• Title/Summary/Keyword: Gamma-ray spectrometry

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A novel barium oxide-based Iraqi sand glass to attenuate the low gamma-ray energies: Fabrication, mechanical, and radiation protection capacity evaluation

  • Al-Saeedi, F.H.F.;Sayyed, M.I.;Kapustin, F.L.;Al-Ghamdi, Hanan;Kolobkova, E.V.;Tashlykov, O.L.;Almuqrin, Aljawhara H.;Mahmoud, K.A.
    • Nuclear Engineering and Technology
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    • v.54 no.8
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    • pp.3051-3058
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    • 2022
  • In the present work, untreated Iraqi sand with grain sizes varied between 100 and 200 ㎛ was used to produce a colored glass sample that has shielding features against the low gamma-ray energy. Therefore, a weight of 70-60 wt % sand was mixed with 9-14 wt% B2O3, 8-10 wt% Na2O, 4-6 wt% of CaO, 3-6 wt% Al2O3, in addition to 0.3% of Co2O3. After melting and annealing the glass sample, the X-ray diffraction spectrometry was applied to affirm the amorphous phase of the fabricated glass samples. Moreover, the X-ray dispersive energy spectrometry was used to measure the chemical composition, and the MH-300A densimeter was applied to measure the fabricated sample's density. The Makishima-Makinzie model was applied to predict the mechanical properties of the fabricated glass. Besides, the Monte Carlo simulation was used to estimate the fabricated glass sample's radiation shielding capacity in the low-energy region between 22.1 and 160.6 keV. Therefore, the simulated linear attenuation coefficient changed between 10.725 and 0.484 cm-1, raising the gamma-ray energy between 22.1 and 160.6 keV. Also, other shielding parameters such as a half-value layer, pure lead equivalent thickness, and buildup factors were calculated.

NEW DEVELOPMENT OF HYPERGAM AND ITS TEST OF PERFORMANCE FOR γ-RAY SPECTRUM ANALYSIS

  • Park, B.G.;Choi, H.D.;Park, C.S.
    • Nuclear Engineering and Technology
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    • v.44 no.7
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    • pp.781-790
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    • 2012
  • The HyperGam program was developed for the analysis of complex HPGe ${\gamma}$-ray spectra. The previous version of HyperGam was mainly limited to the analysis of ${\gamma}$-ray peaks and the manual logging of the result. In this study, it is specifically developed into a tool for the isotopic analysis of spectra. The newly developed features include nuclide identification and activity determination. An algorithm for nuclide identification was developed to identify the peaks in the spectrum by considering the yield, efficiency, energy and peak area for the ${\gamma}$-ray lines emitted from the radionuclide. The detailed performance of nuclide identification and activity determination was accessed using the IAEA 2002 set of test spectra. By analyzing the test spectra, the numbers of radionuclides identified truly (true hit), falsely (false hit) or missed (misses) were counted and compared with the results from the IAEA 2002 tests. The determined activities of the radionuclides were also compared for four test spectra of several samples. The result of the performance test is promising in comparison with those of the well-known software packages for ${\gamma}$-ray spectrum analysis.

Database of virtual spectrum of artificial radionuclides for education and training in in-situ gamma spectrometry

  • Yoomi Choi;Young-Yong Ji;Sungyeop Joung
    • Nuclear Engineering and Technology
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    • v.55 no.1
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    • pp.190-200
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    • 2023
  • As the field of application of in-situ gamma spectroscopy is diversified, proficiency is required for consistent and accurate analysis. In this study, a program was developed to virtually create gamma energy spectra of artificial nuclides, which are difficult to obtain through actual measurements, for training. The virtual spectrum was created by synthesizing the spectra of the background radiation obtained through actual measurement and the theoretical spectra of the artificial radionuclides obtained by a Monte Carlo simulation. Since the theoretical spectrum can only be obtained for a given geometrical structure, representative major geometries for in-situ measurement (ground surface, concrete wall, radioactive waste drum) and the detectors (HPGe, NaI(Tl), LaBr3(Ce)) were predetermined. Generated virtual spectra were verified in terms of validity and harmonization by gamma spectrometry and energy calibration. As a result, it was confirmed that the energy calibration results including the peaks of the measured spectrum and the peaks of the theoretical spectrum showed differences of less than 1 keV from the actual energies, and that the calculated radioactivity showed a difference within 20% from the actual inputted radioactivity. The verified data were assembled into a database and a program that can generate a virtual spectrum of desired condition was developed.

Preparation of Carrier-free Fe-59 by Korean TRIGA Mark Ⅱ Reactor (無擔體 鐵-59製造에 關한 硏究)

  • Park, Keung-Shik
    • Journal of the Korean Chemical Society
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    • v.9 no.2
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    • pp.96-100
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    • 1965
  • Possibility on carrier-free Fe-59 preparation by Korean TRIGA Mark Ⅱ reactor was investigated, namely average cross section on $Co^{59}$(n,p) $Fe^{59}$ reaction, separation by anion exchange resin and radiochemical purity. Radiochemical purity of Fe-59 separated was checked by the method of ${\gamma}$-ray spectrometry with 256-multichannel pulse height analyzer and of half life determination. This method permits Fe-59 preparation with radiochemical purity of > 99.9%.

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Full spectrum estimation of helicopter background and cosmic gamma-ray contribution for airborne measurements

  • Lukas Kotik;Marcel Ohera
    • Nuclear Engineering and Technology
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    • v.55 no.3
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    • pp.1052-1060
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    • 2023
  • The airborne radiation monitoring has been used in geophysics for more than forty years and now it also has its important role in emergency monitoring. The aircraft background and the cosmic gamma-rays contribute to the measured gamma spectrum on the aircraft board. This adverse effect should be eliminated before the data processing. The paper describes two semiparametric methods to estimate the full spectrum aircraft background and cosmic gamma-ray contribution from spectra measured at altitudes where terrestrial contribution is negligible. The methods only assume to know possible peak positions in spectra and their full width at half maximum, that can be easily obtained e.g. from terrestrial measurement. The methods were applied to real experimental data acquired on Mi-17 and Bell 412 helicopter boards. The IRIS airborne gamma-ray spectrometer, with 4×4 L NaI(Tl) crystals, produced by Pico Envirotec Inc., Canada, was used on helicopters' boards. To obtain valid estimate of the aircraft background and the cosmic contribution, the measurements over sea and large water areas were carried out. However, the satisfactory results over inland were also achieved comparing with those acquired over large water areas.

A New Aluminium Container for $\gamma$-Ray Spectrometry Analysis of Radium and Radon (라듐 및 라돈의 감마선 분광 분석을 위한 알루미늄 용기의 제작 및 특성 조사)

  • Lee, Kil Yong;Yoon, Yoon Yeol;Seo, Bum Kyoung
    • Analytical Science and Technology
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    • v.13 no.6
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    • pp.743-750
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    • 2000
  • For the ${\gamma}$-ray spectrometry analysis of radium and radon in environmental samples, plastic Marinelli beakers have been usually used. But, there are two problems; one is the increment of background by adsorption of airborne radon daughters on the plastic beaker, and other is the incompleteness of radioactive equilibrium by the loss of gaseous radon produced during the radioactive equilibrium process. In order to solve these problems, we made aluminium counting container, and investigated its characteristics. We investigated radioactive equilibrium process using the aluminium container. We found that both solid and liquid samples reached at radioactive equilibrium state in the aluminium container without loss of gaseous radon. By the use of the aluminium container, we established radon and radium analysis method of solid and liquid samples using gamma-ray spectrometry.

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A comparative study of different radiometric methodologies for the determination of 226Ra in water

  • Al-Hamarneh, Ibrahim F.;Almasoud, Fahad I.
    • Nuclear Engineering and Technology
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    • v.50 no.1
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    • pp.159-164
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    • 2018
  • An evaluation of various radiometric methods to analyze $^{226}Ra$ in water has been employed on a set of 10 standard solutions of different concentrations in the range of $1-10Bq/L^{-1}$. The analysis was carried out using well-established procedures by means of gamma-ray, alpha-particle and liquid scintillation spectrometry. The feasibility of the various methods has been quantified in terms of relative standard error and percentage error. Correlations between the various methods have been presented and discussed. In general, good agreement was found in the results of various methodologies, which assures the accuracy of the methods and allows for the validation of instrumentation and procedures. Of the different methods adopted here, a combined procedure for the determination of $^{226}Ra$ along with $^{228}Ra$ using Quantulus 1220 ultra-low level background liquid scintillation counting gave the most accurate results.