• 제목/요약/키워드: nuclide analysis

검색결과 78건 처리시간 0.025초

영광 원자력발전소 주변해역 표층퇴적물의 입도와 원소분포 특성 (Characteristics of Particles Size and Element Distribution in the Coastal Bottom Sediments in the Vicinity of Youngkwang Nuclear Power Plant)

  • 은고요나
    • 자원환경지질
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    • 제33권3호
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    • pp.195-204
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    • 2000
  • order to investigate physical characteristics and element concentrations of sediments, coastal bottom sediments were collected at 20 stations in the vicinity of Youngkwang Nuclear Power Plant. After air drying of samples in the laboratory. article size distribution was examined by Master sizer (X-350F), radio-activity by HPGe ${\gamma}$-spectrphotometer, and element concentrations by ICP-AES and AAS. According to particle size analysis , sediments are mainly composed of silt fraction weith 23% of sand, 65% of silt and 12% of clay on average. Most sediments are derived from muddy environment that silt dominates with the characteristics of 5.3${\varsigma}$ mean particle size, poorly sorted, very fine skewed and lepto-kurtic. Only two sediments are well sorted with sandy silt owing to wind, winnowing action, tide and current andits complex reactions. Element concentrations in the coastal bottom sediments are relatively high at finer sediment and show significant relationship with grain size. Index of geoaccumulation by heavy metals at every sampling station is classified as practically unpolluted. The radioactivities of the sediments were measured for 15 isotope elements, and 2 elements of K-40 and Cs-137 were detected in most sediments. The K-40 is the natural nuclide and the artificial nuclide of Cs-137 was thought to be derived from the fallout of past nuclear weapon test. The results of correlation coefficient between grain size and radioactivity shows that the activity of Cs-137 significantly increases in finer grain.

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An assessment of the applicability of multigroup cross sections generated with Monte Carlo method for fast reactor analysis

  • Lin, Ching-Sheng;Yang, Won Sik
    • Nuclear Engineering and Technology
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    • 제52권12호
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    • pp.2733-2742
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    • 2020
  • This paper presents an assessment of applicability of the multigroup cross sections generated with Monte Carlo tools to the fast reactor analysis based on transport calculations. 33-group cross section sets were generated for simple one- (1-D) and two-dimensional (2-D) sodium-cooled fast reactor problems using the SERPENT code and applied to deterministic steady-state and depletion calculations. Relative to the reference continuous-energy SERPENT results, with the transport corrected P0 scattering cross section, the k-eff value was overestimated by 506 and 588 pcm for 1-D and 2-D problems, respectively, since anisotropic scattering is important in fast reactors. When the scattering order was increased to P5, the 1-D and 2-D problem errors were increased to 577 and 643 pcm, respectively. A sensitivity and uncertainty analysis with the PERSENT code indicated that these large k-eff errors cannot be attributed to the statistical uncertainties of cross sections and they are likely due to the approximate anisotropic scattering matrices determined by scalar flux weighting. The anisotropic scattering cross sections were alternatively generated using the MC2-3 code and merged with the SERPENT cross sections. The mixed cross section set consistently reduced the errors in k-eff, assembly powers, and nuclide densities. For example, in the 2-D calculation with P3 scattering order, the k-eff error was reduced from 634 pcm to -223 pcm. The maximum error in assembly power was reduced from 2.8% to 0.8% and the RMS error was reduced from 1.4% to 0.4%. The maximum error in the nuclide densities at the end of 12-month depletion that occurred in 237Np was reduced from 3.4% to 1.5%. The errors of the other nuclides are also reduced consistently, for example, from 1.1% to 0.1% for 235U, from 2.2% to 0.7% for 238Pu, and from 1.6% to 0.2% for 241Pu. These results indicate that the scalar flux weighted anisotropic scattering cross sections of SERPENT may not be adequate for application to fast reactors where anisotropic scattering is important.

放射能 落塵의 核種檢出의 一例 (Radioactive Nuclide Identification of a Fall-Out Sample in Korea)

  • 김종국
    • 대한화학회지
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    • 제6권2호
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    • pp.155-157
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    • 1962
  • A tiny dust found at the balcony of the Institute indicated about 8,0000 counts per minute by T.G.C.-2 Geiger-Muller tube (1.8mg/$cm^2$ window-thickness) at the distance of 2cm from the window. The main fission fragments, as identified by the present analysis, are 12.5day Ba-140 and 33.1 day Ce-141. The gamma energies were determined using $2"{\times}2"$ NaI(Tl) scintillation detector connected to RCL-256 channel pulse heigt analyzer. The beta energies were evaluated by Feather plot.

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DEVELOPMENT OF THE DUAL COUNTING AND INTERNAL DOSE ASSESSMENT METHOD FOR CARBON-14 AT NUCLEAR POWER PLANTS

  • Kim, Hee-Geun;Kong, Tae-Young;Han, Sang-Jun;Lee, Goung-Jin
    • Journal of Radiation Protection and Research
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    • 제34권2호
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    • pp.55-64
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    • 2009
  • In a pressurized heavy water reactor (PHWR), radiation workers who have access to radiation controlled areas submit their urine samples to health physicists periodically; internal radiation exposure is evaluated by the monitoring of these urine samples. Internal radiation exposure at PHWRs accounts for approximately 20 $\sim$ 40% of total radiation exposure; most internal radiation exposure is attributed to tritium. Carbon-14 is not a dominant nuclide in the radiation exposure of workers, but it is one potential nuclide to be necessarily monitored. Carbon-14 is a low energy beta emitter and passes relatively easily into the body of workers by inhalation because its dominant chemical form is radioactive carbon dioxide ($^{14}CO_2$). Most inhaled carbon-14 is rapidly exhaled from the worker's body, but a small amount of carbon-14 remains inside the body and is excreted by urine. In this study, a method for dual analysis of tritium and carbon-14 in urine samples of workers at nuclear power plants is developed and a method for internal dose assessment using its excretion rate result is established. As a result of the developed dual analysis of tritium and carbon-14 in urine samples of radiation workers who entered the high radiation field area at a PHWR, it was found that internal exposure to carbon-14 is unlikely to occur. In addition, through the urine counting results of radiation workers who participated in the open process of steam generators, it was found that the likelihood of internal exposure to either tritium or carbon-14 is extremely low at pressurized water reactors (PWRs).

Development of the Defect Analysis Technology for CANDU Spent Fuel

  • Kim, Yong-Chan;Lee, Jong-Hyeon
    • 방사성폐기물학회지
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    • 제19권2호
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    • pp.215-223
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    • 2021
  • The domestic CANDU nuclear power plants have been operated for a long time and various unforeseen spent fuel defects have been discovered. As the spent fuel defects are important factors in the safety of the nuclear power plant, a study on the analysis of the spent fuel defects to prevent their recurrence is necessary. However, in cases where the fuel rods inside the fuel assembly are defected, it is difficult to dismantle the fuel assembly owing to their welded structure and the facility conditions of the plant. Therefore, it is impossible to analyze the spent fuel defect because it is difficult to visually check the shape of the fuel defect. To resolve these problems, an analysis technology that can predict the number of defected fuel rods and defect size was developed. In this study, we developed a methodology for investigating the root cause of spent fuel defects using a database of the earlier fuel defects in the plants. It is anticipated that in the future this analysis technology will be applied when spent fuel defects occur.

플라스틱 Scintillator와 NaI(TI) 검출기를 이용한 다수의 방사선원 위치를 3차원으로 판별하는 측정시스템 개발 (Development of 3D Radiation Position Identification System of Multiple Radiation Sources using Plastic Scintillator and NaI(TI) Detector)

  • 곽동훈;고태영;이승호
    • 전기전자학회논문지
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    • 제22권3호
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    • pp.638-644
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    • 2018
  • 본 논문에서는 플라스틱 Scintillator와 NaI(TI) 검출기를 이용하여 움직이는 차량 적재물에 존재하는 다수의 방사선원 위치를 3차원으로 판별하는 측정시스템을 제안한다. 제안하는 시스템은 방사선량 측정용 플라스틱 Scintillator, 2채널 펄스 카운터, 핵종 분석용 NaI(TI) 검출기 및 1채널 MCA Board 등으로 구성된다. 방사선원 위치판별 알고리즘은 방사선량의 거리의 자승에 반비례한 특성($1/r^2$)과 장치와의 각도(${\theta}$)에 따른 보상을 통해 계산된 방사선원의 CPS 값의 비율을 SVM 분류를 통하여 방사선원의 위치(X, Y)를 구할 수 있다. (Z) 좌표 값은 단위 시간당 움직이는 대상체의 속도에 따라 정해지게 되며 이는 단위주기당 백그라운드 스펙트럼을 제외한 순수 핵종의 스펙트럼을 분석한 후 핵종 유무 판별을 진행한 뒤 해당 핵종의 위치를 판별하게 된다. 본 논문에서 제안한 시스템의 위치 판별 실험 결과 ${\pm}1m$ 이내의 국제표준오차를 나타내었다. 따라서 본 논문에서 제안한 시스템의 유효성이 입증되었다.

유리화공정 고온영역에서의 방사성 배기체 유동해석 (Numerical Analysis of Off-Gas Flow in Hot Area of the Vitrification Plant)

  • 박승철;강원구;황태원
    • 방사성폐기물학회지
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    • 제5권3호
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    • pp.213-220
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    • 2007
  • 유리화공정 고온영역에서의 방사성 배기체 유동해석을 해석하기 위하여 상용 수치해석 범용 툴인 FLUENT를 이용하여 적용성을 검토하여 보았다. 수치해석을 통하여 유리화공정 원형설비에 영향을 미치는 인자를 파악하였는데, 저온용응로, 배관냉각기 및 고온필터 등의 세 단계로 나누어 해석을 수행하였다. 저온용융로의 경우 폐기물 처리용량에 따른 해석과 저온용융로 내부 과잉산소 공급 비에 따른 연소지연 가능성에 대한 수치해석을 수행하였다. 배관냉각기의 경우에는 각종 수치 모델 및 외벽 열전달계수를 확보하였으며 또한 방사성 핵종의 거동을 모사할 수 있는 수치적 기업을 검토하였다. 이러한 방법론을 적용하여 핵종의 열교환기 내부에서의 응고 특성에 대하여 고찰하였다. 수평 유입형식의 인입관이 있는 일반적인 형상과 유입구가 필터 내부에 수직으로 있는 고온필터의 수치해석을 통하여 인입관의 위치에 따른 고온필터의 작동 특성을 비교하였다.

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유리화공정 고온영역에서의 방사성 배기체 유동해석 (Numerical Analysis of Off-Gas Flow in Hot Area of the Vitrification Plant)

  • 박승철;김병렬;신상운;이진욱;강원구;홍석진
    • 한국방사성폐기물학회:학술대회논문집
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    • 한국방사성폐기물학회 2005년도 추계 학술대회 논문집
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    • pp.69-78
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    • 2005
  • 유리화공정 고온영역에서의 방사성 배기체 유동해석을 통하여 해석에 적합한 모델을 개발하였다. 개발된 모델을 이용한 수치해석을 통하며 유리화공정 원형설비에 영향을 미치는 인자를 파악하였는데, 저온용융로. 배관냉각기 및 고온필터 등의 세 단계로 나누어 해석을 수행하였다. 저온용융로의 경우 폐기물 처리용량에 따른 해석과 저온용융로 내부 과잉산소 공급 비에 따른 연소지연 가능성에 대한 수치해석을 수행하였다. 배관냉각기의 경우에는 각종 수치 모델 및 외벽 열전달계수를 확보하였으며 또한 방사성 핵종의 거동을 모사할 수 있는 수치적 모델을 개발하였다. 이러한 방법론을 적용하여 핵종의 열교환기 내부에서의 응고 특성에 대하여 고찰하였다. 수평 유입형식의 인입관이 있는 일반적인 형상과 유입구가 필터 내부에 수직으로 있는 고온필터의 수치해석을 통하여 인입관의 위치에 따른 고온필터의 작동 특성을 비교하였다.

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Feasibility Study of Beta Detector for Small Leak Detection inside the Reactor Containment

  • Jang, JaeYeong;Schaarschmidt, Thomas;Kim, Yong Kyun
    • Journal of Radiation Protection and Research
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    • 제43권4호
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    • pp.154-159
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    • 2018
  • Background: To prevent small leakage accidents, a real-time and direct detection system for small leaks with a detection limit below that of existing systems, e.g. $0.5gpm{\cdot}hr^{-1}$, is required. In this study, a small-size beta detector, which can be installed inside the reactor containment (CT) building and detect small leaks directly, was suggested and its feasibility was evaluated using MCNPX simulation. Materials and Methods: A target nuclide was selected through analysis of radiation from radionuclides in the reactor coolant system (RCS) and the spectrum was obtained via a silicon detector simulated in MCNPX. A window was designed to reduce the background signal caused by other nuclides. The sensitivity of the detector was also estimated, and its shielding designed for installation inside the reactor CT. Results and Discussion: The beta and gamma spectrum of the silicon detector showed a negligible gamma signal but it also contained an undesired peak at 0.22 MeV due to other nuclides, not the $^{16}N$ target nuclide. Window to remove the peak was derived as 0.4 mm for beryllium. The sensitivity of silicon beta detector with a beryllium window of 1.7 mm thickness was derived as $5.172{\times}10^{-6}{\mu}Ci{\cdot}cc^{-1}$. In addition, the specification of the shielding was evaluated through simulations, and the results showed that the integrity of the silicon detector can be maintained with lead shielding of 3 cm (<15 kg). This is a very small amount compared to the specifications of the lead shielding (600 kg) required for installation of $^{16}N$ gamma detector in inside reactor CT, it was determined that beta detector would have a distinct advantage in terms of miniaturization. Conclusion: The feasibility of the beta detector was evaluated for installation inside the reactor CT to detect small leaks below $0.5gpm{\cdot}hr^{-1}$. In future, the design will be optimized on specific data.

Verification of a novel fuel burnup algorithm in the RAPID code system based on Serpent-2 simulation of the TRIGA Mark II research reactor

  • Anze Pungercic;Valerio Mascolino ;Alireza Haghighat;Luka Snoj
    • Nuclear Engineering and Technology
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    • 제55권10호
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    • pp.3732-3753
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    • 2023
  • The Real-time Analysis for Particle-transport and In-situ Detection (RAPID) Code System, developed based on the Multi-stage Response-function Transport (MRT) methodology, enables real-time simulation of nuclear systems such as reactor cores, spent nuclear fuel pools and casks, and sub-critical facilities. This paper presents the application of a novel fission matrix-based burnup methodology to the well-characterized JSI TRIGA Mark II research reactor. This methodology allows for calculation of nuclear fuel depletion by combination and interpolation of RAPID's burnup dependent fission matrix (FM) coefficients to take into account core changes due to burnup. The methodology is compared to experimentally validated Serpent-2 Monte Carlo depletion calculations. The results show that the burnup methodology for RAPID (bRAPID) implemented into RAPID is capable of accurately calculating the keff burnup changes of the reactor core as the average discrepancies throughout the whole burnup interval are 37 pcm. Furthermore, capability of accurately describing 3D fission source distribution changes with burnup is demonstrated by having less than 1% relative discrepancies compared to Serpent-2. Good agreement is observed for axially and pin-wise dependent fuel burnup and nuclear fuel nuclide composition as a function of burnup. It is demonstrated that bRAPID accurately describes burnup in areas with high gradients of neutron flux (e.g. vicinity of control rods). Observed discrepancies for some isotopes are explained by analyzing the neutron spectrum. This paper presents a powerful depletion calculation tool that is capable of characterization of spent nuclear fuel on the fly while the reactor is in operation.