• Title/Summary/Keyword: Uranium

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RECYCLING OPTION SEARCH FOR A 600-MWE SODIUM-COOLED TRANSMUTATION FAST REACTOR

  • LEE, YONG KYO;KIM, MYUNG HYUN
    • Nuclear Engineering and Technology
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    • v.47 no.1
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    • pp.47-58
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    • 2015
  • Four recycling scenarios involving pyroprocessing of spent fuel (SF) have been investigated for a 600-MWe transmutation sodium-cooled fast reactor (SFR), KALIMER. Performance evaluation was done with code system REBUS connected with TRANSX and TWODANT. Scenario Number 1 is the pyroprocessing of Canada deuterium uranium (CANDU) SF. Because the recycling of CANDU SF does not have any safety problems, the CANDU-Pyro-SFR system will be possible if the pyroprocessing capacity is large enough. Scenario Number 2 is a feasibility test of feed SF from a pressurized water reactor PWR. Thefsensitivity of cooling time before prior to pyro-processing was studied. As the cooling time sensitivity of cooling time before prior to pyro-processing was studied. As the cooling time increases, excess reactivity at the beginning of the equilibrium cycle (BOEC) decreases, thereby creating advantageous reactivity control and improving the transmutation performance of minor actinides. Scenario Number 3 is a case study for various levels of recovery factors of transuranic isotopes (TRUs). If long-lived fission products can be separated during pyroprocessing, the waste that is not recovered is classified as low- and intermediate-level waste, and it is sufficient to be disposed of in an underground site due to very low-heat-generation rate when the waste cooling time becomes >300 years at a TRU recovery factor of 99.9%. Scenario Number 4 is a case study for the recovery factor of rare earth (RE) isotopes. The RE isotope recovery factor should be lowered to ${\leq}20%$ in order to make sodium void reactivity less than <7$, which is the design limit of a metal fuel.

DIAMETRAL CREEP PREDICTION OF THE PRESSURE TUBES IN CANDU REACTORS USING A BUNDLE POSITION-WISE LINEAR MODEL

  • Lee, Sung-Han;Kim, Dong-Su;Lee, Sim-Won;No, Young-Gyu;Na, Man-Gyun;Lee, Jae-Yong;Kim, Dong-Hoon;Jang, Chang-Heui
    • Nuclear Engineering and Technology
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    • v.43 no.3
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    • pp.301-308
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    • 2011
  • The diametral creep of pressure tubes (PTs) in CANDU (CANada Deuterium Uranium) reactors is one of the principal aging mechanisms governing the heat transfer and hydraulic degradation of the heat transport system (HTS). PT diametral creep leads to diametral expansion, which affects the thermal hydraulic characteristics of the coolant channels and the critical heat flux (CHF). The CHF is a major parameter determining the critical channel power (CCP), which is used in the trip setpoint calculations of regional overpower protection (ROP) systems. Therefore, it is essential to predict PT diametral creep in CANDU reactors. PT diametral creep is caused mainly by fast neutron irradiation, temperature and applied stress. The objective of this study was to develop a bundle position-wise linear model (BPLM) to predict PT diametral creep employing previously measured PT diameters and HTS operating conditions. The linear model was optimized using a genetic algorithm and was devised based on a bundle position because it is expected that each bundle position in a PT channel has inherent characteristics. The proposed BPLM for predicting PT diametral creep was confirmed using the operating data of the Wolsung nuclear power plant in Korea. The linear model was able to predict PT diametral creep accurately.

SCANNING ELECTRON MICROSCOPY ANALYSIS OF FUEL/MATRIX INTERACTION LAYERS IN HIGHLY-IRRADIATED U-Mo DISPERSION FUEL PLATES WITH Al AND Al-Si ALLOY MATRICES

  • Keiser, Dennis D. Jr.;Jue, Jan-Fong;Miller, Brandon D.;Gan, Jian;Robinson, Adam B.;Medvedev, Pavel;Madden, James;Wachs, Dan;Meyer, Mitch
    • Nuclear Engineering and Technology
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    • v.46 no.2
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    • pp.147-158
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    • 2014
  • In order to investigate how the microstructure of fuel/matrix-interaction (FMI) layers change during irradiation, different U-7Mo dispersion fuel plates have been irradiated to high fission density and then characterized using scanning electron microscopy (SEM). Specifially, samples from irradiated U-7Mo dispersion fuel elements with pure Al, Al-2Si and AA4043 (~4.5 wt.%Si) matrices were SEM characterized using polished samples and samples that were prepared with a focused ion beam (FIB). Features not observable for the polished samples could be captured in SEM images taken of the FIB samples. For the Al matrix sample, a relatively large FMI layer develops, with enrichment of Xe at the FMI layer/Al matrix interface and evidence of debonding. Overall, a significant penetration of Si from the FMI layer into the U-7Mo fuel was observed for samples with Si in the Al matrix, which resulted in a change of the size (larger) and shape (round) of the fission gas bubbles. Additionally, solid fission product phases were observed to nucleate and grow within these bubbles. These changes in the localized regions of the microstructure of the U-7Mo may contribute to changes observed in the macroscopic swelling of fuel plates with Al-Si matrices.

A Scheme of Better Utilization of PWR Spent Fuels (가압경수로 사용후핵연료 이용확대 방안연구)

  • Chung, B.J.;Kang, C.S.
    • Nuclear Engineering and Technology
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    • v.23 no.2
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    • pp.165-173
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    • 1991
  • The recycle of PWR spent fuels in a CANDU reactor, so called the tandem fuel cycle is Investigated in this study. This scheme of utilizing Pm spent fuels will ease the shortage of spent fuel storage capacity as well as will improve the use of uranium resources. The minimum modification to the design of present CANDU reactor is seeked in the recycle. Nine different fuel types are considered in this work and are classified into two categories: refabrication and reconfiguration For refabrication, PWR spent fuels are processed and refabricated into the present 37 rod lattice structure of fuel bundle, and for reconfiguration, meanwhile, spent fuels are simply disassembled and rods are cut to fit into the present grid configuration of fuel bundle without refabrication. For each fuel option, the neutronics calculation of lattice was conducted to evaluate the allowable burnup and power distribution. The fuel cycle cost of each option was also computed to assess the economic justification. The result show that most tandem fuel cycle options considered in this study are technically feasible as well as economically viable.

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Design Study of A Spent Fuel Shipping Cask for Korea Nuclear Unit-1 (고리 1호기의 기사용 핵연료 집합체 수송용기 설계에 관한 연구)

  • Moo Han Kim;Chang Sun Kang
    • Nuclear Engineering and Technology
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    • v.14 no.4
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    • pp.196-203
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    • 1982
  • To transport the spent fuel assemblies of Korea Nuclear Unit 1, which is a Westinghouse type two loop pressurized water reactor, it has been found that steel is the most appropriate material for the design of a shipping cask in comparison with lead and depleted uranium. The proposed shipping cask will transport nine fuel assemblies at the same time and is well within the weight limit of transportation by unrestricted rail car. The cask requires 33cm thick steel shield and 27cm thick water region to satisfy the 3 feet apart dose rate limit set forth in 10 CFR 71, and 1.27cm thick steel boron fuel basket to hold the fuel elements inside the cask and control the effective multiplication factor. As a safety analysis, the fuel cladding and centerline temperatures were calculated under the accident condition of complete loss of water coolant, and it was found that the temperature was much lower than the limit of the melting point. k$_{eff}$ was calculated with fresh fuel assemblies, which was found to be well lower than 0.95. For shielding computation, the multipurpose Monte Carlo code MORSE-CG and one dimensional discrete ordinates transport code ANISN were used, and the Monte Carlo codes KENO and MORSE-CG were used for criticality calculation. The radiation source terms were calculated using ORIGEN-79.9.

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Characterization of Fe (III)-Reducing Bacteria Isolated from the Sediment of Chunho Reservoir (천호지 저질토에서 분리한 철환원세균의 특성)

  • 안태영;박재홍;이일규;전은형
    • Korean Journal of Microbiology
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    • v.38 no.2
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    • pp.133-138
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    • 2002
  • Microbial Fe (III) reduction is important for the biogeochemical cycle in the sediment of freshwater system. Also, the Fe (III) reducing mechanism make a model of oxidizing organic compounds and reducing toxic heavy metals, such as chrome or uranium. Thirty-seven strains which have Fe (III) reducing activity were isolated from sediments in lake Soyang and Chunho reservoir. The initial concentration of Fe (II) was the highest in sediments of lake Soyang. However, the highest Fe (III) reducing activity was shown in Chunho reservoir. All isolates were tested for Fe (III) reducing activity. Strains C2 and C3, which were isolated from sediments of Chunho reservoir, showed the highest activity. These strains were tested to see if they utilize various electron donors such as glucose, yeast extract, acetate, ethanol and toluene. Significantly, glucose and yeast extract were used as electron donors. Also these strains were conformed to use humid acid and nitrate as electron accepters. The 16S rRNA sequences of strains C2 and C3 were closely related to Aeromonas hydrophila with 95% similarity.

Deposition of Uranium Ions with Modified Pyrrole Polymer Film Electrode (우라늄이온 포집을 위한 수식된 피를 고분자 피막전극)

  • Cha Seong-Keuck;Lee Sang Bong
    • Journal of the Korean Electrochemical Society
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    • v.3 no.3
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    • pp.141-145
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    • 2000
  • Anodically Polymerized conducting Polypyrrole film electrode was employed to Pick up uranyl ion with the type of Gr/ppy, xylenol orange modified electrode. To have Porous and oriented ppy film, NBR was applied as precoating agent. The rate constant of polymerization was $3.22\times10^{-3}s^{-1}$ which was 1.6 times smaller value than bare graphite surface. The deposited amount of uranyl iou on $1.70Ccm^{-2}$ of ppy was $1.55\times10^{-4}g$. The matrix effect in artificial seawater was $6.8\%$. The polymer film electrode has a diffusion controlled process in conduction, but the modified Gr/ppy, $X.O^{4-}UO^+$ type was influenced on the ion doping and electronic conduction of film itself owing to increasing of impedance. The capacitance of electrical double layer was respectively enhanced to 56 and 130 times in Gr/ppy, $X.O.^{4-}$ and Gr/ppy, $X.O^{4-}UO^+$ than Grippy type electrode.

Sensitivity Analysis of Core Neutronic Parameters in Electron Accelerator-driven Subcritical Advanced Liquid Metal Reactor

  • Ebrahimkhani, Marziye;Hassanzadeh, Mostafa;Feghhi, Sayed Amier Hossian;Masti, Darush
    • Nuclear Engineering and Technology
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    • v.48 no.1
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    • pp.55-63
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    • 2016
  • Calculation of the core neutronic parameters is one of the key components in all nuclear reactors. In this research, the energy spectrum and spatial distribution of the neutron flux in a uranium target have been calculated. In addition, sensitivity of the core neutronic parameters in accelerator-driven subcritical advanced liquid metal reactors, such as electron beam energy ($E_e$) and source multiplication coefficient ($k_s$), has been investigated. A Monte Carlo code (MCNPX_2.6) has been used to calculate neutronic parameters such as effective multiplication coefficient ($k_{eff}$), net neutron multiplication (M), neutron yield ($Y_{n/e}$), energy constant gain ($G_0$), energy gain (G), importance of neutron source (${\varphi}^*$), axial and radial distributions of neutron flux, and power peaking factor ($P_{max}/P_{ave}$) in two axial and radial directions of the reactor core for four fuel loading patterns. According to the results, safety margin and accelerator current ($I_e$) have been decreased in the highest case of $k_s$, but G and ${\varphi}^*$ have increased by 88.9% and 21.6%, respectively. In addition, for LP1 loading pattern, with increasing $E_e$ from 100 MeV up to 1 GeV, $Y_{n/e}$ and G improved by 91.09% and 10.21%, and $I_e$ and $P_{acc}$ decreased by 91.05% and 10.57%, respectively. The results indicate that placement of the Np-Pu assemblies on the periphery allows for a consistent $k_{eff}$ because the Np-Pu assemblies experience less burn-up.

DEVELOPMENT OF AN IMPROVED FARE TOOL WITH APPLICATION TO WOLSONG NUCLEAR POWER PLANT

  • Lee, Sun Ki;Hong, Sung Yull
    • Nuclear Engineering and Technology
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    • v.45 no.2
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    • pp.257-264
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    • 2013
  • In Canada Deuterium Uranium (CANDU)-type nuclear power plants, the reactor is composed of 380 fuel channels and refueling is performed on one or two channels per day. At the time of refueling, the fluid force of the cooling water inside the channel is exploited. New fuel added upstream of the fuel channel is moved downstream by the fluid force of the cooling water, and the used fuel is pushed out. Through this process, refueling is completed. Among the 380 fuel channels, outer rows 1 and 2 (called the FARE channel) make the process of using only the internal fluid force impossible because of the low flow rate of the channel cooling water. Therefore, a Flow Assist Ram Extension (FARE) tool, a refueling aid, is used to refuel these channels in order to compensate for the insufficient fluid force. The FARE tool causes flow resistance, thus allowing the fuel to be moved down with the flow of cooling water. Although the existing FARE tool can perform refueling in Korean plants, the coolant flow rate is reduced to below 80% of the normal flow for some time during refueling. A Flow rate below 80% of the normal flow cause low flow rate alarm signal in the plant operation. A flow rate below 80% of the normal flow may cause difficulties in the plant operation because of the increase in the coolant temperature of the channel. A new and improved FARE tool is needed to address the limitations of the existing FARE tool. In this study, we identified the cause of the low flow phenomena of the existing FARE tool. A new and improved FARE tool has been designed and manufactured. The improved FARE tool has been tested many times using laboratory test apparatus and was redesigned until satisfactory results were obtained. In order to confirm the performance of the improved FARE tool in a real plant, the final design FARE tool was tested at Wolsong Nuclear Power Plant Unit 2. The test was carried out successfully and the low flow rate alarm signal was eliminated during refueling. Several additional improved FARE tools have been manufactured. These improved FARE tools are currently being used for Korean CANDU plant refueling.

POST-IRRADIATION ANALYSES OF U-MO DISPERSION FUEL RODS OF KOMO TESTS AT HANARO

  • Ryu, H.J.;Park, J.M.;Jeong, Y.J.;Lee, K.H.;Lee, Y.S.;Kim, C.K.;Kim, Y.S.
    • Nuclear Engineering and Technology
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    • v.45 no.7
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    • pp.847-858
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    • 2013
  • Since 2001, a series of five irradiation test campaigns for atomized U-Mo dispersion fuel rods, KOMO-1, -2, -3, -4, and -5, has been conducted at HANARO (Korea) in order to develop high performance low enriched uranium dispersion fuel for research reactors. The KOMO irradiation tests provided valuable information on the irradiation behavior of U-Mo fuel that results from the distinct fuel design and irradiation conditions of the rod fuel for HANARO. Full size U-Mo dispersion fuel rods of 4-5 $g-U/cm^3$ were irradiated at a maximum linear power of approximately 105 kW/m up to 85% of the initial U-235 depletion burnup without breakaway swelling or fuel cladding failure. Electron probe microanalyses of the irradiated samples showed localized distribution of the silicon that was added in the matrix during fuel fabrication and confirmed its beneficial effect on interaction layer growth during irradiation. The modifications of U-Mo fuel particles by the addition of a ternary alloying element (Ti or Zr), additional protective coatings (silicide or nitride), and the use of larger fuel particles resulted in significantly reduced interaction layers between fuel particles and Al.