• Title/Summary/Keyword: radionuclide distribution

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Effects of Temperature on the Uptake and Retention of Cesium-137 by the Clam Cyclina sinensis (가무락조개에 의한 세슘-137 의 농축(濃縮)과 잔류(殘留)에 미치는 온도(溫度)의 영향)

  • Yoo, Byung-Sun;Lee, Jeong-Ho;Lee, Su-Rae
    • Korean Journal of Environmental Agriculture
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    • v.2 no.1
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    • pp.24-29
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    • 1983
  • The effects of temperature on the uptake of $^{137}Cs$ from seawater and on the retention after its uptake by the clam Cycling sinensis was investigated under laboratory conditions. The clams exhibited a greater bioaccumulation of $^{137}Cs$ in $25^{\circ}C$-acclimated animals than those acclimated at $15^{\circ}C$. The viscera of the clams reached the highest bioconcentration factor after 14 days uptake from seawater, but the tissue distribution pattern of $^{137}Cs$ was little influenced, if any, by the uptake temperature. The uptake rate slightly decreased with an increase of temperature in order of $10^{\circ}C$. The radionuclide accumulated in clams was released again in a radionuclide-free seawater according to a two-exponential compartment model. A temperature increase of $10^{\circ}C$ reduced the biological half-life of the long-lived component with a factor of about two, whereas it caused no change in the short-lived component.

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Establishing the Concept of Buffer for a High-level Radioactive Waste Repository: An Approach (고준위폐기물처분장의 완충재 개념 도출: 접근방안)

  • Lee, Jae Owan;Lee, Minsoo;Choi, Heuijoo
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.13 no.4
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    • pp.283-293
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    • 2015
  • The buffer is a key component of the engineered barrier system in a high-level radioactive waste (HLW) repository. The present study reviewed the requirements and functional criteria of the buffer reported in literature, and also based on the results, proposed an approach to establish a buffer concept which is applicable to an HLW repository in Korea. The hydraulic conductivity, radionuclide-retarding capacity (equilibrium distribution coefficient and diffusion coefficient), swelling pressure, thermal conductivity, mechanical properties, organic carbon content, and illitization rate were considered as major technical parameters for the functional criteria of the buffer. Domestic bentonite (Ca-bentonite) and, as an alternative, MX-80 (Na-bentonite) were proposed for the buffer of an HLW repository in Korea. The technical specifications for those proposed bentonites were set to parameter values that conservatively satisfy Korea's functional criteria for the Ca-bentonite and Swedish criteria for the Na-bentonite. The thickness of the buffer was determined by evaluating the means of shear behavior, radionuclide release, and heat conduction, which resulted in the proper buffer thickness of 0.25 to 0.5 m. However, the final thickness of the buffer should be determined by considering coupled thermal-hydraulic-mechanical evaluation and economics and engineering aspects as well.

Comparison of Compton Image Reconstruction Algorithms for Estimation of Internal Radioactivity Distribution in Concrete Waste During Decommissioning of Nuclear Power Plant (원전 해체 시 방사성 콘크리트 폐기물 내부 방사능 분포 예측을 위한 컴프턴 영상 재구성 방법의 비교)

  • Lee, Tae-Woong;Jo, Seong-Min;Yoon, Chang-Yeon;Kim, Nak-Jeom
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.18 no.2
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    • pp.217-225
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    • 2020
  • Concrete waste accounts for approximately 70~80% of the total waste generated during the decommissioning of nuclear power plants (NPPs). Based upon the concentration of each radionuclide, the concrete waste from the decommissioning can be used in the determination of the clearance threshold used to classify waste as radioactive. To reduce the cost of radioactive concrete waste disposal, it is important to perform decontamination before self-disposal or limited recycling. Therefore, it is necessary to estimate the internal radioactivity distribution of radioactive concrete waste to ensure effective decontamination. In this study, the performance metrics of various Compton reconstruction algorithms were compared in order to identify the best strategy to estimate the internal radioactivity distribution in concrete waste during the decommissioning of NPPs. Four reconstruction algorithms, namely, simple back-projection, filtered back-projection, maximum likelihood expectation maximization (MLEM), and energy-deconvolution MLEM (E-MLEM) were used as Compton reconstruction algorithms. Subsequently, the results obtained by using these various reconstruction algorithms were compared with one another and evaluated, using quantitative evaluation methods. The MLEM and E-MLEM reconstruction algorithms exhibited the best performance in maintaining a high image resolution and signal-to-noise ratio (SNR), respectively. The results of this study demonstrate the feasibility of using Compton images in the estimation of the internal radioactive distribution of concrete during the decommissioning of NPPs.

Characteristics of Occurrence and Distribution of Natural Radioactive Materials, Uranium and Radon in Groundwater of the Danyang Area (단양지역 지하수중 자연방사성물질 우라늄과 라돈의 산출과 분포특징)

  • Cho, Byong Wook;Kim, Moon Su;Kim, Tae Seung;Yun, Uk;Lee, Byeong Dae;Hwang, Jae Hong;Choo, Chang Oh
    • The Journal of Engineering Geology
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    • v.23 no.4
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    • pp.477-491
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    • 2013
  • Natural radionuclides in groundwater in the Danyang area were investigated to characterize the behaviors of uranium and radon with respect to lithology and physico-chemical components, which can aid our understanding of their occurrence, properties, and origins. To this end, a total of 100 groundwater samples were collected and analyzed, and radionuclide levels were used to construct detailed concentration maps. The water type of the groundwater, assessed using a Piper diagram, is mainly Ca-Na-$HCO_3$. The concentrations of uranium range from 0.02 to $251.0{\mu}g/L$ (average, $3.85{\mu}g/L$) and only 1% exceed USEPA's MCL (Maximum Contaminant Level). Uranium is enriched in groundwaters of Cretaceous granites and Precambrian metamorphic rocks, whereas it is depleted in groundwaters of sedimentary rocks. The concentrations of radon range from 13 to 28,470 pCi/L (average, 2397 pCi/L). Only 15% of the samples exceed AMCL (Alternative Maximum Contaminant Level) of 4000 pCi/L. The radon concentration is highest in groundwater of Cretaceous granites and lowest in groundwater of sedimentary rocks. In conclusion, the distribution and occurrence of radionuclides are intimately related to the basic geological characteristics of the rocks in which the radiogenic minerals are primarily contained. The behavior of uranium is only weakly related to that of radon (correlation coefficient = 0.15). There are also weak correlations between radionuclides and the main chemical components, pH, EC, Eh, and well depth. Of note, the correlation coefficient between radon and $SiO_2$ is 0.68, and that between radon and $HCO_3$ is -0.48. Factor analysis shows that radionuclides behave somewhat independently of each other because there are no significant factors that control the behavior of chemical components as well as radionuclides. The detailed concentration maps during this study will be used to establish useful database of radionuclide distribution and geological properties throughout Korea.

Distribution of Some Environmental Radionuclides in Rocks and Soils of Guemjeong-Gu Area in Busan, Korea (부산시 금정구 일대 암석 및 토양에서 일부 환경방사성 핵종들의 분포 특성)

  • Lee, Hyo-Min;Moon, Ki-Hoon;Kim, Jin-Seop;Ahn, Jung-Keun;Kim, Hyun-Chul
    • The Journal of the Petrological Society of Korea
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    • v.17 no.3
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    • pp.179-190
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    • 2008
  • The distribution characteristics of some major environmental radionuclides ($^{40}K$, $^{228}Ac$, $^{226}Ra$, $^{222}Rn$) and U in rocks, soils and soil gas were studied at Geumjeong-Gu, Busan, Korea. The activities of radionuclides in granitic rocks are decreased in the odor of $^{40}K$>thorium decay series>uranium decay series. This reveals that Th was relatively more enriched in granitic rocks than U. The U content and activity of $^{226}Ra$ and $^{228}Ac$, however, don't reflect the fractionation sequence of granitic rocks in the study area. The activities of all these radionuclides and U content in soils are generally higher than in rocks, and their distribution in rocks, soils and soil gas show very low co-relationship. These facts indicate that the activities of radionuclides in soil and soil gas were greatly affected by leaching and adsorption properties of the radionuclides and their parents during weathering and pedogenetic process rather than their concentrations in parent rocks.

Implementation of an Architecture for the Dismantling Digital Mock-up System (해체 디지털목업시스템 아키텍쳐 구현)

  • Park Hee-Seoung;Kim Sung-Kyun;Lee Kune-Woo;Oh Won-Jin
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.3 no.3
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    • pp.237-247
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    • 2005
  • It is necessary to forecast the various dismantling activities prior to dismantling nuclear facilities by using various software instead of a physical mock-up system because the dismantling in a contaminated with radioactivity cause the results of an unexpected situation. The component that needs to develop a dismantling mock-up system was examined. There are many component systems such as a decommissioning database system,3D dosimetric mapping that represents a distribution of a radionuclide contamination, a component of modeling for nuclear facility and devices include the decontamination and decommissioning. The research of software architecture about these components was carried out because these component systems that have been independently doesn't describe not only to visual an activities of Decontamination and Decommissioning(D&D) but also to evaluate it. The result was established an architecture that consist of an visualization module which could be visualized an D&D activities and a simulation module which can be evaluated a dismantling schedule and decommissioning cost.

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Synthesis and Characterization of Polyphase Waste Form to Immobilize High Level Radioactive Wastes (고준위 방사성 폐기물의 고정화를 위한 다상 고화체 합성)

  • Chae Soo-Chun;Jang Young-Nam;Bae In-Kook;Ryu Kyung-Won
    • Economic and Environmental Geology
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    • v.39 no.2 s.177
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    • pp.173-180
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    • 2006
  • The synthesis of polyphase waste form, which is an immobilization matrix fur the high level radioactive wastes, was performed with the mixed composition of garnet and spinel $(Gd_3Fe_5O_{12}+(Ni_xMn_{1-x})(Fe_yCr_{1-y})_2O_4)$ in the range of 1200 to $1400^{\circ}C$. The phases synthesized from all stoichiometric compositions were garnet, perovskite, and spinel. Especially, garnet was synthesized only in the composition of the highest content of Fe(y=0.9), whereas it was not synthesized in other compositions. This result indicated that the content of Fe was closely related to the formation of garnet. The composition of garnet revealed that the content of Gd was exceeded and that of Fe was depleted. Preferential distribution of elements in the phases can be attributed to the nonstoichiometric composition of garnet.

An Analysis of Exposure Dose on Hands of Radiation Workers using a Monte Carlo Simulation in Nuclear Medicine (몬테카를로 모의 모사를 이용한 핵의학과 방사선작업종사자의 손에 대한 피폭선량 분석)

  • Jang, Dong-Gun;Kang, Sesik;Kim, Junghoon;Kim, Changsoo
    • Journal of radiological science and technology
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    • v.38 no.4
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    • pp.477-482
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    • 2015
  • Workers in nuclear medicine have performed various tasks such as production, distribution, preparation and injection of radioisotope. This process could cause high radiation exposure to wokers' hand. The purpose of this study was to investigate shielding effect for r-rays of 140 and 511 keV by using Monte-carlo simulation. As a result, it was effective, regardless of lead thickness for radiation shielding in 140 keV r-ray. However, it was effective in shielding material with thickness of more than only 1.1 mm in 511keV r-ray. And also it doesn't effective in less than 1.1 mm due to secondary scatter ray and exposure dose was rather increased. Consequently, energy of radionuclide and thickness of shielding materials should be considered to reduce radiation exposure.

Calculation of Effective Half-life of Gamma Emission Radionuclide using Bio-kinetic Model (생체역동학 모델을 이용한 감마선 방출 핵종의 유효반감기 계산)

  • Lee, Sang-Kyung;Jeong, Kyu-Hwan;Lee, Ji-Yon;Kim, Bong-Gi;Kim, Jung-Min
    • Journal of Radiation Industry
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    • v.12 no.4
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    • pp.277-285
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    • 2018
  • Patients administered radioisotope for medical purposes are regulated by each country to quarantine them until their body's radioactivity contents decrease below release criteria. To predict the quarantine period and provide it to medical staffs and patients, it is necessary to approach the assessment of the exposure dose of persons due to patients in a realistic manner. For this purpose, a whole-body effective half-life should be applied to the dose assessment equation instead of the physical half-life. In this study, we constructed a bio-kinetic model for each nuclear species based on the ICRP publication to obtain a whole-body effective half-life of 10 unsealed gamma-ray emitting nuclei from the notification of Nuclear Safety and Security Commission, and calculated the effective half-life mathematically by simulating the distribution of the radioisotope administered in the whole body as well as each organ scale. The whole-body effective half-life of $^{198}Au$, $^{67}Ga$, $^{123}I$, $^{111}In$, $^{186}Re$, $^{99m}Tc$, and $^{201}TI$ were 1,93, 2.57, 0.295, 2.805, 1.561, 0.245, and 2.397 days respectively. However, it was found to be undesirable to offer a single value of the effective half-life of $^{125}I$, $^{131}I$, and $^{169}Yb$ because the changes in the effective half-life show no linearity. A bio-kinetic model created for the internal exposure assessment has been shown to be possible to calculate the effective half-life of radioisotopes administered in the patient's body, but subsequent studies of radiolabeled compounds are required as well.

Sorption and Migration Studies of Fission Products for Ground Waste Disposal

  • Lee, Sang-Hoon;Chun, Kwan-Sik;Yoon, Young-Ku
    • Nuclear Engineering and Technology
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    • v.10 no.3
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    • pp.153-163
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    • 1978
  • The problems of solid waste disposal into the ground in connection with environmental aspects in the vicinity of a site would be very significant, though ground disposal for solid waste is safe and economical method. Studies of the waste-movement and migration of radionuclides (Sr-90 and Cs-137) for the disposal into the ground were performed under laboratory and field conditions. Affinity of the soils for radionuclide solution was higher than that in the acid solution. The sorption of radionuclides by the soils showed a time-dependent reation. The migration rates of radiostrontium and radiocesium were a range of 3.73$\times$10$^{-3}$ to 10.9$\times$10$^{-3}$ cm/day. The nuclides in the soil migrate much more slowly than the water, probably due to its high exchange capacity. The observed distribution of tritium was compared with that calculated by a mathematical model based on diffusivity. This study suggests that the tritiated water can be used to trace the movement of ground water.

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