• Title/Summary/Keyword: Neutron and gamma flux

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Modelling atomic relaxation and bremsstrahlung in the deterministic code STREAM

  • Nhan Nguyen Trong Mai;Kyeongwon Kim;Deokjung Lee
    • Nuclear Engineering and Technology
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    • v.56 no.2
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    • pp.673-684
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    • 2024
  • STREAM, developed by the Computational Reactor Physics and Experiment laboratory (CORE) of the Ulsan National Institute of Science and Technology (UNIST), is a deterministic neutron- and photon-transport code primarily designed for light water reactor (LWR) analysis. Initially, the photon module in STREAM did not account for fluorescence and bremsstrahlung photons. This article presents recent developments regarding the integration of atomic relaxation and bremsstrahlung models into the existing photon module, thus allowing for the transport of secondary photons. The photon flux and photon heating computed with the newly incorporated models is compared to results obtained with the Monte Carlo code MCS. The incorporation of secondary photons has substantially improved the accuracy of photon flux calculations, particularly in scenarios involving strong gamma emitters. However, it is essential to note that despite the consideration of secondary photon sources, there is no noticeable improvement in the photon heating for LWR problems when compared to the photon heating obtained with the previous version of STREAM.

Some Improvements of Gamma-ray Measurement for the Determination of the Boron Content (붕소 함량결정을 위한 즉발 감마선 계측법의 개선)

  • Nak Bae Kim;Hae-Ill Bak
    • Nuclear Engineering and Technology
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    • v.16 no.1
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    • pp.18-20
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    • 1984
  • The detection limit of boron has been lowered further in the capture gamma-ray measurement after preconcentration of boron by placing natural lithium brick in front of Ge(Li) detector. The experimental detection limit is found to be 0.30ppm, 0.18ppm, 0.045ppm and 0.090ppm for the samples of aluminum, steel, uranium dioxide and graphite, respectively. An alternate counting technique kas been also used for neglecting the error caused by the fluctuation of neutron flux during counting.

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An Improved Method for the Determination of Scandium by Neutron Activation Analysis (스칸듐定量을 위한 改良된 放射化分析法)

  • Chung, Koo-Soon;Lee, Chul
    • Journal of the Korean Chemical Society
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    • v.8 no.2
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    • pp.88-91
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    • 1964
  • A rapid and simple method is described here for the determination of scandium in monazite by neutron activation analysis. The sample is irradiated for 20 hours at the neutron flux of $10^{12}$ thermal neutrons/$cm^2$/sec in the TRIGA MARK Ⅱ reactor, after which the sample is decomposed by fusion with concentrated sulfuric acid. The scandium-46 together with scandium carrier are separated from the irradiated sample by precipitating with ammonia, and are extracted by solvent extraction of the thiocyanate complex into ether. The induced radioactivity is measured by gamma scintillation spectrometry using the Multichannel Pulse Height Analyzer connected with 2"${\times}$2" NaI(Tl). The chemical yield is determined gravimetrically by precipitating scandium with mandelic acid. In order to check the efficiency of scandium separation and the errors from interfering activities of the other elements, scandium was separated by the cation exchange resin column, and the results from both samples were compared each other, which showed that the chemical procedure used in this work was as selective as the ion-exchange method with respect to scandium separation. The scandium contents in Korean monazite were found to be about 12 p. p. m.

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Validation of the neutron lead transport for fusion applications

  • Schulc, Martin;Kostal, Michal;Novak, Evzen;Czakoj, Tomas;Simon, Jan
    • Nuclear Engineering and Technology
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    • v.54 no.3
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    • pp.959-964
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    • 2022
  • Lead is an important material, both for fusion or fission reactors. The cross sections of natural lead should be validated because lead is a main component of lithium-lead modules suggested for fusion power plants and it directly affects the crucial variable, tritium breeding ratio. The presented study discusses a validation of the lead transport libraries by dint of the activation of carefully selected activation samples. The high emission standard 252Cf neutron source was used as a neutron source for the presented validation experiment. In the irradiation setup, the samples were placed behind 5 and 10 cm of the lead material. Samples were measured using a gamma spectrometry to infer the reaction rate and compared with MCNP6 calculations using ENDF/B-VIII.0 lead cross sections. The experiment used validated IRDFF-II dosimetric reactions to validate lead cross sections, namely 197Au(n, 2n)196Au, 58Ni(n,p)58Co, 93Nb(n, 2n)92mNb, 115In(n,n')115mIn, 115In(n,γ)116mIn, 197Au(n,γ)198Au and 63Cu(n,γ)64Cu reactions. The threshold reactions agree reasonably with calculations; however, the experimental data suggests a higher thermal neutron flux behind lead bricks. The paper also suggests 252Cf isotropic source as a valuable tool for validation of some cross-sections important for fusion applications, i.e. reactions on structural materials, e.g. Cu, Pb, etc.

Analysis of several VERA benchmark problems with the photon transport capability of STREAM

  • Mai, Nhan Nguyen Trong;Kim, Kyeongwon;Lemaire, Matthieu;Nguyen, Tung Dong Cao;Lee, Woonghee;Lee, Deokjung
    • Nuclear Engineering and Technology
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    • v.54 no.7
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    • pp.2670-2689
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    • 2022
  • STREAM - a lattice transport calculation code with method of characteristics for the purpose of light water reactor analysis - has been developed by the Computational Reactor Physics and Experiment laboratory (CORE) of the Ulsan National Institute of Science and Technology (UNIST). Recently, efforts have been taken to develop a photon module in STREAM to assess photon heating and the influence of gamma photon transport on power distributions, as only neutron transport was considered in previous STREAM versions. A multi-group photon library is produced for STREAM based on the ENDF/B-VII.1 library with the use of the library-processing code NJOY. The developed photon solver for the computation of 2D and 3D distributions of photon flux and energy deposition is based on the method of characteristics like the neutron solver. The photon library and photon module produced and implemented for STREAM are verified on VERA pin and assembly problems by comparison with the Monte Carlo code MCS - also developed at UNIST. A short analysis of the impact of photon transport during depletion and thermal hydraulics feedback is presented for a 2D core also from the VERA benchmark.

A Study on the Radioactive Products of Components in Proton Accelerator on Short Term Usage Using Computed Simulation (몬테칼로 시뮬레이션을 활용한 양성자가속기 단기사용 시 구성품의 방사화 평가)

  • Bae, Sang-Il;Kim, Jung-Hoon
    • Journal of radiological science and technology
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    • v.43 no.5
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    • pp.389-395
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    • 2020
  • The evaluation of radioactivated components of heavy-ion accelerator facilities affects the safety of radiation management and the exposure dose for workers. and this is an important issue when predicting the disposal cost of waste during maintenance and dismantling of accelerator facilities. In this study, the FLUKA code was used to simulate the proton treatment device nozzle and classify the radio-nuclides and total radioactivity generated by each component over a short period of time. The source term was evaluated using NIST reference beam data, and the neutron flux generated for each component was calculated using the evaluated beam data. Radioactive isotopes caused by generated neutrons were compared and evaluated using nuclide information from the International Radiation Protection Association and the Korea Radioisotope association. Most of the nuclides produced form of beta rays and electron capture, and short-lived nuclides dominated. However, In the case of 54Mn, which is a radioactive product of iron, the effect of gamma rays should be considered. In the case of tritium generated from a material with a low atomic number, it is considered that handling care should be taken due to its long half-life.

Dosimetric Characteristics of a Thermal Neutron Beam Facility for Neutron Capture Therapy at HANARO Reactor (하나로 원자로 BNCT 열중성자 조사장치에 대한 선량특성연구)

  • Lee, Dong-Han;Suh, So-Heigh;Ji, Young-Hoon;Choi, Moon-Sik;Park, Jae-Hong;Kim, Kum-Bae;Yoo, Seung-Yul;Kim, Myong-Seop;Lee, Byung-Chul;Chun, Ki-Jung;Cho, Jae-Won;Kim, Mi-Sook
    • Progress in Medical Physics
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    • v.18 no.2
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    • pp.87-92
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    • 2007
  • A thermal neutron beam facility utilizing a typical tangential beam port for Neutron Capture Therapy was installed at the HANARO, 30 MW multi-purpose research reactor. Mixed beams with different physical characteristics and relative biological effectiveness would be emitted from the BNCT irradiation facility, so a quantitative analysis of each component of the mixed beams should be performed to determine the accurate delivered dose. Thus, various techniques were applied including the use of activation foils, TLDs and ionization chambers. All the dose measurements were perform ed with the water phantom filled with distilled water. The results of the measurement were compared with MCNP4B calculation. The thermal neutron fluxes were $1.02E9n/cm^2{\cdot}s\;and\;6.07E8n/cm^2{\cdot}s$ at 10 and 20 mm depth respectively, and the fast neutron dose rate was insignificant as 0.11 Gy/hr at 10 mm depth in water The gamma-ray dose rate was 5.10 Gy/hr at 20 mm depth in water Good agreement within 5%, has been obtained between the measured dose and the calculated dose using MCNP for neutron and gamma component and discrepancy with 14% for fast neutron flux Considering the difficulty of neutron detection, the current study support the reliability of these results and confirmed the suitability of the thermal neutron beam as a dosimetric data for BNCT clinical trials.

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Multi-Channel Mechanical Test Machine for HANARO (I)

  • Song, M.S.;Choi, Y.;Cho, M.S.;Kim, B.G.;Kang, Y.H.
    • Proceedings of the Korean Nuclear Society Conference
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    • 2004.10a
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    • pp.979-980
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    • 2004
  • A multi-channel mechanical test machine for HANARO was designed and fabricated based on the design criteria of the multi-channel mechanical test machine sustained at the working conditions of $<400{\square}$, 3 W/g of gamma heating rate, $5{\times}10^{20}\;n/cm^2$, neutron flux and maximum load of 200 MPa. The multi-channel mechanical test machine made of 304 stainless steel consisted of four modules. Two of them locate upper part of the machine and the others locate lower part with 90 degree rotation. Each module was evaluated by determine load-displacement curve of zirconium specimen. Thermal insulators were also made by electron spark-machining of pure aluminum which was prepared in a domestic company.

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A Simultaneous Determination of Chromium, Iron, Lanthanum, Scandium and Zinc in River Water by Neutron Activation (중성자 방사화에 의한 시료중의 크롬, 철, 란탄, 스칸듐 및 아연의 동시정량)

  • Lee Ihn Chong;Kim Si-Joong;Lee Chul
    • Journal of the Korean Chemical Society
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    • v.21 no.6
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    • pp.427-433
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    • 1977
  • A neutron activation method has been developed for the simultaneous determination of chromium, iron, lanthanum, scandium and zinc in river-water samples. The sample is sealed in the silica ampoule without pretreatment and irradiated for a week at a thermal neutron flux of $1{\times}10^{13}n{\cdot}cm^{-2}{\cdot}sec^{-1}$. After cooling for about two days, the elements in the sample are sequentially extracted at different pH by 0.1M oxine-chloroform solution. The organic layers are checked by Gamma-ray spectrometry with $″3\;{\times}\;3″$ NaI (T1) detector connected to a 800-channel pulse hight analyzer. The ppb concentration of the elements in most of river-water samples could be determined by this method. The tracer study for the quantitative separation of the elements was also carried out.

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Study on Dose Rate on the Surface of Cask Packed with Activated Cut-off Pieces from Decommissioned Nuclear Power Plant

  • Park, Kwang Soo;Kim, Hae Woong;Sohn, Hee Dong;Kim, Nam Kyun;Lee, Chung Kyu;Lee, Yun;Lee, Ji Hoon;Hwang, Young Hwan;Lee, Mi Hyun;Lee, Dong Kyu;Jung, Duk Woon
    • Journal of Radiation Protection and Research
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    • v.45 no.4
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    • pp.178-186
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    • 2020
  • Background: Reactor pressure vessel (RV) with internals (RVI) are activated structures by neutron irradiation and volume contaminated wastes. Thus, to develop safe and optimized disposal plan for them at a disposal site, it is important to perform exact activation calculation and evaluate the dose rate on the surface of casks which contain cut-off pieces. Materials and Methods: RV and RVI are subjected to neutron activation calculation via Monte Carlo methodology with MCNP6 and ORIGEN-S program-neutron flux, isotopic specific activity, and gamma spectrum calculation on each component of RV and RVI, and dose rate evaluation with MCNP6. Results and Discussion: Through neutron activation analysis, dose rate is evaluated for the casks containing cut-off pieces produced from decommissioned RV and RVI. For RV cut-off ones, the highest value of dose rate on the surface of cask is 6.97 × 10-1 mSv/hr and 2 m from it is 3.03 × 10-2 mSv/hr. For RVI cut-off ones, on the surface of it is 0.166 × 10-1 mSv/hr and 2 m from it is 1.04 × 10-1 mSv/hr. Dose rates for various RV and RVI cut-off pieces distributed lower than the limit except the one of 2 m from the cask surface of RVI. It needs to adjust contents in cask which carries highly radioactive components in order to decrease thickness of cask. Conclusion: Two types of casks are considered in this paper: box type for very-low-level waste (VLLW) as well as low-level waste (LLW) and cylinder type for intermediate-level waste (ILW). The results will contribute to the development of optimal loading plans for RV and RVI cut-off pieces during the decommissioning of nuclear power plant that can be used to prepare radioactive waste disposal plans for the different types of wastes-ILW, LLW, and VLLW.