• Title/Summary/Keyword: Atmospheric aerosol

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Aerosol Mass Spectrometer (AMS)-Based Real-Time Physicochemical Characterization of Atmospheric Aerosols

  • Kim, Donghwi
    • Mass Spectrometry Letters
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    • v.13 no.2
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    • pp.27-34
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    • 2022
  • Atmospheric aerosols have become a major environmental concern because of their adverse effects on human health, air quality, and climate change. Over the last few decades, several mass spectrometry (MS)-based techniques have been developed and applied in the field of atmospheric aerosol research. Particularly, real-time measurement of ambient aerosols using an aerosol mass spectrometer (AMS) has become one of the most powerful tools for aerosol chemistry. This review provides a brief description of AMS and its applications for understanding the physicochemical properties of atmospheric aerosols, as well as its sources and evolution processes.

Attenuation of the Atmospheric Aerosol Transmissivity due to Air Pollution (대기오염에 의한 대기투과도 감쇠에 대한 연구)

  • Kim, Yoo-Keun;Lee, Hwa-Woon;Lee, Yong-Seob
    • Journal of Korean Society for Atmospheric Environment
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    • v.11 no.E
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    • pp.23-29
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    • 1995
  • Relationship between atmospheric aerosol transmissivity and air pollution was analyzed using observed data in a large industrial city, Pusan, Korea. The atmospheric aerosol transmissivity predicted by method of present study in Pusan was assessed by the method of Yamamoto et al.(1968) in order to set up an empirical model to predict the transmissivity using the various meteorological parameters and air pollution. As a result, good correlation between these tow method re observed. Thus, it is possible to conclude that the parameterization of air pollution suggested by this study is another method to give reliable estimate of atmospheric aerosol transmissivity and direct solar irradiance in Pusan.

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Derivation of aerosol vertical profiles in Seoul based on O4 measurements using UV scanning spectrometer

  • Lee, Hanlim;Hwang, JungBae;Son, Yoonhee
    • Korean Journal of Remote Sensing
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    • v.29 no.3
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    • pp.325-329
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    • 2013
  • This present study describes an application of UV scanning spectrometer $O_4$ data for retrieval of aerosol vertical profiles in Seoul during the measurement period that includes two Asian dust event days. The results show large variations of aerosol load in vertical and temporal scales. Large variations in aerosol were observed at 1 km in height during the daytime in the measurement period when the Asian dust events took place. The aerosol load, however, was found to be largest at the surface compared to those retrieved at the higher atmospheric layers. The results also clearly identified the diurnal patterns of aerosol vertical distributions. The aerosol load was high in the morning and noon whereas it was low in the afternoon. This study demonstrates that UV scanning spectrometer observations of the oxygen dimer can serve as a potential method for determination of atmospheric aerosol vertical distributions and optical properties.

Operational Atmospheric Correction Method over Land Surfaces for GOCI Images

  • Lee, Hwa-Seon;Lee, Kyu-Sung
    • Korean Journal of Remote Sensing
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    • v.34 no.1
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    • pp.127-139
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    • 2018
  • The GOCI atmospheric correction overland surfaces is essential for the time-series analysis of terrestrial environments with the very high temporal resolution. We develop an operational GOCI atmospheric correction method over land surfaces, which is rather different from the one developed for ocean surface. The GOCI atmospheric correction method basically reduces gases absorption and Rayleigh and aerosol scatterings and to derive surface reflectance from at-sensor radiance. We use the 6S radiative transfer model that requires several input parameters to calculate surface reflectance. In the sensitivity analysis, aerosol optical thickness was the most influential element among other input parameters including atmospheric model, terrain elevation, and aerosol type. To account for the highly variable nature of aerosol within the GOCI target area in northeast Asia, we generate the spatio-temporal aerosol maps using AERONET data for the aerosol correction. For a fast processing, the GOCI atmospheric correction method uses the pre-calculated look up table that directly converts at-sensor radiance to surface reflectance. The atmospheric correction method was validated by comparing with in-situ spectral measurements and MODIS reflectance products. The GOCI surface reflectance showed very similar magnitude and temporal patterns with the in-situ measurements and the MODIS reflectance. The GOCI surface reflectance was slightly higher than the in-situ measurement and MODIS reflectance by 0.01 to 0.06, which might be due to the different viewing angles. Anisotropic effect in the GOCI hourly reflectance needs to be further normalized during the following cloud-free compositing.

A Study on the Concentration and Light Extinction of Atmospheric Aerosol in Seoul (서울 대기 에어로솔의 농도와 광소산에 관한 연구)

  • 김필수;오미석;김의훈
    • Journal of Korean Society for Atmospheric Environment
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    • v.7 no.3
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    • pp.227-234
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    • 1991
  • This study deals with concentration and light extinction of atmospheric aerosol in Seoul. From the measured aerosol size distribution for particle diameter ranging from 0.01 $\mum \sim 1.0 \mum$, extinction coefficient is calculated using the Mie theory. The results show that the diurnal variation of aerosol concentration, in general, reveals the lowest concentration in early morning and afternoon, while the highest at about 8 O'clock owing to the heavy traffic and accumulation of air pollution in the low atmosphere. However, aerosol concentration and extinction coefficient on April 7 give low values due to the advective wind. On the other hand, high aerosol concentration and extinction coefficenat are recorded on April 10 although solar radiation is weak. From the distribution of extinction coefficient we can find that aerosol particles of 0.1 $\mum \sim 1.0 \mum$ in diameter are highly effective on light extinction.

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12-year LIDAR Observations of Tropospheric Aerosol over Hefei (31.9°N, 117.2°E), China

  • Wu, Decheng;Zhou, Jun;Liu, Dong;Wang, Zhenzhu;Zhong, Zhiqing;Xie, Chenbo;Qi, Fudi;Fan, Aiyuan;Wang, Yingjian
    • Journal of the Optical Society of Korea
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    • v.15 no.1
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    • pp.90-95
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    • 2011
  • 12-year LIDAR observations of tropospheric aerosol vertical distribution using a Mie scattering LIDAR in Hefei ($31.9^{\circ}N$, $117.2^{\circ}E$) from 1998 to 2009 are presented and analyzed in this paper. Characters of temporal variation and vertical distribution of tropospheric aerosol over Hefei are summarized from the LIDAR measurements. The impacts of natural source and human activities on the aerosol vertical distribution over Hefei could be seen clearly. Dust particles from the north in spring could affect the aerosol distributions below about 12 km over Hefei, and aerosol scale height in April reaches $2.29{\pm}0.68\;km$. Both LIDAR measurements and surface visibility imply that aerosols in the lower troposphere have been increasing since about 2005.

A Study on Atmospheric Correction in Satellite Imagery Using an Atmospheric Radiation Model (대기복사모형을 이용한 위성영상의 대기보정에 관한 연구)

  • Oh, Sung-Nam
    • Atmosphere
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    • v.14 no.2
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    • pp.11-22
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    • 2004
  • A technique on atmospheric correction algorithm to the multi-band reflectance of Landsat TM imagery has been developed using an atmospheric radiation transfer model for eliminating the atmospheric and surface diffusion effects. Despite the fact that the technique of satellite image processing has been continually developed, there is still a difference between the radiance value registered by satellite borne detector and the true value registered at the ground surface. Such difference is caused by atmospheric attenuations of radiance energy transfer process which is mostly associated with the presence of aerosol particles in atmospheric suspension and surface irradiance characteristics. The atmospheric reflectance depend on atmospheric optical depth and aerosol concentration, and closely related to geographical and environmental surface characteristics. Therefore, when the effects of surface diffuse and aerosol reflectance are eliminated from the satellite image, it is actually corrected from atmospheric optical conditions. The objective of this study is to develop an algorithm for making atmospheric correction in satellite image. The study is processed with the correction function which is developed for eliminating the effects of atmospheric path scattering and surface adjacent pixel spectral reflectance within an atmospheric radiation model. The diffused radiance of adjacent pixel in the image obtained from accounting the average reflectance in the $7{\times}7$ neighbourhood pixels and using the land cover classification. The atmospheric correction functions are provided by a radiation transfer model of LOWTRAN 7 based on the actual atmospheric soundings over the Korean atmospheric complexity. The model produce the upward radiances of satellite spectral image for a given surface reflectance and aerosol optical thickness.

Single Particle Analysis of Atmospheric Aerosol Particles Collected in Seoul, 2001, Using Low-Z Particle Electron Probe X-ray Microanalysis (Low-Z Particle Electron Probe X-ray Microanalysis를 이용한 2001년 서울시 대기 중 입자상 물질 분석)

  • Koo Hee Joon;Kim HyeKyeong;Ro Chul-Un
    • Journal of Korean Society for Atmospheric Environment
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    • v.20 no.6
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    • pp.823-832
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    • 2004
  • Atmospheric aerosol particles collected in Seoul on four single days, each in every seasons of 2001, were characterized and classified on the basis of their chemical species using low-Z particle electron probe X-ray microanalysis (low-Z particle EPMA). Low-Z particle EPMA technique can analyze both the size and the chemical species of individual aerosol particles of micrometer size and provide detailed information on the size distribution of each chemical species. The major chemical species observed in Seoul aerosol were aluminosilicate, silicon dioxide, calcium carbonate, organic, carbon-rich, marine originated, and ammonium sulfate particles, etc. The soil originated species, such as aluminosilicate, silicon dioxide, and calcium carbonate were the most popular in the coarse fraction, meanwhile, carbonaceous and ammonium sulfate were the dominant species found in the fine fraction. Marine originated species such as sodium nitrate was frequently encountered, up to 30% of the analyzed aerosol particles.

Development of High Spectral Resolution Lidar System for Measuring Aerosol and Cloud

  • Zhao, Ming;Xie, Chen-Bo;Zhong, Zhi-Qing;Wang, Bang-Xin;Wang, Zhen-Zhu;Dai, Pang-Da;Shang, Zhen;Tan, Min;Liu, Dong;Wang, Ying-Jian
    • Journal of the Optical Society of Korea
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    • v.19 no.6
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    • pp.695-699
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    • 2015
  • A high spectral resolution lidar (HSRL) system based on injection-seeded Nd:YAG laser and iodine absorption filter has been developed for the quantitative measurement of aerosol and cloud. The laser frequency is stabilized at 80 MHz by a frequency locking system and the absorption line of iodine cell is selected at the 1111 line with 2 GHz width. The observations show that the HSRL can provide vertical profiles of particle extinction coefficient, backscattering coefficient and lidar ratio for cloud and aerosol up to 12 km altitude, simultaneously. For the measured cases, the lidar ratios are 10~20 sr for cloud, 28~37 sr for dust, and 58~70 sr for urban pollution aerosol. It reveals the potential of HSRL to distinguish the type of aerosol and cloud. Time series measurements are given and demonstrate that the HSRL has ability to continuously observe the aerosol and cloud for day and night.

Detection and Classification of Major Aerosol Type Using the Himawari-8/AHI Observation Data (Himawari-8/AHI 관측자료를 이용한 주요 대기 에어로솔 탐지 및 분류 방법)

  • Lee, Kwon-Ho;Lee, Kyu-Tae
    • Journal of Korean Society for Atmospheric Environment
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    • v.34 no.3
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    • pp.493-507
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    • 2018
  • Due to high spatio-temporal variability of amount and optical/microphysical properties of atmospheric aerosols, satellite-based observations have been demanded for spatiotemporal monitoring the major aerosols. Observations of the heavy aerosol episodes and determination on the dominant aerosol types from a geostationary satellite can provide a chance to prepare in advance for harmful aerosol episodes as it can repeatedly monitor the temporal evolution. A new geostationary observation sensor, namely the Advanced Himawari Imager (AHI), onboard the Himawari-8 platform, has been observing high spatial and temporal images at sixteen wavelengths from 2016. Using observed spectral visible reflectance and infrared brightness temperature (BT), the algorithm to find major aerosol type such as volcanic ash (VA), desert dust (DD), polluted aerosol (PA), and clean aerosol (CA), was developed. RGB color composite image shows dusty, hazy, and cloudy area then it can be applied for comparing aerosol detection product (ADP). The CALIPSO level 2 vertical feature mask (VFM) data and MODIS level 2 aerosol product are used to be compared with the Himawari-8/AHI ADP. The VFM products can deliver nearly coincident dataset, but not many match-ups can be returned due to presence of clouds and very narrow swath. From the case study, the percent correct (PC) values acquired from this comparisons are 0.76 for DD, 0.99 for PA, 0.87 for CA, respectively. The MODIS L2 Aerosol products can deliver nearly coincident dataset with many collocated locations over ocean and land. Increased accuracy values were acquired in Asian region as POD=0.96 over land and 0.69 over ocean, which were comparable to full disc region as POD=0.93 over land and 0.48 over ocean. The Himawari-8/AHI ADP algorithm is going to be improved continuously as well as the validation efforts will be processed by comparing the larger number of collocation data with another satellite or ground based observation data.