• Title/Summary/Keyword: Fission Measurement

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A 235U mass measurement method for UO2 rod assembly based on the n/γ joint measurement system

  • Yang, Jianqing;Zhang, Quanhu;Su, Xianghua;Li, Sufen;Zhuang, Lin;Hou, Suxia;Huo, Yonggang;Zhou, Hao;Liu, Guorong
    • Nuclear Engineering and Technology
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    • v.52 no.5
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    • pp.1036-1042
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    • 2020
  • Fast-Neutron Multiplicity Counter based on Liquid Scintillator Detector can directly measure the fast neutron multiplicity emitted by UO2 rod. HPGe gamma spectrometer; which has superior energy resolution; is routinely used for the gamma energy spectrum measurement. Combing Fast-Neutron Multiplicity Counter and HPGe γ-spectrometer, the n/γ joint measurement system is developed. The fast neutron multiplicity and gamma energy spectrum of UO2 rod assemblies under different conditions are measured by the n/γ joint measurement system. The induced fission rate and the 235U abundance, thereby the 235U mass; can be obtained for UO2 rod assemblies. The 235U mass deviation of the measured value from the reference value is less than 5%. The results show that the n/γ joint measurement system is effective and applicable in the measurement of the 235U mass in samples.

Calibration of digital wide-range neutron power measurement channel for open-pool type research reactor

  • Joo, Sungmoon;Lee, Jong Bok;Seo, Sang Mun
    • Nuclear Engineering and Technology
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    • v.50 no.1
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    • pp.203-210
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    • 2018
  • As the modernization of the nuclear instrumentation system progresses, research reactors have adopted digital wide-range neutron power measurement (DWRNPM) systems. These systems typically monitor the neutron flux across a range of over 10 decades. Because neutron detectors only measure the local neutron flux at their position, the local neutron flux must be converted to total reactor power through calibration, which involves mapping the local neutron flux level to a reference reactor power. Conventionally, the neutron power range is divided into smaller subranges because the neutron detector signal characteristics and the reference reactor power estimation methods are different for each subrange. Therefore, many factors should be considered when preparing the calibration procedure for DWRNPM channels. The main purpose of this work is to serve as a reference for performing the calibration of DWRNPM systems in research reactors. This work provides a comprehensive overview of the calibration of DWRNPM channels by describing the configuration of the DWRNPM system and by summarizing the theories of operation and the reference power estimation methods with their associated calibration procedure. The calibration procedure was actually performed during the commissioning of an open-pool type research reactor, and the results and experience are documented herein.

Measurement and Analyses of Radiation -Assessment of Defected Fuel by Analysis of Reactor Coolant Activities- (방사선 측정 및 해석 연구 -원자로 냉각수중의 방사능해석에 의한 결함핵연료봉의 평가-)

  • Yang, Jae-Choon;Oh, Hi-Peel;Jun, Jae-Shik;Lee, Ho-Yon;Oh, Heon-Jin;Chung, Moon-Kyu;Park, Hae-Yong
    • Journal of Radiation Protection and Research
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    • v.11 no.2
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    • pp.139-145
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    • 1986
  • An improved mothod of assessing fuel status by analyzsis of the fission product in the reactor coolant system is proposed. The release mechanism of specific fission products is established for determination of the coefficients in the equations which relate the radioactivities with the amount of defected fuel. Knock-out and migration models are employed in the formulation of the release mechanism. The influence of the tramp uranium is quantified. Sample calculations were made for KNU 1 reactor system using the I-131 and I-133 concentrations in the primary coolant. The estimated number of defected fuel pins in the third and sixth cycles appeared to be $9.34{\pm}1.13\;and\;0.294{\pm}0.092$, respectively.

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Separation and Purification for the Determination of Zirconium and Its Isotopes in PWR Spent Nuclear Fuels (PWR 사용후핵연료 중 Zr 및 Zr 동위원소 정량을 위한 분리 및 정제)

  • Kim, Jung Suk;Jeon, Young Shin;Park, Yong Joon;Lee, Chang Heon;Kim, Won Ho
    • Analytical Science and Technology
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    • v.11 no.6
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    • pp.421-428
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    • 1998
  • A method has been studied to separate Zr from various fission products in PWR spent nuclear fuels. A solution containing metal ions in place of radioactive fission products was prepared. The Zr was separated with 5 M HCl followed by eluting metal ions such as Ce, Nd, Cs, Rb, Ba, Sr, Ru, Rh, Pd, Ag and Cd with 12 M HCl on Dowex $1{\times}8$, anion exchange resin. The recovery of Zr was more than 95%. The purification of Zr was carried out on anion exchange resin, Dowex $1{\times}8$, in 5 M HCl in order to remove Mo causing isobaric effect during mass spectrometry. The method was applied to separate Zr from a spent PWR fuel. From mass spectrometric measurement, the purified Zr portion was not showed the isobars from other elements such as Mo and Sr.

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CERAMOGRAPHY ANALYSIS OF MOX FUEL RODS AFTER AN IRRADIATION TEST

  • Kim, Han-Soo;Jong, Chang-Yong;Lee, Byung-Ho;Oh, Jae-Yong;Koo, Yang-Hyun
    • Nuclear Engineering and Technology
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    • v.42 no.5
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    • pp.576-581
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    • 2010
  • KAERI (Korea Atomic Energy Research Institute) fabricated MOX (Mixed Oxide) fuel pellets as a cooperation project with PSI (Paul Scherrer Institut) for an irradiation test in the Halden reactor. The MOX pellets were fitted into fuel rods that included instrumentation for measurement in IFE (Institutt for Energiteknikk). The fuel rods were assembled into the test rig and irradiated in the Halden reactor up to 50 MWd/kgHM. The irradiated fuel rods were transported to the IFE, where ceramography was carried out. The fuel rods were cut transversely at the relatively higher burn-up locations and then the radial cross sections were observed. Micrographs were analyzed using an image analysis program and grain sizes along the radial direction were measured by the linear intercept method. Radial cracks in the irradiated MOX were observed that were generally circumferentially closed at the pellet periphery and open in the hot central region. A circumferential crack was formed along the boundary between the dark central and the outer regions. The inner surface of the cladding was covered with an oxide layer. Pu-rich spots were observed in the outer region of the fuel pellets. The spots were surrounded by many small pores and contained some big pores inside. Metallic fission product precipitates were observed mainly in the central region and in the inside of the Pu spots. The average areal fractions of the metallic precipitates at the radial cross section were 0.41% for rod 6 and 0.32% for rod 3. In the periphery, pore density smaller than 2 ${\mu}m$ was higher than that of the other regions. The grain growth occurred from 10 ${\mu}m$ to 12 ${\mu}m$ in the central region of rod 6 during irradiation.

Development status of microcell UO2 pellet for accident-tolerant fuel

  • Kim, Dong-Joo;Kim, Keon Sik;Kim, Dong Seok;Oh, Jang Soo;Kim, Jong Hun;Yang, Jae Ho;Koo, Yang-Hyun
    • Nuclear Engineering and Technology
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    • v.50 no.2
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    • pp.253-258
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    • 2018
  • A microcell $UO_2$ pellet, as an accident-tolerant fuel pellet, is being developed to enhance the accident tolerance of nuclear fuels under accident conditions as well as the fuel performance under normal operation conditions. Improved capture-ability for highly radioactive and corrosive fission product (Cs and I) is the distinct feature of a ceramic microcell $UO_2$ pellet, and the enhanced pellet thermal conductivity is that of a metallic microcell $UO_2$ pellet. The fuel temperature can be effectively decreased by enhanced thermal conductivity. In this study, the material concepts of metallic and ceramic microcell $UO_2$ pellets were designed, and the fabrication process of microcell $UO_2$ pellets embodying the designed concept was developed. We successfully implemented the microcell $UO_2$ pellets and produced microcell $UO_2$ pellets. In addition, an assessment of the out-of-pile properties of a microcell $UO_2$ pellet was performed, and the in-reactor performance and behavior of the developed microcell pellets were evaluated through a Halden irradiation test. According to the expectations, the excellent performance of the microcell $UO_2$ pellets was confirmed by the online measurement data of the Halden irradiation test.

Calculation and measurement of Al prompt capture gammas above water in a pool-type reactor

  • Czakoj, Tomas;Kostal, Michal;Losa, Evzen;Matej, Zdenek;Simon, Jan;Mravec, Filip;Cvachovec, Frantisek
    • Nuclear Engineering and Technology
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    • v.54 no.10
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    • pp.3824-3832
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    • 2022
  • Prompt capture gammas are an important part of the fission reactor gamma field. Because some of the structural materials after neutron capture can emit photons with high energies forming the dominant component of the gamma spectrum in the high energy region, the following study of the high energy capture gamma was carried out. High energy gamma radiation may play a major role in areas of the radiation sciences as reactor dosimetry. The HPGe measurements and calculations of the high-energy aluminum capture gamma were performed at two moderator levels in the VR-1 pool-type reactor. The result comparison for nominal levels was within two sigma uncertainties for the major 7.724 MeV peak. A larger discrepancy of 60% was found for the 7.693 MeV peak. The spectra were also measured using a stilbene detector, and a good agreement between HPGe and stilbene was observed. This confirms the validity of stilbene measurements of gamma flux. Additionally, agreement of the wide peak measurement in 7-9.2 MeV by stilbene detector shows the possibility of using the organic scintillators as an independent power monitor. This fact is valid in these reactor types because power is proportional to the thermal neutron flux, which is also proportional to the production of capture gammas forming the wide peak.

Resonance Integral of Neptunium(237Np) from Energy Dependent Differential Neutron Capture Cross-Section by Using the Linac TOF Method and C6D6 Scintillation Spectrometer

  • Lee, Sam-Yol
    • Journal of the Korean Society of Radiology
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    • v.5 no.4
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    • pp.217-221
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    • 2011
  • $^{237}Np$ is very important material in the fission products of nuclear reactors. Resonance integral(RI) tests of this material is necessary to check between the experiments and the evaluated data. Such feedback to the evaluated data is very important to correct data and improve of codes. The RI for the $^{237}Np(n,{\gamma})^{238}Np$ reaction were measured by using the 46-MeV electron linear accelerator (linac) at the Research Reactor Institute, Kyoto University (KURRI). The measurement was performed in the energy region from 0.005 eV and 10 keV. RI obtained as 804.7 barns, compared with those of the evaluated data in JENDL-4.0 and Mughabghab.

Crystallite Size Measurement of Uranium Oxide Fuel Powders by Neutron Diffraction (중성자 회절에 의한 산화우라늄 핵연료 분말의 결정크기 측정)

  • 류호진;강권호;문제선;송기찬;최용남
    • Journal of Powder Materials
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    • v.10 no.5
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    • pp.318-324
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    • 2003
  • The nano-scale crystallite sizes of uranium oxide powders in simulated spent fuel were measured by the neutron diffraction line broadening method in order to analyze the sintering behavior of the dry process fuel. The mixed $UO_2$ and fission product powders were dry-milled in an attritor for 30, 60, and 120 min. The diffraction patterns of the powders were obtained by using the high resolution powder diffractometer in the HANARO research reactor. Diffraction line broadening due to crystallite size was measured using various techniques such as the Stokes' deconvolution, profile fitting methods using Cauchy function, Gaussian function, and Voigt function, and the Warren-Averbach method. The non-uniform strain, stacking fault and twin probability were measured using the information from the diffraction pattern. The realistic crystallite size could be obtained after separation of the contribution from the non-uniform strain, stacking fault and twin.

Elastic Modulus Measurement of a Dry Process Fuel Pellet by Resonant Ultrasound Spectroscopy (초음파 공진 분석법을 이용한 건식공정 핵연료 소결체의 탄성계수 측정)

  • 류호진;강권호;문제선;송기찬;정현규;정용무
    • Journal of Powder Materials
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    • v.11 no.4
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    • pp.314-321
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    • 2004
  • The elastic moduli of simulated dry process fuels with varying composition and density were measured in order to analyze the mechanical properties of a dry process fuel pellet. Resonant ultrasound spectroscopy(RUS) which can determine all elastic moduli with one set of measurements for a rectangular parallelepiped sample was used to measure the elastic moduli of UO$_{2}$ and simulated dry process fuel. The simulated dry process fuel showed a higher value of Young's modulus than UO$_2$ due to the presence of metallic precipitates and solid solution elements in the UO$_{2}$ matrix. The correlation between Young's modulus and porosity(P) of simulated dry process fuel was found to be 231.4-651.8 P (GPa) at room temperature. Dry process fuel with a higher burnup showed higher Young's modulus because total content of fission product element was increased.