• Title/Summary/Keyword: Nuclear Transmutation

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Effect of Target Material and the Neutron Spectrum on Nuclear Transmutation of 99Tc and 129I in Nuclear Reactors (표적물질 및 중성자 스펙트럼이 99Tc과 129I의 원자로 내부 핵변환에 미치는 영향)

  • Kang, Seung-gu;Lee, Hyun-chul
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.16 no.2
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    • pp.195-202
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    • 2018
  • As a rule, geological disposal is considered a safe method for final disposal of high-level radioactive waste. However, some long-lived fission products like $^{99}Tc$ and $^{129}I$ contained in spent nuclear fuel are highly mobile as less sorbing anionic species in the subsurface environment and can mainly cause exposure dose to the ecosystem by emission of beta rays in the hundreds of keV range. Therefore, if these two nuclides can be separated and converted with high efficiency into radioactively unharmful nuclides, this would have a positive effect on disposal safety. One candidate method is to transmute these two nuclides in nuclear reactors into short-lived nuclides or into stable nuclides. For this purpose, it is necessary to evaluate which reactor type is more efficient in burning these two nuclides. In this study, the simulation results of nuclear transmutation of $^{99}Tc$ and $^{129}I$ in light water reactor (PWR), heavy water reactor (CANDU) and fast neutron reactor (SFR, MET-1000) are compared and discussed.

CFD ANALYSIS OF HEAVY LIQUID METAL FLOW IN THE CORE OF THE HELIOS LOOP

  • Batta, A.;Cho, Jae-Hyun;Class, A.G.;Hwang, Il-Soon
    • Nuclear Engineering and Technology
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    • v.42 no.6
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    • pp.656-661
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    • 2010
  • Lead-alloys are very attractive nuclear coolants due to their thermo-hydraulic, chemical, and neutronic properties. By utilizing the HELIOS (Heavy Eutectic liquid metal Loop for Integral test of Operability and Safety of PEACER$^2$) facility, a thermal hydraulic benchmarking study has been conducted for the prediction of pressure loss in lead-alloy cooled advanced nuclear energy systems (LACANES). The loop has several complex components that cannot be readily characterized with available pressure loss correlations. Among these components is the core, composed of a vessel, a barrel, heaters separated by complex spacers, and the plenum. Due to the complex shape of the core, its pressure loss is comparable to that of the rest of the loop. Detailed CFD simulations employing different CFD codes are used to determine the pressure loss, and it is found that the spacers contribute to nearly 90 percent of the total pressure loss. In the system codes, spacers are usually accounted for; however, due to the lack of correlations for the exact spacer geometry, the accuracy of models relies strongly on assumptions used for modeling spacers. CFD can be used to determine an appropriate correlation. However, application of CFD also requires careful choice of turbulence models and numerical meshes, which are selected based on extensive experience with liquid metal flow simulations for the KALLA lab. In this paper consistent results of CFX and Star-CD are obtained and compared to measured data. Measured data of the pressure loss of the core are obtained with a differential pressure transducer located between the core inlet and outlet at a flow rate of 13.57kg/s.

RADIAL UNIFORMITY OF NEUTRON IRRADIATION IN SILICON INGOTS FOR NEUTRON TRANSMUTATION DOPING AT HANARO

  • KIM MYONG-SEOP;LEE CHOONG-SUNG;OH SOO-YOUL;HWANG SUNG-YUL;JUN BYUNG-JIN
    • Nuclear Engineering and Technology
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    • v.38 no.1
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    • pp.93-98
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    • 2006
  • The radial uniformity of neutron irradiation in silicon ingots for neutron transmutation doping (NTD) at HANARO is examined by both calculations and measurements. HANARO has two NTD holes named NTD1 and NTD2. We have been using the NTD2 hole for 5 in. NTD commercial service, and we intend to use two holes for 6 in. NTD. The objective of this study is to predict the radial uniformity of 6 in. NTD at the two holes. The radial neutron flux distributions inside single crystal and noncrystal silicon loaded at the NTD2 hole are calculated by the VENTURE code. For NTD1, the radial distributions of the reaction rate for a 6 in. NTD with a neutron screen are calculated by MCNP, and measured by gold wire activation. The results of the measurements are compared with those of the calculations. From the VENTURE calculation, it is confirmed that the neutron flux distribution in the single crystal silicon is much flatter than that in the non-crystal silicon. The non-uniformities of the measurements for radial neutron irradiation are slightly larger than those of the calculations. However, excluding local dips in the measurements, the overall trends of the distributions are similar. The radial resistivity gradient (RRG) for a 5 in. silicon ingot is estimated to be about $1.5\%$. For a 6 in. ingot, the RRG of a silicon ingot irradiated at HANARO is predicted to be about $2.1\%$. Also, from the experimental results, we expect that the RRG would not be larger than $4.4\%$.

NEW EVALUATION METHODS FOR RADIAL UNIFORMITY IN NEUTRON TRANSMUTATION DOPING

  • Kim, Hak-Sung;Lim, Jae-Yong;Pyeon, Cheol-Ho;Misawa, Tsuyoshi;Shiroya, Seiji;Park, Sang-Jun;Kim, Myong-Seop;Oh, Soo-Youl;Jun, Byung-Jin
    • Nuclear Engineering and Technology
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    • v.42 no.4
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    • pp.442-449
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    • 2010
  • Recently, the neutron irradiation for large diameter silicon (Si)-ingots of more than 8" diameter is requested to satisfy the demand for the neutron transmutation doping silicon (NTD-Si). By increasing the Si-ingot diameter, the radial non-uniformity becomes larger due to the neutron attenuation effect, which results in a limit of the feasible diameter of the Si-ingot. The current evaluation method has a certain limit to precisely evaluate the radial uniformity of Si-ingot because the current evaluation method does not consider the effect of the Si-ingot diameter on the radial uniformity. The objective of this study is to propose a new evaluation method of radial uniformity by improving the conventional evaluation approach. To precisely predict the radial uniformity of a Si-ingot with large diameter, numerical verification is conducted through comparison with the measured data and introducing the new evaluation method. A new concept of a gradient is introduced as an alternative approach of radial uniformity evaluation instead of the radial resistivity gradient (RRG) interpretation. Using the new concept of gradient, the normalized reaction rate gradient (NRG) and the surface normalized reaction rate gradient (SNRG) are described. By introducing NRG, the radial uniformity can be evaluated with one certain standard regardless of the ingot diameter and irradiation condition. Furthermore, by introducing SNRG, the uniformity on the Si-ingot surface, which is ignored by RRG and NRG, can be evaluated successfully. Finally, the radial uniformity flattening methods are installed by the stainless steel thermal neutron filter and additional Si-pipe to reduce SNRG.

Integral nuclear data validation using experimental spent nuclear fuel compositions

  • Gauld, Ian C.;Williams, Mark L.;Michel-Sendis, Franco;Martinez, Jesus S.
    • Nuclear Engineering and Technology
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    • v.49 no.6
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    • pp.1226-1233
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    • 2017
  • Measurements of the isotopic contents of spent nuclear fuel provide experimental data that are a prerequisite for validating computer codes and nuclear data for many spent fuel applications. Under the auspices of the Organisation for Economic Co-operation and Development (OECD) Nuclear Energy Agency (NEA) and guidance of the Expert Group on Assay Data of Spent Nuclear Fuel of the NEA Working Party on Nuclear Criticality Safety, a new database of expanded spent fuel isotopic compositions has been compiled. The database, Spent Fuel Compositions (SFCOMPO) 2.0, includes measured data for more than 750 fuel samples acquired from 44 different reactors and representing eight different reactor technologies. Measurements for more than 90 isotopes are included. This new database provides data essential for establishing the reliability of code systems for inventory predictions, but it also has broader potential application to nuclear data evaluation. The database, together with adjoint based sensitivity and uncertainty tools for transmutation systems developed to quantify the importance of nuclear data on nuclide concentrations, are described.

미임계 핵변환로 최적 냉각재 선정

  • 한석중;김도형;유동한;신운철;박원석
    • Proceedings of the Korean Nuclear Society Conference
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    • 1998.05a
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    • pp.690-695
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    • 1998
  • 원자력시설에서 배출되는 고준위 방사선 페기물이나 TRU 둥의 심지층처분의 보완책으로서 핵변환 (Transmutation) 처리방안이 연구되고 있다 이 핵변환시스템의 냉각재로서 액체금속류가 고려되고 있다. 본 연구에서는 핵변환로에 적합한 냉각물질을 도출하기 위해서 보다 합리적인 선정방법으로서 의사결정방법을 이용하여 중점비교 대상인 나트륨(Na), 나트륨-칼륨 합금(Na-K alloy), 납(Pb), 납-비스므스 합금(Pb-Bi alloy)에 대한 정량적 평가를 시도하였다. 아울러 이 냉각재 후보물질에 대한 냉각재로서의 적합성 여부를 비교 검토하였다. 본 방법을 이용한 결과 핵 변화로의 냉각재로서는 납-비스므스 합금이 가장 적합한 것으로 평가되었다.

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Numerical studies on the important fission products for estimating the source term during a severe accident

  • Lee, Yoonhee;Cho, Yong Jin;Lim, Kukhee
    • Nuclear Engineering and Technology
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    • v.54 no.7
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    • pp.2690-2701
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    • 2022
  • In this paper, we select important fission products for the estimation of the source term during a severe accident of a PWR. The selection is based on the numerical results obtained from depletion calculations for the typical PWR fuel via the in-house code named DEGETION (Depletion, Generation, and Transmutation of Isotopes on Nuclear Application), release fractions of the fission products derived from NUREG-1465, and effective dose conversion coefficients from ICRP 119. Then, for the selected fission products, we obtain the adjoint solutions of the Bateman equations for radioactive decay in order to determine the importance of precursors producing the aforementioned fission products via radioactive decay, which would provide insights into the assumption used in MACCS 2 for a level 3 PSA analysis in which up to six precursors are considered in the calculations of radioactive decays for the fission product after release from the reactor.

CONTRIBUTION OF HANARO IRRADIATION TECHNOLOGIES TO NATIONAL NUCLEAR R&D

  • Choo, Kee Nam;Cho, Man Soon;Yang, Sung Woo;Park, Sang Jun
    • Nuclear Engineering and Technology
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    • v.46 no.4
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    • pp.501-512
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    • 2014
  • HANARO is a multipurpose research reactor located at the Korea Atomic Energy Research Institute (KAERI). Since the commencement of its operation in 1995, various neutron irradiation facilities, such as rabbit irradiation facilities, fuel test loop (FTL) facilities, capsule irradiation facilities, and neutron transmutation doping (NTD) facilities, have been developed and actively utilized for various nuclear material irradiation tests requested by users from research institutes, universities, and industries. Most irradiation tests have been related to national R&D relevant to present nuclear power reactors such as the ageing management and safety evaluation of the components. Based on the accumulated experience as well as the sophisticated requirements of users, HANARO has recently supported national R&D projects relevant to new nuclear systems including the System-integrated Modular Advanced Reactor (SMART), research reactors, and future nuclear systems. This paper documents the current state and utilization of irradiation facilities in HANARO, and summarizes ongoing research efforts to deploy advanced irradiation technology.

Conceptual Design Based on Scale Laws and Algorithms Sub-critical Transmutation Reactors

  • Lee, Kwang-Gu;Chang, Soon-Heung
    • Proceedings of the Korean Nuclear Society Conference
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    • 1997.10a
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    • pp.475-480
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    • 1997
  • In order to conduct the effective integration of computer-aided conceptual design for integrated nuclear power reactor, not only is a smooth information flow required, but also decision making fur both conceptual design and construction process design must be synthesized. In addition to the aboves, the relations between the one step and another step and the methodologies to optimize the decision variables are verified, in this paper especially, that is, scaling laws and scaling criteria. In the respect with the running of the system, the integrated optimization process is proposed in which decisions concerning both conceptual design are simultaneously made. According to the proposed reactor types and power levels, an integrated optimization problems are formulated. This optimization is expressed as a multi-objective optimization problem. The algorithm for solving the problem is also presented. The proposed method is applied to designing a integrated sub-critical reactors.

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