• Title/Summary/Keyword: Atmospheric aerosol

Search Result 741, Processing Time 0.022 seconds

VARIABILITY OF THE TRENDS OBSERVED FROM SEAWIFS-DERIVED SUB-MICRON AEROSOL FRACTION OVER EAST ASIAN SEAS BASED ON DIFFERENT CLOUD MASKING ALGORITHMS

  • Li, Li-Ping;Fukushima, Hajime;Takeno, Keisuke
    • Proceedings of the KSRS Conference
    • /
    • v.1
    • /
    • pp.316-319
    • /
    • 2006
  • Monthly-mean aerosol parameters derived from the 1998-2004 SeaWiFS observations over East Asian waters are analyzed. SeaWiFS GAC Level 1 data covering the Northeast Asian area are collected and processed by the standard atmospheric correction algorithm released by the SeaWiFS Project to produce daily aerosol optical thickness (AOT) and ${{\AA}}ngstr{\ddot{o}}m$ exponent imageries. Monthly mean AOT and ${{\AA}}ngstr{\ddot{o}}m$ exponent values are extracted from the daily composite images for six study areas chosen from the surrounding waters of Japan. A slight increasing trend of ${{\AA}}ngstr{\ddot{o}}m$ exponent is found and interpreted as about 4-5% increase in submicron fraction of aerosol optical thickness at 550nm. Two cloud screening methods, including the standard cloud masking method of SeaWiFS and the one based on the local variance method, are applied to the SeaWiFS data processing, in an attempt to inspect the influence to the observed statistical uptrend which probably induced by different cloud mask algorithms. The variability comes from the different cloud masking algorithms are discussed.

  • PDF

Characteristics of Aerosol Particle Concentration by the Versatile Aerosol Concentration Enrichment System (VACES) (VACES을 이용한 대기 중 입자상물질의 농축기술 및 특성 연구)

  • Park, Jeong-Ho
    • Journal of Environmental Science International
    • /
    • v.21 no.11
    • /
    • pp.1339-1348
    • /
    • 2012
  • The versatile aerosol concentration enrichment system (VACES) have proven useful for providing elevated levels of atmospheric aerosol to human and animal exposures. In this study, we describe a VACES and tests conducted to both optimize the enhancement factor (EF) and characterize how it depends on experiment conditions. Particle number concentrations were measured from upstream and downstream of the system by scanning mobility particle sizer (SMPS) with a long differential mobility analyzer (DMA) in combination with a condensation particle counter (CPC). SMPS was used for to determine VACES particle EF. Particle EF tends to increase for higher the saturator temperature ($T_{Sat}$) and lower the condenser temperature ($T_{Con}$). $T_{Con}$ higher than $0^{\circ}C$ and $T_{Sat}$ lower than $50^{\circ}C$ was the best to obtain the most increase in particle concentration. Correlation analysis of EF with factor variables of $T_{Sat}$ and $T_{Con}$ resulted in correlation 0.662 and 0.416, respectively. With all five predictor variables included in a multiple regression model, the EF had a liner correlation with $R^2=0.643$.

Assessment of Long-Range Transport of Atmospheric Pollutants using a Trajectory Model with the puff Concept (퍼프 유적선모델에 의한 대기오염물질의 장거리수송량의 평가)

  • 정관영
    • Journal of Korean Society for Atmospheric Environment
    • /
    • v.12 no.2
    • /
    • pp.167-177
    • /
    • 1996
  • To investigate the source-receptor relationships aerosol model has been used to simulate the distribution behavior of the yellow sand. Data for meteorological fields were obtained by Meso-scale Analysis and Prediction Model System/Seoul National University (MAPMS/SNU) for five days (10-14 April 1988). To obtain the distributions of concentration of yellow sand,the aerosol model has been modified to allow quantifications of relative concentration distributions of yellow sand. Source regions of yellow sand were delineated by soil maps of China and emission rate as a function of wind stress(Westphal et al., 1987). Using 3-dimensional wind fields the backward trajectories from 3 receptor grids at the layer of .sigma. =0.95, 0.9, 0.85, 0.8 were calculated. In order to facilitate quantitative assessment of source-receptor relationships, it was assumed that the perturbations in along-trajectory and cross-trajectory proceed linearly with time, in accord with Gaussian distribution characteristics. On the basis of this assumption, the probability fields were calculated from every grid point with source strength 1. Using these probability fields and emission retes, the potential contributions of upstream sources along the trajectories were estimated. The results of this study indicate that the application of trajectory modeling is useful in investigating the quantitative relationship between source and receptor regions.

  • PDF

Retrieval of Dust Backscatter Coefficient using Quartz Raman Channel in Lidar Measurements (석영 라만 채널을 이용한 황사 후방 산란 계수 산출)

  • Noh, Young-Min;Mueller, Detlef;Lee, Han-Lim
    • Journal of Korean Society for Atmospheric Environment
    • /
    • v.28 no.1
    • /
    • pp.86-93
    • /
    • 2012
  • We present a retrieval method to obtain dust backscatter coefficient from the mixed Asian dust and pollutant layer. In the present study, vertically resolved quartz (silicon dioxide, silica) concentration was calculated using Raman scattering signals from quartz at 546 nm. Dust concentration was obtained based on typical mass percentage of quartz in Asian dust. The highest value of dust concentration at 3.7 km in March 21, 2010 was 22.3 and 10.9 ${\mu}gm^{-3}$ according to the quartz percentage in Asian dust as 65 and 30% based on literature survey, respectively. OPAC (Optical Properties of Aerosol and Clouds) simulations were conducted to calculate dust backscatter coefficient. The retrieved dust concentration was used as an input parameter for the OPAC calculations. Utilization of quartz Raman channel in Lidar measurements is considered useful for distinguishing optical properties of dust and nondust aerosol in the mixing state of Asian dust.

Time Resolved Analysis of Water Soluble Organic Carbon by Aerosol-into-Mist System (분진-미스트 시스템을 이용한 실시간 수용성 유기탄소 분석)

  • Cho, In-Hwan;Park, Da-Jeong;Bae, Min-Suk
    • Journal of Korean Society for Atmospheric Environment
    • /
    • v.31 no.6
    • /
    • pp.497-507
    • /
    • 2015
  • Real-time and quantitative measurement of the chemical composition in ambient aerosols represents one of the most challenging problems in the field of atmospheric chemistry. In the present study, time resolved application by Aerosol-into-Mist System (AIMS) following by total organic carbon analyzer (TOC) has been developed. The unique aspect of the combination of these two techniques is to provide quantifiable water soluble organic carbon (WSOC) information of particle-phase organic compounds on timescales of minutes. We also demonstrated that the application of the AIMS method is not limited to water-soluble organic carbon but inorganic ion compounds. By correlating the volume concentrations by optical particle sizer (OPS), water soluble organic carbon can be highly related to the secondary organic products. AIMS-TOC method can be potentially applied to probe the formation and evolution mechanism of a variety of SOA behaviors in ambient air.

Mass Size Distribution of Atmospheric Aerosol Particles with Nanosampler Cascade Impactor in Jinju City (다단 임팩터 Nanosampler를 이용한 진주시 대기에어로졸입자의 입경별 질량농도 특성)

  • Park, Jeong-Ho;Jang, Min-Jae;Kim, Hyoung-Kab
    • Journal of Environmental Science International
    • /
    • v.24 no.5
    • /
    • pp.679-687
    • /
    • 2015
  • Atmospheric aerosol particles were investigated at GNTECH university in Jinju city. Samples were collected using the Nanosampler period from January to December 2014. The Nanosampler is a 6 stage cascade impactor(1 stage : > $10{\mu}m$, 2 stage : $2.5{\sim}10{\mu}m$, 3 stage : $1.0{\sim}2.5{\mu}m$, 4 stage : $0.5{\sim}10{\mu}m$, 5 stage : $0.1{\sim}0.5{\mu}m$, back-up : < $0.1{\mu}m$) with the stages having 50% cut-off ranging from 0.1 to $10{\mu}m$ in aerodynamic diameter. The mass size distribution of Atmospheric aerosol particles was unimodal with peak at $1.0{\sim}2.5{\mu}m$ or $0.5{\sim}1.0{\mu}m$. The annual average concentrations of TSP, $PM_{10}$, $PM_{2.5}$, $PM_1$, $PM_{0.5}$ and $PM_{0.1}$ were $44.0{\mu}g/m^3$, $40.3{\mu}g/m^3$, $31.4{\mu}g/m^3$, $18.0{\mu}g/m^3$, $8.0{\mu}g/m^3$, $3.0{\mu}g/m^3$, respectively. On average $PM_{10}$, $PM_{2.5}$, $PM_1$, $PM_{0.5}$ and $PM_{0.1}$ make up 0.91, 0.70, 0.41, 0.19 and 0.07 of TSP, respectively. The annual average of $PM_{2.5}/PM_{10}$ ratio was 0.77.

Seasonal Variation and Measurement Uncertainty of UV Aerosol Optical Depth Measured at Gwangju, Korea (자외선 영역의 에어로졸 광학 깊이의 계절 분포 및 불확실도의 계산)

  • Kim, Jeong-Eun;Kim, Young-Joon
    • Journal of Korean Society for Atmospheric Environment
    • /
    • v.21 no.6
    • /
    • pp.631-637
    • /
    • 2005
  • A UV-MFRSR instrument was used to measure the global and diffuse irradiances in 7 narrowband channels in the UV range 299.4, 304.4, 310.9, 317.3. 324.5, 331.3 and 367.4 nm at Gwangju ($35^{circ}\;13'N\;126^{circ}\;50'E$), Korea. Spectral UV-AOD was retrieved using the Langley plot method for data collected from April 2002 to July 2004. Temporal variation of AOD at 367.4 nm ($AOD_{367nm}$) showed a maximum in June ($0.95\pm0.43$) and a minimum in February ($0.31\pm0.14$). Clear seasonal variation of $AOD_{367nm}$ was observed with average values of $0.68\pm0.29,\;0.82\pm0.41,\;0.48\pm0.22\;and\;0.42\pm0.21$ in spring, summer, fall and winter, respectively, Average Angstrom exponent for the entire monitoring period was $2.03\pm0.75$ in the UV-A ($324.5\∼367.4$ nm) range. Seasonal variation of the Angstrom exponent showed a maximum in spring and a minimum in summer. The lowest Angstrom exponent in summer might be due to hygroscopic growth of particles under conditions of high relative humidity. UV-AOD changes under different atmospheric conditions were also analyzed. Uncertainty in retrieving spectral UV-AOD was also estimated to range between $\pm0.218\;at\;304.4\;nm\;and\;\pm0.135\;at\;367.4\;nm$. Major causes of uncertainty were total column ozone retrieval and extraterrestrial irradiance retrieval at shorter and longer wavelengths, respectively.

Composition of Organic Compounds in the Ambient PM10 of the Anmyon Island (안면도 미세먼지 내 유기성분들의 분포 특성)

  • Lee, Ji Yi;Hwang, Eun Jin;Lim, Hyung Bae;Kim, Yu Won;Kim, Eun Sil;Kim, Yong Pyo
    • Particle and aerosol research
    • /
    • v.9 no.3
    • /
    • pp.187-197
    • /
    • 2013
  • To understand the characteristics of organic aerosol(OA) at the background atmosphere of Korea, an observation of atmospheric PM10 was conducted at a Global Atmospheric Watch(GAW) station operated by the Korean Meteorological Administration at Anmyon Island during 2010. Various organic compounds were analyzed from 26 samples by using a gas chromatography-mass spectrometer. Water soluble organic carbon(WSOC) was also analyzed by using a total organic carbon(TOC) analyzer. Among 6 classes with 68 target compounds detected, the classes of n-alkanoic and alkenoic acids ($326.67{\pm}75.40ngm^{-3}$) and dicarboxylic acids ($323.74{\pm}361.89ngm^{-3}$) were found to be major compound classes in the atmosphere of Anmyon Island. Compared to the previous results reported for 2005 spring samples at Gosan site, the concentrations of organic compounds at Anmyon Island were 3-10 times higher than Gosan site due to the difference of location and sampling period. The concentrations of organic compounds were varied with the atmospheric conditions. Significant increase of the concentrations of dicarboxylic and carboxylic acids in the smog episode indicated that secondary oxidation of organic compounds was major factor to increase OA concentration during smog episode in the Anmyon Island. It was found that the compositions of the OA measured at Anmyon Island were dependent on the air parcel trajectories.

Composition and Characteristics of ionic Components of Aerosols Collected at Gosan Site in Jeiu Island, Korea

  • Kang, Chang-Hee;Kim, Won-Hyung;Hu, Chul-Goo;Kim, Yong-Pyo;Shim, Shang-Gyoo;Hong, Min-Sun;Kim, Ki-Hyun
    • Journal of Korean Society for Atmospheric Environment
    • /
    • v.19 no.E4
    • /
    • pp.177-186
    • /
    • 2003
  • The total of 1,454 aerosol samples were collected by high volume tape sampler at the Gosan Site in Jeju Island from 1992 to 1999, and the major water-soluble ionic components were chemically analyzed. The mean concentrations of nss-S $O_4$$^{2-}$, N $H_4$$^{+}$, and N $O_3$$^{[-10]}$ showed high values, which were 6.73, 1.45, and 1.45 ${\mu}{\textrm}{m}$/㎥, respectively, while $Ca^{2+}$ and $K^{+}$ concentrations were low with the values of 0.49 and 0.42 $\mu\textrm{g}$/㎥. The concentrations of most components increased in spring but decreased in summer, especially with the remarkable increase of $Ca^{2+}$ and N $O_3$$^{[-10]}$ concentrations in spring. The seasonal comparison of nss-S $O_4$$^{2-}$ concentrations showed higher values with the order of spring > fall 〉 winter〉 summer, but spring 〉 winter〉 fall 〉 summer for N $O_3$$^{[-10]}$ Meanwhile, the concentration levels of N $a^{+}$ and C $l^{[-10]}$ increased more in winter season. According to the investigation of wind direction effect, the concentrations of most aerosol ionic components showed higher values consistently at the westerly and northerly wind conditions. Based on the factor analysis, the atmospheric aerosols in the Gosan Site are considered to be largely affected by marine sources, followed by anthropogenic and soil sources.urces..

Characteristics of Aerosol and Cloud Condensation Nuclei Concentrations Measured over the Yellow Sea on a Meteorological Research Vessel, GISANG 1 (기상 관측선 기상 1호에서 관측한 황해의 에어로졸과 구름응결핵 수농도 특성 연구)

  • Park, Minsu;Yum, Seong Soo;Kim, Najin;Cha, Joo Wan;Ryoo, Sang Boom
    • Atmosphere
    • /
    • v.26 no.2
    • /
    • pp.243-256
    • /
    • 2016
  • Total number concentration of aerosols larger than 10 nm ($N_{CN10}$), 3 nm ($N_{CN3}$), and cloud condensation nuclei ($N_{CCN}$) were measured during four different ship cruises over the Yellow Sea. Average values of $N_{CN10}$ and $N_{CCN}$ at 0.6% supersaturation were 6914 and $3353cm^{-3}$, respectively, and the minimum value of $N_{CN10}$ was $2000cm^{-3}$, suggesting significant anthropogenic influence even at relatively clean marine environment. Although $N_{CN10}$ and $N_{CN3}$ increased near the coast due to anthropogenic influence, $N_{CCN}$ was relatively constant and therefore $N_{CCN}/N_{CN10}$ ratio tended to decrease, suggesting that coastal aerosols were relatively less hygroscopic. In general $N_{CN10}$, $N_{CN3}$, and $N_{CCN}$ during the cruises seemed to be significantly influenced by wet scavenging effects (e.g. fog) and boundary layer height variation. Only one new particle formation (NPF) event was observed during the measurement period. Interestingly, the NPF event occurred during a dust storm event and spatial scale of the NPF event was estimated to be larger than 100 km. These results demonstrate that aerosol and CCN concentration over the Yellow Sea can vary due to various different factors.