• Title/Summary/Keyword: spent fuels

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Study on Decay Characteristics Change of Spent Fuel Materials by DUPIC Fuel Cycle (DUPIC핵연료주기에 의한 사용 후 경수로핵연료의 방사선적 특성변화 분석)

  • Choi, Jong-Won;Ko, Won-Il;Lee, Jae-Sol;Park, Hyun-Soo
    • Journal of Radiation Protection and Research
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    • v.21 no.1
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    • pp.27-39
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    • 1996
  • The change in spent fuel characteristics by DUPIC fuel cycle(burnup of spent PWR fuel again in CANDU) is examined with time elapse since discharge. Major characteristics examined include isotopic concentration, radioactivity, decay heat radiotoxicity and radiation source-term of spent fuel material, which is existing in a type of spent PWR and DUPIC fuel. Behaviors of major nuclides contributing to such changes are also analyzed in terms of radionuclide concentration. From the analysis, the change in radionuclide concentration by DUPIC shows approximately 2% decrease in actinides concentration and 20% increase in fission products concentration. Radioactivity and decay heat of spent DUPIC fuel does not depend upon radionuclides concentrations, which is a unique in sence of general characteristics of spent fuel. In terms of gamma spectrum, spent DUPIC fuel shows lower values than that of spent PWR fuel by 40 to 50% in the range of $0.01{\sim}0.575$ MeV but much higher over 3.5MeV. Neutron Intensities of both spent fuels are mainly determined by $({\alpha},\;n)$ reaction and spontaneous fission reaction of actinides. Of them, especially, the spontaneous fission reaction Is a major neutron source-term, which causes that neutron intensities of spent DUPIC fuel $having{\sim}3.3$ times higher Cm-244 concentration are ${\sim}4$ times higher than that of spent PWR fuel.

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Effectiveness of the neutron-shield nanocomposites for a dual-purpose cask of Bushehr's Water-Water Energetic Reactor (VVER) 1000 nuclear-power-plant spent fuels

  • Rezaeian, Mahdi;Kamali, Jamshid;Ahmadi, Seyed Javad;Kiani, Mohammad Amin
    • Nuclear Engineering and Technology
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    • v.49 no.7
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    • pp.1563-1570
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    • 2017
  • In order to perform dry interim storage and transportation of the spent-fuel assemblies of the Bushehr Nuclear Power Plant, dual-purpose casks can be utilized. The effectiveness of different neutron-shield materials for the dual-purpose cask was analyzed through a set of calculations carried out using the Monte Carlo N-Particle (MCNP) code. The dose rate for the dual-purpose cask utilizing the recently developed materials of $epoxy/clay/B_4C$ and $epoxy/clay/B_4C/carbon$ fiber was less than the allowable radiation level of 2 mSv/h at any point and 0.1 mSv/h at 2 m from the external surface of the cask. By utilization of $epoxy/clay/B_4C$ instead of an ethylene glycol/water mixture, the dose rates on the side surface of the cask due to neutron sources and consequent secondary gamma rays will be reduced by 17.5% and 10%, respectively. The overall dose rate in this case will be reduced by 11%.

Long-term Dissolution Behavior of Cesium from Spent PWR Fuel in Contact with Compacted Bentonite under Synthetic Granitic Groundwater

  • Chun, Kwan-Sik;Kim, Seung-Soo;Bak, Seong-Jea;Park, Jongwon
    • Proceedings of the Korean Radioactive Waste Society Conference
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    • 2004.06a
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    • pp.167-173
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    • 2004
  • The amount of cesium released from the leaching of spent fuels in contact with and without the compacted bentonite bloc]t which was compacted as the density of $1.4g/\textrm{cm}^3$, up to 5.7 years were measured and the empirical formula of the fractional release rate of cesium were derived from these measured values. The empirical formulas show that the long-term release rate of cesium under a repository would become a constant, as about $3{\times}10_{-6}$ fraction/day, after a certain period. The cumulative fractions of cesium released from the spent fuel with bentonite and with copper and stainless steel sheets were steadily increased, but the fraction from bare fuel was rapidly increased and then sluggishly increased. However, the remained value except its gap inventory from the cumulative fraction of cesium released from bare fuel was almost very close to the others. This suggests that the initial release of cesium from bare fuel might be dependant on its gap inventory.

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DETERMINATION OF THE TRANSURANIC ELEMENTS INVENTORY IN HIGH BURNUP PWR SPENT FUEL SAMPLES BY ALPHA SPECTROMETRY-II

  • Joe, Kih-Soo;Song, Byung-Chul;Kim, Young-Bok;Jeon, Young-Shin;Han, Sun-Ho;Jung, Euo-Chang;Song, Kyu-Seok
    • Nuclear Engineering and Technology
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    • v.41 no.1
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    • pp.99-106
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    • 2009
  • The contents of transuranic elements ($^{237}Np$, $^{238}Pu$, $^{239}Pu$, $^{240}Pu$, $^{241}Am$, $^{244}Cm$, and $^{242}Cm$) in high-burnup spent fuel samples ($35.6{\sim}53.9\;GWd/MtU$) were determined by alpha spectrometry. Anion exchange chromatography and diethylhexyl phosphoric acid extraction chromatography were applied for the separation of these elements from the uranium matrix. The measured values of the nuclides were compared with ORIGEN-2 calculations. For plutonium, the measurements were higher than the calculations by about $2.6{\sim}32.7%$ on average according to each isotope, and those for americium and curium were also higher by about $35.9{\sim}63.1%$. However, for $^{237}Np$, the measurements were lower by about 52% on average for the samples.

Structural Analysis of Advanced Spent Fuel Conditioning Process Facility (차세대관리 종합공정 실증시설의 구조해석)

  • 구정회;정원명;조일제;국동학;유길성
    • Proceedings of the Korean Radioactive Waste Society Conference
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    • 2003.11a
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    • pp.411-420
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    • 2003
  • An advanced spent fuel conditioning process (ACP) is developing for the safe and effective management of spent fuels which arising from the domestic nuclear power plants. And its demonstration facility is under design. This facility will be prepared by modifying IMEF's reserve hot cell facility which reserved for future usage by considering the characteristics of ACP. This study presents a basic structural architecture design and analysis results of ACP hot cell including modification of the IMEF. The results of this study will be used for the detail design of ACP demonstration facility, and utilized as basic data for the licensing of the ACP facility.

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A Study on Thermal Load Management in a Deep Geological Repository for Efficient Disposal of High Level Radioactive Waste

  • Jongyoul Lee;Heuijoo Choi;Dongkeun Cho
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.20 no.4
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    • pp.469-488
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    • 2022
  • Technology for high-level-waste disposal employing a multibarrier concept using engineered and natural barrier in stable bedrock at 300-1,000 m depth is being commercialized as a safe, long-term isolation method for high-level waste, including spent nuclear fuel. Managing heat generated from waste is important for improving disposal efficiency; thus, research on efficient heat management is required. In this study, thermal management methods to maximize disposal efficiency in terms of the disposal area required were developed. They efficiently use the land in an environment, such as Korea, where the land area is small and the amount of waste is large. The thermal effects of engineered barriers and natural barriers in a high-level waste disposal repository were analyzed. The research status of thermal management for the main bedrocks of the repository, such as crystalline, clay, salt, and other rocks, were reviewed. Based on a characteristics analysis of various heat management approaches, the spent nuclear fuel cooling time, buffer bentonite thermal conductivity, and disposal container size were chosen as efficient heat management methods applicable in Korea. For each method, thermal analyses of the disposal repository were performed. Based on the results, the disposal efficiency was evaluated preliminarily. Necessary future research is suggested.

Design and Structural Safety Evaluation of Canister for Dry Storage System of PWR Spent Nuclear Fuels

  • Taehyung Na;Youngoh Lee;Taehyeon Kim;Donghee Lee
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.21 no.4
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    • pp.559-570
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    • 2023
  • The aim of this study is to ensure the structural integrity of a canister to be used in a dry storage system currently being developed in Korea. Based on burnup and cooling periods, the canister is designed with 24 bundles of spent nuclear fuel stored inside it. It is a cylindrical structure with a height of 4,890 mm, an internal diameter of 1,708 mm, and an inner length of 4,590 mm. The canister lid is fixed with multiple seals and welds to maintain its confinement boundary to prevent the leakage of radioactive waste. The canister is evaluated under different loads that may be generated under normal, off-normal, and accident conditions, and combinations of these loads are compared against the allowable stress thresholds to assess its structural integrity in accordance with NUREG-2215. The evaluation result shows that the stress intensities applied on the canister under normal, off-normal, and accident conditions are below the allowable stress thresholds, thus confirming its structural integrity.

Image reconstruction algorithm for momentum dependent muon scattering tomography

  • JungHyun Bae;Rose Montgomery;Stylianos Chatzidakis
    • Nuclear Engineering and Technology
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    • v.56 no.5
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    • pp.1553-1561
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    • 2024
  • Nondestructive radiography using cosmic ray muons has been used for decades to monitor nuclear reactor and spent nuclear fuel storage. Because nuclear fuel assemblies are highly dense and large, typical radiation probes such as x-rays cannot penetrate these target imaging objects. Although cosmic ray muons are highly penetrative for nuclear fuels as a result of their relatively high energy, the wide application of muon tomography is limited because of naturally low cosmic ray muon flux. This work presents a new image reconstruction algorithm to maximize the utility of cosmic ray muon in tomography applications. Muon momentum information is used to improve imaging resolution, as well as muon scattering angle. In this work, a new convolution was introduced known as M-value, which is a mathematical integration of two measured quantities: scattering angle and momentum. It captures the objects' quantity and density in a way that is easy to use with image reconstruction algorithms. The results demonstrate how to reconstruct images when muon momentum measurements are included in a typical muon scattering tomography algorithm. Using M-value improves muon tomography image resolution by replacing the scattering angle value without increasing computation costs. This new algorithm is projected to be a standard nondestructive radiography technique for spent nuclear fuel and nuclear material management.