• Journal of Radiation Protection and Research
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• 제48권4호
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• pp.184-196
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• 2023

Background: Radiation protection is crucial in various fields due to the harmful effects of radiation. Shielding is used to reduce radiation exposure, but gamma radiation poses challenges due to its high energy and penetration capabilities. Materials and Methods: This work investigates the radiation shielding properties of polyvinylidene fluoride (PVDF) samples containing different weight fraction of tungsten carbide (WC), tungsten trioxide (WO₃), and tungsten disulfide (WS₂). Parameters such as the mass attenuation coefficient (MAC), half-value layer (HVL), mean free path (MFP), effective atomic number (Z_eff), and macroscopic effective removal cross-section for fast neutrons (Σ_R) were calculated using the Phy-X/PSD software. EpiXS simulations were conducted for MAC validation. Results and Discussion: Increasing the weight fraction of the additives resulted in higher MAC values, indicating improved radiation shielding. PVDF-xWC showed the highest percentage increase in MAC values. MFP results indicated that PVDF-0.20WC has the lowest values, suggesting superior shielding properties compared to PVDF-0.20WO₃ and PVDF-0.20WS₂. PVDF-0.20WC also exhibited the highest Z_eff values, while PVDF-0.20WS₂ showed a slightly higher increase in Z_eff at energies of 0.662 and 1.333 MeV. PVDF-0.20WC has demonstrated the highest Σ_R value, indicating effective shielding against fast neutrons, while PVDF-0.20WS₂ had the lowest Σ_R value. The Monte Carlo N-Particle Transport version 5 (MCNP5) simulations showed that PVDF-xWC attenuates gamma radiation more than pure PVDF, significantly decreasing the dose equivalent rate. Conclusion: Overall, this research provides insights into the radiation shielding properties of PVDF mixtures, with PVDF-xWC showing the most promising results.