• Title/Summary/Keyword: Neutron spectroscopy

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Measurement of undesirable neutron spectrum in a 120 MeV linac

  • Yihong Yan ;Xinjian Tan;Xiufeng Weng ;Xiaodong Zhang ;Zhikai Zhang ;Weiqiang Sun ;Guang Hu ;Huasi Hu
    • Nuclear Engineering and Technology
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    • v.55 no.10
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    • pp.3591-3598
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    • 2023
  • Photoneutron background spectroscopy observations at linac are essential for directing accelerator shielding and subtracting background signals. Therefore, we constructed a Bonner Sphere Spectrometer (BSS) system based on an array of BF3 gas proportional counter tubes. Initially, the response of the BSS system was simulated using the MCNP5 code. Next, the response of the system was calibrated by using neutrons with energies of 2.86 MeV and 14.84 MeV. Then, the system was employed to measure the spectrum of the 241Am-Be neutron source, and the results were unfolded by using the Gravel and EM algorithms. Using the validated system, the undesirable neutron spectrum of the 120 MeV electron linac was finally measured and acquired. In addition, it is demonstrated that the equivalent undesirable neutron dose at a distance of 3.2 m from the linac is 19.7 mSv/h. The results measured by the above methods could provide guidance for linac-related research.

Surface Characterization of the d-PMMA Thin Films Treated by Oxygen Plasma (산소 플라즈마 처리된 d-PMMA 박막의 표면특성 분석)

  • Kim, Soong-Hoon;Choi, Dong-Jin;Lee, Jeong-Su;Choi, Ho-Suk
    • Polymer(Korea)
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    • v.33 no.3
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    • pp.263-267
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    • 2009
  • In order to improve the hydrophilic property on the surface of d-PMMA(deuterated poly-(methyl methacrylate)) film, it was exposed to oxygen plasma, All experimental conditions were same except to plasma exposure time that was varied from 0 to 180 s, The effects according to the exposure time were identified using contact angles, X-ray reflectometer(XRR), neutron reflectometer(NR), and X-ray photoelectron spectroscopy(XPS). By confirming that as the exposure time increases, water contact angle decreases while the composition of oxygen increases, it was confirmed that the composition of oxygen has a huge influence on improving the hydrophilic property. The physical characters as a function of the exposure time were investigated by the XRR. By analyzing complementally the results of the XRR, NR, and XPS, more detailed chemical bonding conditions were studied by obtaining not only composition of the carbon and oxygen but that of the hydrogen.

An Improved Proton Recoil Telescope Detector for Fast Neutron Spectroscopy

  • Chung, Moon-Kyu;Kang, Hee-Dong;Park, Tong-Soo
    • Nuclear Engineering and Technology
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    • v.5 no.3
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    • pp.191-201
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    • 1973
  • For fast neutron spectroscopy in MeV region, a recoil proton telescope detector was designed and constructed so as to increase in detection efficiency without appreciable deterioration in energy resolution by adopting a special type of recoil proton radiator which is a combination of a ring-shaped vertical radiator and a cone-shaped horizontal radiator at a certain geometry. A neutron stopper was built in the detector system to minimize the background due to direct exposure of the Si(Li) detectors to primary incident neutrons. The detection efficiency and the energy resolution calculated at various neutron energies and geometries are given and these characteristics of the detector system were tested by 14.1 MeV neutrons. As the calculation predicted, the relative detection efficiency in case of the combined radiator system is almost 2.2 times of that for a single, ring-shaped vertical radiator system. The calculated energy resolution is 3.7% FWHM, whereas the measured resolution was 3.9% which means resolution broadening of approximately. 30% was resulted by introducing a combined radiator system into the telescope. Increase in background less than 40% was also observed.

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Green synthesis of Lead-Nickel-Copper nanocomposite for radiation shielding

  • B.M. Chandrika;Holaly Chandrashekara Shastry Manjunatha;R. Munirathnam;K.N. Sridhar;L. Seenappa;S. Manjunatha;A.J. Clement Lourduraj
    • Nuclear Engineering and Technology
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    • v.55 no.12
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    • pp.4671-4677
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    • 2023
  • For the first time Pb, Ni, and Cu nanocomposites were synthesized by versatile solution combustion synthesis using Aloevera extract as a reducing agent, to study the potential applications in X-ray/gamma, neutron, and Bremsstrahlung shielding. The synthesized Lead-Nickel-Copper (LNC) nanocomposites were characterized by PXRD, SEM, UV-VIS, and FTIR for the confirmation of successful synthesis. PXRD analysis confirmed the formation of multiphase LNC NCs and the Scherrer equation and the W-H plot gave the average crystal sizes of 19 nm and 17 nm. Surface morphology using SEM and EDX confirmed the presence of LNC NCs. Strong absorption peaks were analyzed by UV visible spectroscopy and the direct energy gap is found to be 3.083 eV. Functional groups present in the LNC NCs were analyzed by FTIR spectroscopy. X-ray/gamma radiation shielding properties were measured using NaI(Tl) detector coupled with MCA. It is found to be very close to Pb. Neutron shielding parameters were compared with traditional shielding materials and found LNC NCs are better than lead and concrete. Secondary radiation shielding known as Bremsstrahlung shielding characteristics also studied and found that LNC NCs are best in secondary radiation shielding. Hence LNC NCs find shielding applications in ionizing radiation such as X-ray/gamma and neutron radiation.

Measurements of Neutron Activation and Dose Rate Induced by High-Energy Medical Linear Accelerator

  • Kwon, Na Hye;Jang, Young Jae;Kim, Jinsung;Kim, Kum Bae;Yoo, Jaeryong;Ahn, So Hyun;Kim, Dong Wook;Choi, Sang Hyoun
    • Progress in Medical Physics
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    • v.32 no.4
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    • pp.145-152
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    • 2021
  • Purpose: During the treatments of cancer patients with a linear accelerator (LINAC) using photon beams with energies ≥8 MV, the components inside the LINAC head get activated through the interaction of photonuclear reaction (γ, n) and neutron capture (n, γ). We used spectroscopy and measured the dose rate for the LINAC in operation after the treatment ended. Methods: We performed spectroscopy and dose rate measurements for three units of LINACs with a portable high-purity Germanium (HPGe) detector and a survey meter. The spectra were obtained after the beams were turned off. Spectroscopy was conducted for 3,600 seconds, and the dose rate was measured three times. We identified the radionuclides for each LINAC. Results: According to gamma spectroscopy results, most of the nuclides were short-lived radionuclides with half-lives of 100 days, except for 60Co, 65Zn, and 181W nuclides. The dose rate for three LINACs obtained immediately in front of the crosshair was in the range of 0.113 to 0.129 µSv/h. The maximum and minimum dose rates measured on weekends were 0.097 µSv/h and 0.092 µSv/h, respectively. Compared with the differences in weekday data, there was no significant difference between the data measured on Saturday and Sunday. Conclusions: Most of the detected radionuclides had half-lives <100 days, and the dose rate decreased rapidly. For equipment that primarily used energies ≤10 MV, when the equipment was transferred after at least 10 minutes after shutting it down, it is expected that there will be little effect on the workers' exposure.

A study of neutron activation analysis compared to inductively coupled plasma atomic emission spectrometry for geological samples in Iran

  • Mohammadzadeh, Mohammad;Ajami, Mona;shadeghipanah, Arash;Rezvanifard, Mehdi
    • Nuclear Engineering and Technology
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    • v.50 no.8
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    • pp.1349-1354
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    • 2018
  • Inductively Coupled Plasma Atomic Emission Spectroscopy (ICP-AES) is widely used for the determination of trace elements in geological samples in Iran. In this paper, we have calculated the detection limits of neutron activation analysis (NAA) for some of the common elements in such samples utilizing the ORIGEN and MCNP codes and verified the simulations using the experimental results of three soil standard reference materials, namely, G02.SRM, G18.SRM, and G28.SRM. The results show that while the detection limit of ICP-AES method is usually in the mg/kg range, it is represented to the ${\mu}g/kg$ range for most of the elements of interest using the NAA method, and the simulations can be verified in a tolerance range of 20%.

Brief Introduction to Angle-Resolved Photoemission Spectroscopy

  • Kim, Hyeong-Do
    • Proceedings of the Korean Vacuum Society Conference
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    • 2012.02a
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    • pp.82-82
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    • 2012
  • Angle-resolved photoemission spectroscopy (ARPES) is a powerful tool to investigate the electronic structure of a single-crystalline solid. After the development of a two-dimensional electron detector, it became a basic experimental method in solid state physics comparable to other powerful tools such as x-ray and neutron scatterings. In this tutorial, I talk briefly on the basic principle of ARPES and its recent and future direction of development.

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Measuring and unfolding fast neutron spectra using solution-grown trans-stilbene scintillation detector

  • Nguyen Duy Quang;HongJoo Kim;Phan Quoc Vuong;Nguyen Duc Ton;Uk-Won Nam;Won-Kee Park;JongDae Sohn;Young-Jun Choi;SungHwan Kim;SukWon Youn;Sung-Joon Ye
    • Nuclear Engineering and Technology
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    • v.55 no.3
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    • pp.1021-1030
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    • 2023
  • We propose an overall procedure for measuring and unfolding fast neutron spectra using a trans-stilbene scintillation detector. Detector characterization was described, including the information on energy calibration, detector resolution, and nonproportionality response. The digital charge comparison method was used for the investigation of neutron-gamma Pulse Shape Discrimination (PSD). A pair of values of 600 ns pulse width and 24 ns delay time was found as the optimized conditions for PSD. A fitting technique was introduced to increase the trans-stilbene Proton Response Function (PRF) by 28% based on comparison of the simulated and experimental electron-equivalent distributions by the Cf-252 source. The detector response matrix was constructed by Monte-Carlo simulation and the spectrum unfolding was implemented using the iterative Bayesian method. The unfolding of simulated and measured spectra of Cf-252 and AmBe neutron sources indicates reliable, stable and no-bias results. The unfolding technique was also validated by the measured cosmic-ray induced neutron flux. Our approach is promising for fast neutron detection and spectroscopy.

Ability of non-destructive assay techniques to identify sophisticated material partial defects

  • Lloyd, Cody;Goddard, Braden
    • Nuclear Engineering and Technology
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    • v.52 no.6
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    • pp.1252-1258
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    • 2020
  • This study explores the ability of non-destructive assay techniques to detect a partial material defect in which 100 g of plutonium are diverted from the center of a 1000 g can of PuO2 powder. Four safeguards measurements techniques: neutron multiplicity counting, calorimetry, gravimetry, and gamma ray spectroscopy are used in an attempt to detect the defect. Several materials are added to the partial defect PuO2 can to replicate signatures of the diverted material. 252Cf is used to compensate for the doubles neutron counts, 241Am is used to compensate for the decay heat, and aluminum is used to compensate for the weight. Although, the doubles and triples difference before and after diversion are statistically indistinguishable with the AWCC in fast and thermal mode, the difference in the singles counts are statistically detectable in both modes. The relatively short half-life of 252Cf leads to a decrease (three sigma uncertainty) in the doubles neutron counts after 161 days. Combining this with the precise quantity of 241Am needed (10.7 g) to mimic the heat signature and the extreme precision in 252Cf mass needed to defeat neutron multiplicity measurements gives reassurance in the International Atomic Energy Agency's ability to detect partial material defects.

A study on point defects induced with neutron irradiation in silicon wafer (중성자 조사에 의해 생성된 점결함 연구)

  • 김진현;류근걸
    • Proceedings of the Korean Institute of Electrical and Electronic Material Engineers Conference
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    • 2002.07a
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    • pp.62-66
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    • 2002
  • The conventional floating zone(FZ) crystal and Czochralski(CZ) silicon crystal have resistivity variations longitudinally as well as radially The resistivity variations of the conventional FZ and CZ crystal are not conformed to requirement of dopant distribution for power devices and thyristors. These resistivity variations in conventional cystals limits the reverse breakdown voltage that could be achieved and forced designers of high power diodes and thyristors to compromise the desired current-voltage characteristics. So to produce high Power diodes and thyristors, Neutron Transmutation Doping(NTD) technique is the one method just because NTD silicon provides very homogeneous distribution of doping concentration. This procedure involves the nuclear transmutation of silicon to phosphorus by bombardment of neutron to the crystal according to the reaction $^{30}$ Si(n,${\gamma}$)longrightarrow$^{31}$ Silongrightarrow(2.6 hr)$^{31}$ P+$\beta$$^{[-10]}$ . The radioactive isotope $^{31}$ Si is formed by $^{31}$ Si capturing a neutron, which then decays into the stable $^{31}$ P isotope (i.e., the donor atom), whose distribution is not dependent on the crystal growth parameters. In this research, neutron was irradiated on FZ silicon wafers which had high resistivity(1000~2000 Ω cm), for 26 and 8.3hours for samples of HTS-1 and HTS-2, and 13, 3.2, 2.0 hours for samples of IP-1, IP-2 and IP-3, respectively, to compare resistivity changes due to time differences. The designed resistivities were approached, which were 2.l Ωcm for HTS-1, 7.21 Ω cm for HTS-2, 1.792cm for IP-1, 6.83 Ωcm for IP-2, 9.23 Ωcm for IP-3, respectively. Point defects were investigated with Deep Level Transient Spectroscopy(DLTS). Four different defects were observed at 80K, 125K, 230K, and above 300K.

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