanazawa. Bull. Japan Sea Res. Inst., Kanazawa Univ., 33, 77-86.
  24. Tang N., M. Tabata, V.F. Mishukov, V. Sergienko, A. Toriba, R. Kizu, and K. Hayakawa (2002b) Comparison of atmospheric nitropolycyclic aromatic hydrocarbons in Vladivostok, Kanazawa and Toyama. J. Health Sci., 48(1), 30-36. https://doi.org/10.1248/jhs.48.30
  25. Tang N., T. Hattori, R. Taga, K. Igarashi, X.Y. Yang, K. Tamura, H. Kakimoto, V.F. Mishukov, A. Toriba, R. Kizu, and K. Hayakawa (2005) Polycyclic aromatic hydrocarbons and nitropolycyclic aromatic hydrocarbons in urban air particulates and their relationship to emission sources in the Pan-Japan Sea countries. Atmos. Environ., 39(32), 5817-5826. https://doi.org/10.1016/j.atmosenv.2005.06.018
  26. Tokiwa H. and Y. Ohnishi, and H.S. Rosenkranz (1986) Mutagenicity and carcinogenicity of nitroarenes and their sources in the environment. Crit. Rev. Toxicol., 17(1), 23-58. https://doi.org/10.3109/10408448609037070
  27. Ward J.H. (1963) Hierarchical grouping to ptimize an objective function. J. Am. Stat. Assoc., 58(301), 236- 244. https://doi.org/10.1080/01621459.1963.10500845
  28. Yang X.Y., Y. Okada, N. Tang, S. Matsunaga, K. Tamura, J.-M. Lin, T. Kameda, A. Toriba, and K. Hayakawa (2007) Long-range transport of polycyclic aromatic hydrocarbons from China to Japan. Atmos. Envrion., 41(13), 2710-2718. https://doi.org/10.1016/j.atmosenv.2006.11.052

피인용 문헌

  1. Recent Changes in Atmospheric Polycyclic Aromatic Hydrocarbons (PAHs) and Nitropolycyclic Aromatic Hydrocarbons (NPAHs) in Shenyang, China vol.12, pp.4, 2011, https://doi.org/10.1080/15275922.2011.622347
  2. Characteristics of Atmospheric Polycyclic Aromatic Hydrocarbons and Nitropolycyclic Aromatic Hydrocarbons in Hanoi-Vietnam, as a Typical Motorbike City vol.32, pp.2, 2012, https://doi.org/10.1080/10406638.2012.679015
  3. Atmospheric Behaviors of Polycyclic Aromatic Hydrocarbons in East Asia vol.36, pp.3, 2014, https://doi.org/10.3123/jemsge.2014.016
  4. vol.33, pp.4, 2016, https://doi.org/10.2108/zs150211
  5. Review on the Concentrations of Benzo[a]pyrene in the Indian Environment Since 1983 vol.37, pp.4, 2017, https://doi.org/10.1080/10406638.2016.1140658
  6. Partitioning of dioxins (PCDDs/Fs) in ambient air at urban residential locations vol.11, pp.7, 2009, https://doi.org/10.1007/s13762-013-0389-7
  7. Environmental Behaviors and Toxicities of Polycyclic Aromatic Hydrocarbons and Nitropolycyclic Aromatic Hydrocarbons vol.64, pp.2, 2009, https://doi.org/10.1248/cpb.c15-00801
  8. Simultaneous Determination of Polycyclic Aromatic Hydrocarbons and Their Nitro-derivatives in Airborne Particulates by Using Two-dimensional High-performance Liquid Chromatography with On-line Reducti vol.11, pp.4, 2009, https://doi.org/10.5572/ajae.2017.11.4.283