Sr-Nd 동위원소를 이용한 국내 퇴적황사의 발원지 규명: 2007년 봄철 황사

Source Identification for Asian Dust Deposited on Domestic Area Using Sr-Nd Isotope Ratios in Spring, 2007

  • 발행 : 2008.06.28

초록

최근 국내의 황사 발생일수 및 강도가 급증하고 있으며, 사회경제적으로 황사에 의한 유형적 및 무형적 피해의 규모 및 정도가 심각한 실정이다. 현재 황사 발원지에서 사막화방지를 위한 조림/녹화사업이 국가차원은 물론 민간차원에서도 활발히 진행되고 있으나, 사막지역의 광대함, 발원지의 기후 및 토양 조건, 그리고 현지 원주민의 경제적 낙후성 등으로 인하여, 단기간 내에 그 목적을 달성하기가 어려운 실정이다. 따라서 현재 국내에서 발생하는 황사에 의한 피해를 최소화하는 것이 중요하다. 황사피해에 대처하기 위해서는 우선 황사의 발원지에 따른 황사의 유해성을 파악하고, 황사 발원지 중 어느 지역으로부터 발원하는 황사가 우리나라에 피해를 주는 지에 대한 과학적인 자료가 필요하다. 이번 연구에서는 지질물질의 기원을 추적하는 데에 많이 이용되고 있는 Sr-Nd 동위원소 조성비를 이용하여 2007년 봄철에 우리나라에 발생하였던 황사의 발원지를 규명하였다. 황사 발원지 토양 및 국내에서 발생한 퇴적황사의 Sr-Nd 동위원소 조성비의 분석결과, 황사 발원지는 황토고원일 가능성이 매우 높게 나타났으며, 오도스 사막 또한 가능성이 있는 것으로 판단된다.

Recently, the occurrence and intensity of Asian Dust have dramatically increased in Korean peninsula, resulting in severe damages to the domestic social and economic field. The most useful way to prevent the damage of Asian Dust is the restraint of the occurrence of Asian Dust itself. However, Asian dust is the one of the natural phenomena, thus there is a basic limit to manage the Asian Dust. Though it is impossible to restrain the occurrence of Asian Dust in short time at present, it is a urgent matter to minimize the damage of Asian Dust. It is necessary to construct the basic data for understanding the harmfulness of Asian Dust, and to elucidate the source area of Asian Dust in connection with the maleficence of itself. In this study, the source area of Asian Dust in spring, 2007, is investigated using the Sr-Nd isotopic ratios which is the most common method to trace the source of geological materials. The relationships of Sr-Nd isotope ratios indicate that Asian Dust was originated from Central Loess Plateau and/or Ordos desert in spring, 2007.

키워드

참고문헌

  1. Asahara Y., Tanaka, T., Kamioka, H. and Nishimura, A. (1995) Asian continental nature of $^{87}Sr/^{86}Sr$ ratios in north central Pacific sediments. Earth Planet. Sci. Lett., v. 133, p. 105-116 https://doi.org/10.1016/0012-821X(95)00048-H
  2. Asahara, Y. (1999) $^{87}Sr/^{86}Sr$ variation in north Pacific sediments: a record of the Milankovitch cycle in the past 3 million years. Earth Planet. Sci. Lett., v. 171, p. 453-464 https://doi.org/10.1016/S0012-821X(99)00158-2
  3. Biscaye, P.E., Grousset , F.E., Revel, M., Van der Gaast, S., Zielinski, G.A., Vaars, A. and Kukla, G. (1997) Asian provenance of glacial dust (stage 2) in the Greenland Ice sheet Project 2 ice core, summit, Greenland. Journal of Geophysical Research 102, 26765-26781 https://doi.org/10.1029/97JC01249
  4. Bory, A.J., Biscaye, P.E., Svensson, A. and Grousset, F. E. (2002) Seasonal variability in the origin of recent atmospheric mineral dust at Northgrip, Greenland. Earth Planet. Sci. Lett., v. 190, 123-134
  5. Chadwick, O.A., Derry, L.A., Vitousek, P.M., Huebert, B.J. and Hedin, L.O. (1999) Changing sources of nutrients during four million years of ecosystem development. Nature, v. 397, p. 491-497 https://doi.org/10.1038/17276
  6. Chen, J., Li, G., Yang, J., Rao, W., Lu, H., Balsam, W., Sun Y. and Ji, J. (2007) Nd and Sr isotopic characteristics of Chinese deserts: Implications for the provenances of Asian dust. Geochim. et Cosmochim. acta, v. 74, p. 3904-3914
  7. Chun, Y.S., Cho, K.S., Kim, Y.H. and Lee, J.K. (2003) The Features of Asian Dust Events Originated in Keoeolchin Sandy Land. J. Korean Meteor. Soc., v. 39, p. 251-263
  8. Chun, Y., Boo, K.-O., Kim, J., Park, S.-U. and Lee, M. (2001) Synopsis, transport, and physical characteristics of Asian dust in Korea. J. Geophysic. Res., v. 106, p. 18461-18469 https://doi.org/10.1029/2001JD900184
  9. Chung, Y.-S., Kim, H.-S., Dulam, J. and Harris, J. (2003) On heavy dustfall observed with explosive sandstorms in Chongwon-Chongju, Korea in 2002. Atmos. Environ., v. 37, p. 3425-3433 https://doi.org/10.1016/S1352-2310(03)00360-1
  10. Duce, R.A. (1995) Sources, distribution, and fluxes of mineral aerosols and their relationship to climate. In: Charlson, R.J. and Heintzenberg, J., Editors, 1995. Aerosol Forcing of Climate, Wiley, New York, p. 43-72
  11. Gallet, S., Jahn, B. and Torii, M. (1996) Geochemical characterization of the Luochuan loess-paleosol sequence, China, and plaleoclimatic implications. Chem. Geol., v. 133, p. 67-88 https://doi.org/10.1016/S0009-2541(96)00070-8
  12. Gao, T., Yu, X., Mu, Q., Li, H., Li, X. and Si, Y. (2003) Climatology and trends of the temporal and spatial distribution of sandstorms in inner Mongolia. Water, Air, and Soil Pollution Focus, v. 32, p. 51-66
  13. Grousset, F., Ginoux, P., Bory, A. and Biscaye, P.F. (2003) Case study of a Chinese dust plume reaching the French Alps. Geophysic. Res. Lett., v. 30, p. 10-11
  14. Husar, R.B., Tratt, D.M., Schichtel, B.A., Falke, S.R., Li, F., Jaffe, D., Gasso, S., Gill, T., Laulainen, N.S., Lu, F., Reheis, M.C., Chun, Y., Westphal, D., Holben, B.N., Gueymard, C., McKendry, I., Kuring, N., Feldman, G.C., McClain, C., Frouin, R.J., Merrill, J., DuBois, D., Vignola, F., Murayama, T., Nickovic, S., Wilxon, W.E., Sassen, K. and Sugimoto, N. (2001). The Asian dust events of April 1998. J. Geophysic. Res., v. 106, p. 18317-18330 https://doi.org/10.1029/2000JD900788
  15. Kanayama, S., Yabuki, S., Yanagisawa, F. and Motoyama, R. (2002), The chemical and strontium isotope composition of atmospheric aerosols over Japan: the contribution contribution of long-range-transported Asian dust (Kosa). Atmos. Environ., v. 36, p. 5159-5175 https://doi.org/10.1016/S1352-2310(02)00587-3
  16. Korea Meteorological Administration (KMA) (http:// www.kma.go.kr)
  17. Kurosaki, Y. and Mikami, M. (2003) Recent frequent dust events and their relation to surface wind in East Asia. Geophysic. Res. Lett., v. 30, no. 14, p. 1-4
  18. Liu, C.Q., Masuda, A., Okada, A., Yabuki, S. and Fan, Z.L. (1994) Isotope geochemistry of Quaternary deposits from the arid lands in northern China. Earth Planet. Sci. Lett., v. 127, p. 25-38
  19. Nakai, S.N., Halliday, A.N. and Rea, D.K. (1993) Provenance of dust in the Pacific Ocean. Earth Planet. Sci. Lett., v. 119, p. 143-157 https://doi.org/10.1016/0012-821X(93)90012-X
  20. Nakano T., Yokoo Y., Nishikawa M. and Koyanagi H. (2004) Regional Sr-Nd isotopic ratios of soil minerals in northern China as Asian dust fingerprints. Atmos. Environ., v. 38, p. 3061-3067 https://doi.org/10.1016/j.atmosenv.2004.02.016
  21. Sheehy, D.A. (1992) A perspective on desertification of grazing land and ecosystems in North China. Ambio, v. 21, p. 303-307
  22. Sun, J., Liu, T. and Lei, Z. (2000) Source of heavy dust fall in Beijing, China on 16 April, 1998. Geophysic. Res. Lett., v. 27, p. 2105-2108 https://doi.org/10.1029/1999GL010814
  23. Sun, J., Zhang, M. and Liu, T. (2002) Spatial and temporal characteristics of dust storms in China and its surrounding regions, 1960-1999: relations to source area and climate. J. Geophysic. Res., v. 106, p. 18325-18333
  24. Wang Y., Yang J., Chen J., Ahang, K. and Rao, W. (2007) The Sr and Nd isotopic variations of the Chinese Loess Plateau during the past 7 Ma: Implications for the East Asian winter monsson and source areas of loess. PALAEO, v. 249, p. 351-361 https://doi.org/10.1016/j.palaeo.2007.02.010
  25. Wenbo R., Jiedong Y., Jun C. and Gaojun L. (2006) Sr-Nd isotope geochemistry of eolian dust of the arid-semiarid areas in China: Implications for loess provenance and monsoon evolution. Chinese Sci. Bull., v. 51, no. 12, p. 1404-1412
  26. Wilkening, K.E., Barrie, L.A. and Engle, M.A. (2000) Trans-Pacific air pollution. Science, v. 290, p. 65-67 https://doi.org/10.1126/science.290.5489.65
  27. Xuan, J. and Sokolik, N. (2002) Characterization of sources and emission rates of minera dust in forthern China. Atmos. Environ., v. 36, p. 4863-4867 https://doi.org/10.1016/S1352-2310(02)00585-X
  28. Yokoo Y., Nakano T., Nishikawa M. and Quan H. (2001) The importance of Sr isotopic compositions as an indicator of acid-soluble minerals in arid soils in China, Water, Air, and Soil Pollution, v. 130, p. 763-768 https://doi.org/10.1023/A:1013897821493
  29. Yokoo Y., Nakano T., Nishikawa M. and Quan H. (2004) Mineralogical variation of Sr-Nd isotopic and elemental compositions in loess and desert sand from the central Loess Plateau in China as a provenance tracer of wet and dry deposition in the northwestern Pacific, Chem. Geol., v. 204, p. 45-62 https://doi.org/10.1016/j.chemgeo.2003.11.004
  30. Zhang, X., Arimoto, R., Gao, J.J., An, Z. and Wang, D. (2001) Atmopheric dust aerosol over the Tibetan plateau. J. Geophysic. Res., v. 106, p. 18471-18476 https://doi.org/10.1029/2000JD900672
  31. Zhu, Z.X., Wang, W., Wu, G., Kang, C., Zhu, F.Y. and Wang, T. (1992) China: desertification mapping and desert reclamation. World Atlas of Desertification, United Nations Environment Programme, p. 46-49
  32. Bogaard, A. E. and Stobberingh, E. E. (2000) Epidemiology of resistance to antibiotics links between animals and humans. Int. J. Antimicobiol. Ag., v. 14, p. 327-335 https://doi.org/10.1016/S0924-8579(00)00145-X