DOI QR코드

DOI QR Code

Isomorphous Substitution of Fe in Sodalite and Its Electric Characterization

  • Kim, Chy-Hyung (Department of Chemistry and Physics and Optical Engineering, Chongju University) ;
  • Jung, Chi-Sup (Department of Chemistry and Physics and Optical Engineering, Chongju University)
  • Published : 1993.04.20

Abstract

Experiment on isomorphous substitution of Al by Fe in sodalite framework was carried out using dry way method at 800-900$^{\circ}$C in nitrogen atmosphere. The substitution of Fe was possible up to 25 mole% with some deviation of symmetry in sodalite cage. The cubic unit cell parameter increased with increasing Fe content. It showed ionic semiconducting property, especially the highest conductivity and the lowest activation energy in 10 mole% Fe-substituted sodalite which could behave as a superionic conductor at above 400$^{\circ}$C. When more Fe was introduced into sodalite the electronic conductivity was improved at high temperature. But the relative electronic contribution was found to be lower compared with ionic contribution at high temperature. In infrared spectra some major absorption bands of sodalite shifted to lower wave numbers due to heavier Fe atoms substitution in Al lattice sites.

Keywords

References

  1. Hydrothermal Chemistry of Zeolites R. M. Barrer;FRS
  2. Zeolites and Clay Minerals as Sorbents and Molecular Sieves R. M. Barrer;FRS
  3. Hydrothermal Chemistry of Zeolites R. M. Barrer;FRS
  4. Studies in Surface Science and Catalysis v.28 W. J. Ball;J. Dwyer;A. A. Garforth;W. J. Smith
  5. J. Catal. v.100 R. Szostak;T. L. Thomas
  6. J. Chem. Soc., Chem. Commun. R. Szostak;T. L. Thomass
  7. J. Chem. Soc., (A) R. M. Barrer;J. F.Cole
  8. Zeolite Chemistry and Catalysis J. A. Rabo
  9. Inorganic Chemistry: Principles of Structure and Reactivity J. E. Huheey
  10. Vibrational Spectra and Structure of Silicates A. N. Lazarev;V. C. Farmer(translated ed.)
  11. U. S. Patent, 3,028,395 H. W. Kovenhowen;W. H. J. Stork

Cited by

  1. ChemInform Abstract: Isomorphous Substitution of Fe in Sodalite and Its Electric Characterization. vol.24, pp.46, 1993, https://doi.org/10.1002/chin.199346008
  2. Isomorphous gallium substitution in the alumosilicate sodalite framework: synthesis and structural studies of chloride and bromide containing phases vol.222, pp.7, 2007, https://doi.org/10.1524/zkri.2007.222.7.341
  3. Gallium substitution in the alumosilicate framework: synthesis and structural studies of hydro sodalites vol.223, pp.3, 2008, https://doi.org/10.1524/zkri.2008.0015
  4. Isomorphous framework cation substitution in the alumosilicatesodalites: synthesis, structural and spectroscopic studies of nitritecontaining phases vol.223, pp.9, 1993, https://doi.org/10.1524/zkri.2008.1018