• Title/Summary/Keyword: tritium

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Safety Analysis on the Tritium Release Accidents

  • Yang, Hee joong
    • Journal of Korean Society for Quality Management
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    • v.19 no.2
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    • pp.96-107
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    • 1991
  • At the design stage of a plant, the plausible causes and pathways of release of hazardous materials are not clearly known. Thus there exist large amount of uncertainties on the consequences resulting from the operation of a fusion plant. In order to better handle such uncertain circumstances, we utilize the Probabilistic Risk Assessment(PRA) for the safety analyses on fusion power plant. In this paper, we concentrate on the tritium release accident. We develop a simple model that describes the process and flow of tritium, by which we figure out the locations of tritium inventory and their vulnerability. We construct event tree models that lead to various levels of tritium release from abnormal initiating events. Branch parameters on the event tree are assessed from the fault tree analysis. Based on the event tree models we construct influence diagram models which are more useful for the parameter updating and analysis. We briefly discuss the parameter updating scheme, and finally develop the methodology to obtain the predictive distribution of consequences resulting from the operating a fusion power plant. We also discuss the way to utilize the results of testing on sub-systems to reduce the uncertain ties on over all system.

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Observation of Bottom Water Renewal and Export Production in the Japan Basin, East Sea Using Tritium and Helium Isotopes

  • Hahm, Do-Shik;Kim, Kyung-Ryul
    • Ocean Science Journal
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    • v.43 no.1
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    • pp.39-48
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    • 2008
  • Tritium ($^3H$ or T) has been produced mostly by atmospheric nuclear weapon tests, and entered the ocean in the form of water (HTO). As tritium exists as water itself, it has been regarded as an ideal tool to study the transport of water masses. In April 2001 we collected water samples in the western Japan Basin (WJB) for tritium and helium measurement. The timely sampling provided direct evidence of the bottom water formation, resulting in the drastic increase in tritium concentration from 0.3 TU in 2000 to 0.67 TU in 2001. Considering that the new bottom waters were found mostly in the WJB, it implies that maximum 1% of the whole bottom layer below 2600 m should be replaced with the surface water during the severely cold winter 2000 2001. $^3H-^3He$ age, showing the elapsed time since the water left from the surface, can be used to calculate oxygen utilization rate by dividing AOU by the age. Under the condition of 90% oxygen saturation in the surface water, the integration of OUR in the water column below 200 m yields net oxygen consumption of 12 mol $(O_2)m^{-2}yr^{-1}$, which corresponds to the export production of $99\;g\;C\;m^{-2}yr^{-1}$. This estimate is comparable to a previous estimate based on satellite data and implies that the ratio of export to primary production(f-ratio) is as high as 0.5 in the WJB.

Tritium Fuel Cycle of the International Thermonuclear Experimental Reactor (국제핵융합실험로 삼중수소 연료주기)

  • Song, Kyu-Min;Sohn, Soon Hwan;Chung, Hongsuk;Yun, Sei-Hun;Jung, Ki Jung
    • Korean Chemical Engineering Research
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    • v.50 no.4
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    • pp.595-603
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    • 2012
  • International Thermonuclear Experimental Reactor (ITER) will be constructed in 2019 according to the JIA (Joint Implementation Agreement) of 7 countries. The ITER fusion fuel cycle consists of fusion vacuum vessel, tritium plant and fuelling system. The tritium plant provides the functions of storage, delivery, separation, removal and recovery of the deuterium and tritium used as fusion fuels for the ITER. The tritium plant systems supply deuterium and tritium from external sources and treat all tritiated fluids from ITER operation through Storage and Delivery System (SDS), Tokamak Exhaust Processing (TEP), Isotope Separation System (ISS), Water Detritiation System & Atmosphere Detritiation System (WDS & ADS) and Analysis System (ANS). In this paper, the functions and design requirements of the major systems in the tritium plant and the status of R&D are described. Korean party is developing the SDS for ITER tritium plant and partially attaining the WDS technology through the construction and operation experience of the Wolsong Tritium Removal Facility (WTRF). Now it is expected that researchers in other fields such as chemical engineering take part in the development of upcoming technologies for ISS and TEP.

An Assessment on the Contribution of $^3$He to the Tritium Generation in the CANDU PHWR (가압중수로에서 헬륨-3이 삼중수소의 생성에 미치는 영향평가)

  • Kwak, Sung-Woo;Chung, Bum-Jin
    • Journal of Radiation Protection and Research
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    • v.22 no.2
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    • pp.119-125
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    • 1997
  • PHWR achieves high neutron economy by adopting heavy water as its moderator and coolant. On the other hand it permits much tritium generation, compared to LWR, due to the neutron capture reaction of deuterium in heavy water. Meanwhile in the reactor core, $^3He formed as the result of-decay of tritium, captures a thermal neutron and transforms to tritium again. The existing calculation models on tritium generation in PHWR neglect the contribution of $^3He$ in both moderator and coolant due to its relatively low solubility. However the neutron capture cross-section of $^3He$ is almost $1.6{\times}10^7$ times as large as that of deuterium. That means that the dissolved amount of 0.03 ppm of $^3He$ in heavy water is enough to generate the same amount of tritium as that generated by the deuterium of total heavy water in the system. This study dealt with the contribution of $^3He$ to tritium generation. As a sample case, the contribution of $^3He$ to the tritium generation in Wolsong #1 was evaluated and compared to the measured values. According to the result of this study, it is concluded that $^3He$ in coolant contributes very much to the tritium generation but that in moderator shows negligible effects due to the low solubility and $^4He$ cover gas. At the beginning of the plant operation, the contribution of $^3He$ is slightly greater than the measured value but agrees well with the measured as the operating time increases.

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A Study on Groundwater Age Dating Methods Using Tritium (삼중수소를 이용한 지하수 연령측정 방법에 관한 연구)

  • 오진석;김선준
    • Journal of the Korean Society of Groundwater Environment
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    • v.2 no.2
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    • pp.49-57
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    • 1995
  • Areas of Chungyang in Chungcheongnamdo, Cheju island and Georgia in U.S.A. were selected to calculate their groundwater ages and dispersion parameters using tritium. Piston flow model, Completely mixing model and Dispersion binomial model which calculate men residence times, and Dispersion normal model and Dispersion model(C$\_$FF) which calculate mean residence times and dispersion parameters simultaneously were applied. Since the input data, tritium concentrations of rainwaters, lack in part, tritium input function was prepared using the correlation of tritium concentrations of rainwaters of Pohang, Korea and Ottawa, Canada. Similar results of PFM and DBM reflect the intrinsical similarity of two models, assumption of low dispersion. The ages of sites of showing relatively higher tritium concentrations than other sites in the sam, region were not calculated by CMM. Since the calculations of DNM and DM(C$\_$FF/) provide the combination of wide ranges of parameters and groundwater ages, the ranges of dispersion parameters were narrowed down under the assumption that ages calculated by PFM and DBM are correct. Since large variation of tritium concentrations of outflows in a same region may reflect the different characteristics of each groundwater flow regime, using only one specific model on a whole region is not recommended.

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Evaluation Model and Experimental Validation of Tritium in Agricultural Plant (농작물의 삼중수소 오염평가 모델 개발 및 실험검증)

  • Kang Hee Suk;Keum Dong-kwon;Lee Hansoo;In Jun;Choi Yong Ho;Lee Chang Woo
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.3 no.4
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    • pp.319-328
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    • 2005
  • This paper describes a compartment dynamic model for evaluating the contamination level of kritium in agricultural plants exposed by accidentally released tritium. The present model uses a time-dependent growth equation of plant so that it can predict the effect of growth stage of plant during the exposure time. The model including atmosphere, soil and plant compartments is described by a set of nonlinear ordinary differential equations, and is able to predict time-dependent concentrations of tritium in the compartments. To validate the model, a series of exposure experiments of HTO vapor on Chinese cabbage and radish was carried out at the different growth stage of each plant. At the end of exposure, the tissue free water(TFWT) and the organically bound tritium(OBT) were measured. The measured concentrations were agreed well with model predictions.

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Methodological Study on Measurement of Hydrogen Abundance in Hydrogen Isotopes System by Low Resolution Mass Spectrometry

  • Lia, Jin-Ying;Shib, Lei;Hub, Shi-Lin
    • Mass Spectrometry Letters
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    • v.2 no.1
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    • pp.1-7
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    • 2011
  • China's rapid economic growth has resulted in significant environmental side effects. Therefore, China has been interested in reducing her dependence on foreign oil and gas by developing technologies needed for hydrogen, in addition to her increasing energy mix of nuclear and renewable energy form, such as solar and wind power. There are three isotopes of hydrogen, i.e. protium (P or H), deuterium (D), and tritium (T). Both deuterium and tritium are important materials in nuclear fuel cycle industry. Tritium is one of the critical radioactive nuclides. Planning for and implementing contamination control as a part of normal operation and maintenance activities is an important function in any hydrogen facility, especially tritium facility. The development of hydrogen isotopes analysis is the key issues in this area. Mass spectrometry (MS) with medium (about 600) and high resolution (> 1,400) is commercially available; however, the routine analysis of hydrogen isotopes is done with low-resolution MS (< 200) in China. This paper summarizes the progress of MS measurement technology for hydrogen isotope abundance in China, focusing on our lab's research program and technical status. An analyzing method has been introduced for accurate measurement of tritium abundance in the H.D.T system by low resolution MAT-253 MS. The quotient of compression ratio coefficient is determined by building up equipment for laboratory-scale preparation of secondary standard gases and by considering the difference in sensitivity between hydrogen isotopes. The results show that the measured value is reproducible within the relative error range of 0.8% for gas samples of different tritium abundance.

Model for assessing the contamination of agricultural plants by accidentally released tritium (삼중수소 사고유출로 인한 농작물 오염 평가 모델)

  • Keum, Dong-Kwon;Lee, Han-Soo;Kang, Hee-Suk;Choi, Young-Ho;Lee, Chang-Woo
    • Journal of Radiation Protection and Research
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    • v.30 no.1
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    • pp.45-54
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    • 2005
  • A dynamic compartment model was developed to appraise the level of the contamination of agricultural plants by accidentally released tritium from nuclear facility. The model consists of a set of inter-connected compartments representing atmosphere, soil and plant. In the model three categories of plant are considered: leafy vegetables, grain plants and tuber plants, of which each is modeled separately to account for the different transport pathways of tritium. The predictive accuracy of the model was tested through the analysis of the tritium exposure experiments for rice-plants. The predicted TFWT(tissue free water tritium) concentration of the rice ear at harvest was greatly affected by the absolute humidity of air, the ratio of root uptake, and the rate of rainfall, while its OBT(organically bound tritium) concentration the stowing period of the ear, the absolute humidity of air and the content of hydrogen in the organic phase. There was a good agreement between the model prediction and the experimental results lot the OBT concentration of the ear.

A Study on Bioassay of Tritium($^{3}H$) Radioacitivity (三重水素($^{3}H$) 放射能의 生理分析에 關한 硏究)

  • 황선태;오필재;김원식
    • Journal of Korean Society for Atmospheric Environment
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    • v.3 no.1
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    • pp.27-33
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    • 1987
  • The environment and biological studies of tritium have been carried out in the advanced countries since the mid 1950's. In the case of a potential tritium exposure, the usual procedure is trifium bioassay (as HTO) in human urine in order to determine the amount of tritium deposited in the body called tritium body burden. The maximum permissible body burden(MPBB) of tritium in total body is about $30{\mu}Ci/{\ell}$ for body tissue. In the bioassay, the most common investigation level for detection of tritium in urine is 1/10th of MPBB. For this bioassay project, the first priority is given to obtaining a quench correction curve. This consideration is necessary because of the variability in color of human urine specimens. Quenching effect in this case mainly is caused by the absorption of scintillation light flashes by the urine sample. By the least squares method on the statistical basis, an estimated formula for quench correction curve was determined to be Y = 0.771 + 1.836 ${\tmes}10^{-4}$X, where the efficiency(Y) was ranged from about 12% to 31% in the liquid scientillation counting. In this paper, a brief theory concerning the biological half-life of tritium and the retention formula to apply to systematically distributed tritium are described.

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