• Title/Summary/Keyword: irradiated fuel

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Performance of U3Si-Al dispersion fuel at HANARO full-power condition

  • Chae, Heetaek;Lee, Choong Sung;Park, Jong Man;Kim, Heemoon;Kim, Yeon Soo
    • Nuclear Engineering and Technology
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    • v.50 no.6
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    • pp.899-906
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    • 2018
  • The irradiation performance of $U_3Si$ dispersion fuel in an Al matrix, $U_3Si-Al$, under the Hi-Flux Advanced Neutron Application Reactor (HANARO) design full-power condition of 30 MW was tested for full-power qualification of the fuel. A test assembly was fabricated containing 18 fuel rods made with atomized $U_3Si$ powder manufactured at the Korea Atomic Energy Research Institute. The test assembly was irradiated for 188 full-power operation days in the HANARO subject to the normal fuel-loading scheme and achieved about 60 at% U-235 average burnup and 75 at% U-235 peak burnup. The maximum linear power of the test assembly was 98 kW/m. Nondestructive and destructive postirradiation examinations were conducted. The measured postirradiation examination data were compared with data from previous irradiations and the design criteria required for HANARO fuel. Consequently, it was concluded that in-pile performance was acceptable and fuel integrity was maintained, and the behavior satisfied the fuel design requirements.

Improvement of delayed hydride cracking assessment of PWR spent fuel during dry storage

  • Hong, Jong-Dae;Yang, Yong-Sik;Kook, Donghak
    • Nuclear Engineering and Technology
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    • v.52 no.3
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    • pp.614-620
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    • 2020
  • In a previous study, delayed hydride cracking (DHC) assessment of pressurized water reactor (PWR) spent fuel during dry storage using the threshold stress intensity factor (KIH) was performed. However, there were a few limitations in the analysis of the cladding properties, such as oxide thickness and mechanical properties. In this study, those models were modified to include test data for irradiated materials, and the cladding creep model was introduced to improve the reliability of the DHC assessment. In this study, DHC susceptibility of PWR spent fuel during dry storage depending on the axial elevation was evaluated with the improved assessment methodology. In addition, the sensitivity of affecting parameters such as fuel burnup, hydride thickness, and crack aspect ratio are presented.

Determination of plutonium and uranium content and burnup using six group delayed neutrons

  • Akyurek, T.;Usman, S.
    • Nuclear Engineering and Technology
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    • v.51 no.4
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    • pp.943-948
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    • 2019
  • In this study, investigation of spent fuel was performed using six group delayed neutron parameters. Three used fuels (F1, F2, and F11) which are burnt over the years in the core of Missouri University of Science and Technology Reactor (MSTR), were investigated. F16 fresh fuel was used as plutonium free fuel element and compared with irradiated used fuels to develop burnup and Pu discrimination method. The fast fission factor of the MSTR was calculated to be 1.071 which was used for burnup calculations. Burnup values of F2 and F11 fuel elements were estimated to be 1.98 g and 2.7 g, respectively. $^{239}Pu$ conversion was calculated to be 0.36 g and 0.50 g for F2 and F11 elements, respectively.

Modeling on thermal conductivity of MOX fuel considering its microstructural heterogeneity

  • Lee, Byung-Ho;Koo, Yang-Hyun;Sohn, Dong-Seong
    • Proceedings of the Korean Nuclear Society Conference
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    • 1999.10a
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    • pp.247-247
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    • 1999
  • This paper describes a new mechanistic thermal conductivity model considering the heterogeneous microstructure of MOX fuel. Even though the thermal conductivities of MOX have been investigated numerously by experimental measurements and theoretical analyses, they show the large scattering making the performance analysis of MOX fuel difficult. Therefore, a thermal conductivity model that depends on the heterogeneous microstructure of MOX fuel has been developed by using a general two-phase thermal conductivity model. In order to apply this model for developing the thermal conductivity for heterogeneous MOX fuel, the fuel is assumed to consist of Purich particles and U02 matrix including Pu02 in solid solution. Since little relevant data on Purich particles is available, FIGARO and SiemensKWU results are only used to characterize the microstructure of unirradiated and irradiated fuel. Philliponneaus and HALDEN models are selected for the local thermal conductivities for Purich particles and matrix, respectively. Then by combining the two models, overall thermal conductivity of MOX fuel is obtained. The new proposed model estimates the MOX thermal conductivity about 10% less than the value of U02 fuel, which is in the range of MOX thermal conductivity from HALDEN. The developed thermal conductivity model has been incorporated into KAERIs fuel performance code, COSMOS, and then verified using the measured data in the FIGARO program. Comparison of predicted and measured temperatures shows the reasonable agreement within acceptable error bounds together with satisfactory results for the fission gas release and gap pressure.essure.

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COMPARISON OF DIFFUSION COEFFICIENTS AND ACTIVATION ENERGIES FOR AG DIFFUSION IN SILICON CARBIDE

  • KIM, BONG GOO;YEO, SUNGHWAN;LEE, YOUNG WOO;CHO, MOON SUNG
    • Nuclear Engineering and Technology
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    • v.47 no.5
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    • pp.608-616
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    • 2015
  • The migration of silver (Ag) in silicon carbide (SiC) and $^{110m}Ag$ through SiC of irradiated tristructural isotropic (TRISO) fuel has been studied for the past three to four decades. However, there is no satisfactory explanation for the transport mechanism of Ag in SiC. In this work, the diffusion coefficients of Ag measured and/or estimated in previous studies were reviewed, and then pre-exponential factors and activation energies from the previous experiments were evaluated using Arrhenius equation. The activation energy is $247.4kJ{\cdot}mol^{-1}$ from Ag paste experiments between two SiC layers produced using fluidized-bed chemical vapor deposition (FBCVD), $125.3kJ{\cdot}mol^{-1}$ from integral release experiments (annealing of irradiated TRISO fuel), $121.8kJ{\cdot}mol^{-1}$ from fractional Ag release during irradiation of TRISO fuel in high flux reactor (HFR), and $274.8kJ{\cdot}mol^{-1}$ from Ag ion implantation experiments, respectively. The activation energy from ion implantation experiments is greater than that from Ag paste, fractional release and integral release, and the activation energy from Ag paste experiments is approximately two times greater than that from integral release experiments and fractional Ag release during the irradiation of TRISO fuel in HFR. The pre-exponential factors are also very different depending on the experimental methods and estimation. From a comparison of the pre-exponential factors and activation energies, it can be analogized that the diffusion mechanism of Ag using ion implantation experiment is different from other experiments, such as a Ag paste experiment, integral release experiments, and heating experiments after irradiating TRISO fuel in HFR. However, the results of this work do not support the long held assumption that Ag release from FBCVD-SiC, used for the coating layer in TRISO fuel, is dominated by grain boundary diffusion. In order to understand in detail the transport mechanism of Ag through the coating layer, FBCVD-SiC in TRISO fuel, a microstructural change caused by neutron irradiation during operation has to be fully considered.

Breakup Characteristics of Fuel Droplet Including Nanoparticles (나노 입자가 포함된 연료 액적의 분열 특성 연구)

  • Lee, Jae Bin;Shin, Dong Hwan;Lee, Min Jung;Kim, Namil;Lee, Seong Hyuk
    • Journal of ILASS-Korea
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    • v.17 no.4
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    • pp.192-196
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    • 2012
  • This paper reports on breakup characteristics of fuel droplet which includes metal nanoparticles. In order to develop a new injection system for nanoparticle-coated layers overcoming the conventional flame spray system, fundamental experiments were conducted to examine the interaction between a fuel droplet with nanoparticles and the external energy induced by the laser. In the experiments, this study used nickel nanoparticles whose size was under 100 nm to mix with kerosene as the fuel, and utilized a syringe pump and a metal needle to inject a fuel droplet. In particular, the Nd-YAG laser was adopted to give additional energy to the nanoparticles for evaporation of a fuel droplet containing nanoparticles. When the laser energy as 96 mJ was irradiated during the injection, it was observed that such an explosive evaporation occurred to break up a fuel droplet including nanoparticles, making the rapid increase in the ratio surface area to liquid volume. From this work, we suggest the possibility that the laser energy can be used for rapid evaporation of a fuel droplet.

COSMOS : A Computer Code for the Analysis of LWR $UO_2$ and MOX Fuel Rod

  • Koo, Yang-Hyun;Lee, Byung-Ho;Sohn, Dong-Seong
    • Nuclear Engineering and Technology
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    • v.30 no.6
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    • pp.541-554
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    • 1998
  • A computer code COSMOS has been developed based on the CARO-D5 for the thermal analysis of LWR UO$_2$ and MOX fuel rod under steady-state and transient operating conditions. The main purpose of the COSMOS, which considers high turnup characteristics such as thermal conductivity degradation with turnup and rim formation at the outer part of fuel pellet, is to calculate temperature profile across fuel pellet and fission gas release up to high burnup. A new mechanistic fission gas release model developed based on physical processes has been incorporated into the code. In addition, the features of MOX fuel such as change in themo-mechanical properties and the effect of microscopic heterogeneity on fission gas release have been also taken into account so that it can be applied to MOX fuel. Another important feature of the COSMOS is that it can analyze fuel segment refabricated from base irradiated fuel rods in commercial reactors. This feature makes it possible to analyze database obtained from international projects such as the MALDEN and RISO, many of which were collected from refabricated fuel segments. The capacity of the COSMOS has been tested with some number of experimental results obtained from the HALDEN, RISO and FIGARO programs. Comparison with the measured data indicates that, although the COSMOS gives reasonable agreement, the current models need to be improved. This work is being performed using database available from the OECD/NEA.

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Channel Gap Measurements of Irradiated Plate Fuel and Comparison with Post-Irradiation Plate Thickness

  • James A. Smith;Casey J. Jesse;William A. Hanson;Clark L. Scott;David L. Cottle
    • Nuclear Engineering and Technology
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    • v.55 no.6
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    • pp.2195-2205
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    • 2023
  • One of the salient nuclear fuel performance parameters for new fuel types under development is changes in fuel thickness. To test the new commercially fabricated U-10Mo monolithic plate-type fuel, an irradiation experiment was designed that consisted of multiple mini-plate capsules distributed within the Advanced Test Reactor (ATR) core, the mini-plate 1 (MP-1) experiment. Each capsule contains eight mini-plates that were either fueled or "dummy" plates. Fuel thickness changes within a fuel assembly can be characterized by measuring the gaps between the plates ultrasonically. The channel gap probe (CGP) system is designed to measure the gaps between the plates and will provide information that supports qualification of U-10Mo monolithic fuel. This study will discuss the design and the results from the use of a custom-designed CGP system for characterizing the gaps between mini-plates within the MP-1 capsules. To ensure accurate and repeatable data, acceptance and calibration procedures have been developed. Unfortunately, there is no "gold" standard measurement to compare to CGP measurements. An effort was made to use plate thickness obtained from post-irradiation measurements to derive channel gap estimates for comparison with the CGP characterization.

Proposal of a prototype plant based on the exfoliation process for the treatment of irradiated graphite

  • Pozzetto, Silvia;Capone, Mauro;Cherubini, Nadia;Cozzella, Maria Letizia;Dodaro, Alessandro;Guidi, Giambattista
    • Nuclear Engineering and Technology
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    • v.52 no.4
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    • pp.797-801
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    • 2020
  • Most of irradiated graphite that should be disposed comes from moderators and reflectors of nuclear power plants. The quantity of irradiated graphite could be higher in the future if high-temperature reactors (HTRs) will be deployed. In this case noteworthy quantities of fuel pebbles containing semi-graphitic carbonaceous material should be added to the already existing 250,000 tons of irradiated graphite. Industry graphite is largely used in industrial applications for its high thermal and electrical conductivity and thermal and chemical resistance, making it a valuable material. Irradiated graphite constitutes a waste management challenge owing to the presence of long-lived radionuclides, such as 14C and 36Cl. In the ENEA Nuclear Material Characterization Laboratory it has been successfully designed a procedure based on the exfoliation process organic solvent assisted, with the purpose of investigate the possibility of achieving graphite significantly less toxic that could be recycled for other purpose [1]. The objective of this paper is to evaluate the possibility of the scalability from laboratory to industrial dimensions of the exfoliation process and provide the prototype of a chemical plant for the treatment of irradiated graphite.

EPMA Analysis of Inter-reaction Layer in Irradiated U3Si-Al Fuels (EPMA를 이용한 U3Si/Al 조사 핵연료의 반응층 분석)

  • Jung, Yang-Hong;Yoo, Byung-Ok;Kim, Hee-Moon;Park, Jong-Man;Kim, Myung-Han
    • Analytical Science and Technology
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    • v.17 no.4
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    • pp.355-362
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    • 2004
  • Fission products and Inter reaction layer of $U_3Si-Al$ dispersion fuel, irradiated in HANARO research reactor with 121 kW/m of maximum liner power and 63 at% of average burn-up, was characterization by EPMA (Electron Probe Micro Analyzer). The fuel punching system developed by Irradiated Materials Examination Facility (IMEF) has used to make these samples for the EPMA. With this system a very small and thin specimen which is 1.57 mm in diameter and 2 mm in thickness respectively has been fabricated to protect the EPMA operator from high radioactive fuel and to mini-mize the equivalent dose rate less than 150 mSv/h. EPMA was performed to observe layers of sectional, Inter-reaction and oxide with specimens of cutting and polished. Stoichiometry in the Inter-reaction layer with $16{\mu}m$ of thickness was $U_{2.84}$ Si $Al_{14}$ with calibration of $UO_2$ and $U_{3.24}$ Si $Al_{14.1}$ with calibration of standard specimen. metallic precipitates in this layer were not observed using fission products examination.