• Journal of Radiation Protection and Research
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• v.28 no.2
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• pp.109-116
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• 2003

Based on the necessity to evaluate the activation products inventory during decommissioning lot domestic nuclear power plants, a preliminary estimation of the activation products inventory for Kori unit 1, which is getting close to the end of lifetime, was carried out with ANISN and ORIGEN2 code. In order to calculate neutron nux using ANISN code, the reactor was divided into 9 zones from core to bioshield concrete for radial direction. Also :he cross-section of main nuclides were calibrated with neutron flux in the reactor pressure vessel(RPV) region. The results showed that 95 % of tile total radioactivity in RPV from reactor shutdown to 10 years came from the nuclides of $^{55}Fe,\;^{59}Ni,\;^{63}Ni\;and\;^{60}Co$. And the total radioactivity with cooling of more than 50 years after decommissioning was no more than 0.2 % of at the time of shutdown. Considering the weight of RPV is 210 tons, the total radioactivity of RPV reached to $5.25{\times}10^{6}GBq$ at shutdown time. As compared with the total radioactivity of bioshield concrete at reactor shutdown time, the radioactivity after tooling more than 10 years was below 1 %.

• Analytical Science and Technology
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• v.16 no.2
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• pp.110-116
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• 2003

A study has been done on the separation of iodide from spent pressurized water reactor (PWR) fuels and its quantitative determination using ion chromatography. Spent PWR fuels were dissolved with mixed acid of nitric and hydrochloric acids (80 : 20 molL%) which can oxidize iodide to iodate to prevent it from be vaporized. After reducing ${IO_3}^-$ ­to $I_2$ in 2.5 M $HNO_3$ with $NH_2OH{\cdot}HCl$, Iodine was selectively separated from actinides and all other fission products with carbontetrachloride and back-extracted with 0.1 M $NaHSO_3$. Recovered iodide was determined using the ion chromatograph of which the column was installed in a glove box for the analysis of radioactive materials. In practice, spent PWR fuel with 42,000~44,000 MWd/MtU was analyzed and its quantity was compared to that calculated by burnup code, ORIGEN2. The agreement was achieved with a deviation of -8.3~-0.5% from the ORIGEN 2 data, $324.5{\sim}343.6{\mu}g/g$.

• Journal of Radiation Protection and Research
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• v.18 no.2
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• pp.27-35
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• 1993

A shielding analysis of the shipping cask for transporting the CANDU spent fuel bundles has been studied. Radiation source term has been calculated on spent fuel with burn-up of 7,800 MWD/MTU and 5 years cooling time by ORIGEN2 code. The shielding calculation for the cask capable of transporting 378 bundles of CANDU spent fuel has been made by use of 1-D ANISN and 2-D DOT 4.2 codes. As a result of analysis, the optimum shield thickness of cask was obtained. And it is proved that the safety in radiation shielding under normal transport and hypothetical accident conditions is confirmed to satisfy the allowable values specified in IAEA Safety Series No. 6 and the Korean Atomic Law.

• Journal of Radiation Protection and Research
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• v.31 no.2
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• pp.105-113
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• 2006

The oxidizing species are generated from the radiolysis of groundwater in the pore of buffer material around the canister used for the disposal of spent fuels. A mathematical model was introduced to calculate the cathodic current density induced by the oxidant around the canister, which determined the corrosion of carbon steel. An analytical solution was derived to get the cathodic current density in the cylindrical coordinate. The cathodic current densities from both the rectangular coordinate and cylindrical coordinate were compared with each other. The source terms and absorbed dose rate for the calculation of the radiolysis were calculated using the ORIGEN2 and MCNP computer code, respectively. The radius of the canister was determined with the new model in order to prevent the local corrosion. The results showed that the new solution made the cathodic current density around 25 % lower than the Marsh model.

• Journal of Radiation Protection and Research
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• v.13 no.2
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• pp.78-87
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• 1988

This article suggests the radionuclides which should be considered more important to the offsite consequence assesment during a nuclear power plant accident. For this purpose, the relative importance to the early health effects of released radionuclides on the major organs during the accident is estimated under the assumption of the same release fraction. The inventories of the 25 elements, 54 nuclides selected in the Reactor Safety Study are calculated by ORIGEN 2 code. The organs of interest in the estimation are G. I. track, bone marrow, thyroid and lung. The result shows the relative potential importance of radionuclides as follows: For G.I. track, Np, Ce, Ru, Y, and Zr are of importance in sequence, Np, I, La, Sr, Ba for bone marrow, I and Te for thyroid, Cm, Ce, Ru, Pu, Zr for lung. In addition to iodine and noble gases, therefore, the potential contribution of those nuclides listed above to the offsite consequences should not be overlooked for some accidents of particular sequence.

• Nuclear Engineering and Technology
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• v.43 no.6
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• pp.583-592
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• 2011

The radiological characteristics for waste classification were assessed for neutron-activated decommissioning wastes from a CANDU reactor. The MCNP/ORIGEN2 code system was used for the source term analysis. The neutron flux and activation cross-section library for each structural component generated by MCNP simulation were used in the radionuclide buildup calculation in ORIGEN2. The specific activities of the relevant radionuclides in the activated metal waste were compared with the specified limits of the specific activities listed in the Korean standard and 10 CFR 61. The time-average full-core model of Wolsong Unit 1 was used as the neutron source for activation of in-core and ex-core structural components. The approximated levels of the neutron flux and cross-section, irradiated fuel composition, and a geometry simplification revealing good reliability in a previous study were used in the source term calculation as well. The results revealed the radioactivity, decay heat, hazard index, mass, and solid volume for the activated decommissioning waste to be $1.04{\times}10^{16}$ Bq, $2.09{\times}10^3$ W, $5.31{\times}10^{14}\;m^3$-water, $4.69{\times}10^5$ kg, and $7.38{\times}10^1\;m^3$, respectively. According to both Korean and US standards, the activated waste of the pressure tubes, calandria tubes, reactivity devices, and reactivity device supporters was greater than Class C, which should be disposed of in a deep geological disposal repository, whereas the side structural components were classified as low- and intermediate-level waste, which can be disposed of in a land disposal repository. Finally, this study confirmed that, regardless of the cooling time of the waste, 15% of the decommissioning waste cannot be disposed of in a land disposal repository. It is expected that the source terms and waste classification evaluated through this study can be widely used to establish a decommissioning/disposal strategy and fuel cycle analysis for CANDU reactors.

• Nuclear Engineering and Technology
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• v.43 no.2
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• pp.149-158
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• 2011

Metal waste generated from the pyroprocessing of 10 MtU of spent fuel was classified by comparing the specific activity of a relevant radionuclide with the limit value of the specific activity specified in the Korean acceptance criteria for a lowand intermediate-level waste repository. A Korean Optimized Fuel Assembly design with a 17${\times}$17 array, an initial enrichment of 4.5 weight-percent, discharge burn-up of 55 GWD/MtU, and a 10-year cooling time was considered. Initially, the mass and volume of each structural component of the assembly were calculated in detail, and a source term analysis was subsequently performed using ORIGEN-S for these components. An activation cross-section library generated by the KENO-VI/ORIGEN-S module was utilized for top-end and bottom-end pieces. As a result, an Inconel grid plate, a SUS plenum spring, a SUS guide tube subpart, SUS top-end and bottom-end pieces, and an Inconel top-end leaf spring were determined to be unacceptable for the Gyeongju low- and intermediate-level waste repository, as these waste products exceeded the acceptance criteria. In contrast, a Zircaloy grid plate and guide tube can be placed in the Gyeongju repository. Non-contaminated Zircaloy cladding occupying 76% of the metal waste was found to have a lower level of specific activity than the limit value. However, Zircaloy cladding contaminated by fission products and actinides during the decladding process of pyroprocessing was revealed to have 52 and 2 times higher specific activity levels than the limit values for alpha and $^{90}Sr$, respectively. Finally, it was found that 88.7% of the metal waste from the 17${\times}$17 Korean Optimized Fuel Assembly design should be disposed of in a deep geological repository. Therefore, it can be summarized that separation technology with a higher decontamination factor for transuranics and strontium should be developed for the efficient management of metal waste resulting from pyroprocessing.

• Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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• v.17 no.1
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• pp.121-126
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• 2019

The radionuclide inventory prediction of a nuclear power plant can help establish decommissioning plan by providing information of radiation environment. Accumulated radionuclides in reactors and related facilities after reactor shutdown can be divided into neutron activated materials and contaminated materials. Among the neutron activated radionuclides, $^{36}Cl$ and $^{41}Ca$ are important from the viewpoint of disposal because of its long half-life and physiochemical characteristics. In this research, we calculated the radionuclides of $^{36}Cl$ and $^{41}Ca$ in bioshielding concrete by estimating the neutron flux and cross section using the MCNPX. And we evaluated the inventories of $^{36}Cl$ and $^{41}Ca$ using the activation calculation code ORIGEN2.

• Journal of Radiation Protection and Research
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• v.37 no.4
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• pp.202-207
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• 2012

The radioactivity inventory significantly affects all steps of decommissioning projects including planning, cost estimation, risk assessment, waste management and site remediation. The decommissioning project of the KRR-2 was completed in 2009 and a large amount of activated concrete waste was generated. The bioshield concrete, containing minute amount of impurity elements, was activated by neutron reaction during the operation of the reactor. A variety radionuclides was generated in the concrete, including $^3H$, $^{14}C$, $^{55}Fe$, $^{60}Co$ $^{63}Ni$, $^{134}Cs$, $^{152}Eu$ and $^{154}Eu$. In this paper, the comparison between the calculated results and previous measured results was carried out to estimate the inventory of the bioshield concrete of the KRR-2. The combined computer codes of MCNP5 and ORIGEN 2.1 for calculation of the distribution of neutron flux, cross-section and generation of radionuclides were used. The results were shown that 99.8% of the total radioactivity of $^3H$, $^{55}Fe$, $^{60}Co$ and $^{152}Eu$ in the bioshield concrete 12 years after shutdown. The effects on the variation of inventory were analysed depending on the operation periods and the cooling times in the bioshield concrete.

• Proceedings of the Materials Research Society of Korea Conference
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• 2003.11a
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• pp.228-228
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• 2003

차세대관리 종합공정에서 취급되는 기준 방사선원은 경수로에서 배출된 우라늄-235 농축도 3.5 wt%, 연소도는 43 Gwd/tU 이며 냉각기간은 10년인 사용후핵연료이다. 사용후핵연료의 기준 사양과 차세대관리 종합공정의 특성에 따라 최대 1,385 TBq의 방사선원이 핫셀내에 존재하게 되며, 핫셀 차폐벽은 총 방사능량에 대한 차폐능을 가져야 한다. 최대 방사선원에 대한 핫셀 차폐벽의 중성자에 대한 차폐능을 평가하기 위하여, 본 연구에서는 ORIGEN-2 코드를 이용하여 사용후핵연료에서 발생하는 핵종 및 핵종량을 평가하였으며, 이 자료를 기초로 하여 중성자 선원항을 SOURCES코드를 이용하여 계산하였다.