• Title/Summary/Keyword: Ambient aerosol

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Characterization of Atmospheric Dispersion Pattern from Large Sources in Chungnam, Korea (충남지역 대형사업장의 대기오염물질 확산 특성 파악)

  • Choi, Woo Yeong;Park, Min Ha;Jung, Chang Hoon;Kim, Yong Pyo;Lee, Ji Yi
    • Particle and aerosol research
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    • v.17 no.3
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    • pp.55-69
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    • 2021
  • Chungnam region accounts for the largest SOX (22.8%) emission with the second-largest NOX (10.8%) emission in Korea due to the integration of many large industrial sources including a steel mill, coal-fired power plants, and petrochemical complex. Air pollutants emitted by large industrial sources can cause harmful problems to humans and the environment. Thus, it is necessary to understand dispersion patterns of air pollutants from large industrial sources in Chungnam to characterize atmospheric contamination in Chungnam and the surrounding area. In this study, seasonal atmospheric dispersion characteristics for SOX, NOX, and PM2.5 from ten major point sources in Chungnam were evaluated using HYSPLIT 4 model, and their contributions to SO2, NO2 concentrations in the regions near the source areas were estimated. The predictions of the HYSPLIT 4 model show a seasonal different dispersion pattern, in which air pollutants were dispersed toward the southeast in winter while, northeast in summer. In summer, due to weaker wind speed, air pollutants concentrations were higher than in winter, and they were dispersed to the metropolitan area. The local emissions of air pollutants in Taean area had a greater influence on the ambient SO2 and NO2 concentrations at Taean, whereas SOX and NOX emissions from large sources located at Seosan showed relatevely little effect on the ambient ambient SO2 and NO2 concentrations at Seosan.

Effect of Air Stagnation Conditions on Mass Size Distributions of Water-soluble Aerosol Particles (대기 정체와 수용성 에어로졸 입자의 질량크기분포의 관계)

  • Park, Seungshik;Yu, Geun-Hye
    • Journal of Korean Society for Atmospheric Environment
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    • v.34 no.3
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    • pp.418-429
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    • 2018
  • Measurements of 24-hr size-segregated ambient particles were made at an urban site of Gwangju under high pressure conditions occurred in the Korean Peninsula late in March 2018. The aim of this study was to understand the effect of air stagnation on mass size distributions and formation pathways of water-soluble organic and inorganic components. During the study period, the $NO_3{^-}$, $SO_4{^{2-}}$, $NH_4{^+}$, water-soluble organic carbon (WSOC), and humic-like substances(HULIS) exhibited mostly bi-modal size distributions peaking at 1.0 and $6.2{\mu}m$, with predominant droplet modes. In particular, outstanding droplet mode size distributions were observed on March 25 when a severe haze occurred due to stable air conditions and long range transport of aerosol particles from northeastern regions of China. Air stagnation conditions and high relative humidity during the study period resulted in accumulation of primary aerosol particles from local emission sources and enhanced formation of secondary ionic and organic aerosols through aqueous-phase oxidations of $SO_2$, $NO_2$, $NH_3$, and volatile organic compounds, leading to their dominant droplet mode size distributions at particle size of $1.0{\mu}m$. From the size distribution of $K^+$ in accumulation mode, it can be inferred that in addition to the secondary organic aerosol formations, accumulation mode WSOC and HULIS could be partly attributed to biomass burning emissions.

Quantitative Source Estimation of Particulate Matters in Suwon Area Using the Target Transformation Factor Analysis Based on Size Segregation Scheme (입경 분류에 입각하여 목표변환 인자분석법을 이용한 수원지역 분진 오염원의 정량적 기여도 추정)

  • 김동술;이태정
    • Journal of Korean Society for Atmospheric Environment
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    • v.9 no.1
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    • pp.44-50
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    • 1993
  • The suspended particulate matters had been collected by a cascade impactor having 9 size fragnated stages for 2 years (Dec. 1989 to Nov. 1991) in Kyung Hee University-Suwon Campus. The particulate matters were then collected on each stage by membrane filters. The weight concentration on each stage was estimated by a microbalance and further chemical element concentrations were determined by an XRF system. The study focused on developing of a receptor model using the TTFA (target transformation factor analysis) to apportion aerosol mass with the 30 ambient data sets. Each data set consists of the 8 size-ranged subdata sets characterized by 13 element variables. Even though a couple of sources could not be identified, three to five sources were extracted from each aerosol size-range, and then 9 statistical source profiles were generated. Finally, source contribution of particulate matters on each size-range could be estimated in Suwon area.

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Quantitative Source Estimation of Particulate Matters in Pusan Area Using the Target Transformation Factor Analysis (Target Transformation Factor Analysis를 이용한 부산시 분진오염원의 양적 추정)

  • 김태오;김동술;나진균
    • Journal of Korean Society for Atmospheric Environment
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    • v.6 no.2
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    • pp.135-146
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    • 1990
  • The purpose of the study was to identify sources of particulate matters statistically and to estimate the mass contribution quantitatively in the Pusan metropolitan area. Then, the study has used the TTFA (target transformation factor analysis) model, a receptor model, to apportion aerosol mass with the raw data of 106 ambient samples characterized by 24 heavy metal variables. The TTFA was extensively applied to generate source profiles and their aerosol mass contributions. Though a couple of sources were not identified, four to seven sources were able to be extracted at 3 different sites (Jang Rim-Dong, Kwang Bok-Dong, and Kwang An-Dong) in Pusan area and finally mass conributions could be calculated.

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Numerical evaluation of risk rates for contamination sources in a minienvironment (클린룸 국소환경에서 오염원의 위험율에 대한 수치해석적 평가)

  • Noh, Kwang-Chul
    • Particle and aerosol research
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    • v.14 no.4
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    • pp.181-189
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    • 2018
  • In this study, the risk rates of different contamination sources of the contaminant in a minienvironment were analyzed through Computational Fluid Dynamics (CFD) simulation. The airflow pattern characteristics can only predict the qualitative variation of contaminant concentration, but cannot evaluate the quantitative variations in the risk rate of sources. From the results, the ambient contamination sources mainly affect wafers in the Front Opening Unified Pod (FOUP), whereas the internal contamination sources mainly affect wafers laid on the robot arm in the minienvironment. And the purging plenum system is very useful in protecting the wafers in the FOUP from contaminants transferred from the Fan Filter Unit (FFU). However, this system is unable to protect the wafers on the robot arm from internal contaminants and the wafers in the FOUP from sources of the interface between the FOUP and the minienvironment.

Characterization of Particle Losses in a Perma Pure Dryer

  • R. B. Xiang;Lee, K. W.;C. H. Jung;Kim, J. Y.;Park, B. C.
    • Proceedings of the Korea Air Pollution Research Association Conference
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    • 2002.04a
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    • pp.237-238
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    • 2002
  • Particle - bound water changes the physical and chemical properties of aerosol particles, such as size and light scattering properties. Consequently, it is necessary to remove water vapor from ambient aerosols before aerosol particles are sized and counted. Silicon gel diffusion dryer is commonly employed for this purpose. However, it can not be operated continuously While in operation, silicon gel becomes progressively more loaded with water and must periodically be regenerated by drying off the water. (omitted)

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Effect of Ambient Temperature on the Distribution of Atmospheric Concentrations of Polycyclic Aromatic Hydrocarbons in the Vapor and Particulate Phases (대기 중 다환방향족탄화수소의 기체-입자상 농도분포에 미치는 주변 온도의 영향)

  • 백성옥;최진수
    • Journal of Korean Society for Atmospheric Environment
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    • v.14 no.2
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    • pp.117-132
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    • 1998
  • The main purposes of this study are to investigate the distributional characteristics of polycyclic aromatic hydrocarbons (PAH) in the vapor and particulate phases in the ambient atmosphere, and to evaluate the effect of ambient temperature on the vapor-particle partitioning during the sampling period. A total of 64 samples were collected during a period of 1995 to 1996, using a medium-volume sampler with XAD-2 adsorbents and quartz fiber filters. Analyses of PAH were carried out using HPLC with UV and Fluorescence detections. In this study, a significant seasonal variation in the distributions was observed, reflecting the effect of ambient temperature on the vapor-particle partitioning of PAH. The relationship between the vapor-particle distributions of the 3 to 5 rings PAH and ambient temperature is considered to be well described using the Langmuir adsorption concept. The estimated empirical constants for each PAH in the relationship, particularly for the more volatile compounds, were also comparable with results from other studies. However, it is still difficult to accurately estimate the initial vapor-particle distribution of PAH in the ambient air, since it is not known to what extent the trapped vapours originated from the particles laden in the filter by being volatilized or from the air samples initially present in the vapour phase. The distribution factors for volatile PAH with 3 to 4 rings appeared to be comparable with those in the literature. It should be noted, however, that these distribution factors give information only about the distribution of PAH between the two phases under a specific sampling condition, and hence may provide only semi -quantitative information on the vapor-particle distributions in the atmosphere.

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Concentrations of Particulate and Gaseous Ionic and Organic Species in the Ambient Air of the Yochon Industrial Estate (여천공단 대기 중의 입자상 및 기세상 이온성분과 유기화합물의 농도)

  • 김용표;이종훈;진현철;문길주
    • Journal of Korean Society for Atmospheric Environment
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    • v.13 no.4
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    • pp.269-284
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    • 1997
  • The ambient concentrations of gaseous and particulate phase ionic species and gaseous organic species in the Yochon industrial estate were measured during the spring ans summer of 1996. A three-stage filter pack sampler was used to collect particles and gaseous species, and stainless steel air sampling containers were used to collect air samples for organic species analyses. The concentrations of ions in aerosol wree comparable to those measured in Seoul. Aerosols measured were acidic, thus, most volatile acidic species were in the gas phase. The concentrations of organic species were highly variable, implying those were strongly dependent on the emissions of organic species from petrochemical plants. The concentrations of a few hazardous organic components were higher than those in Seoul or some populated areas in USA.

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Characteristics of Ambient Aerosol Sizers (대기 에어로졸 입경분포 측정기의 특성 비교)

  • 배귀남;김민철;지준호;이승복;문길주
    • Proceedings of the Korea Air Pollution Research Association Conference
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    • 2003.11a
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    • pp.211-212
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    • 2003
  • 지금까지는 주로 대기질 기준을 근거로 24시간 평균 TSP(total suspended particulates), PM$_{10}$, PM$_{2.5}$를 측정하여 왔다. 대기 에어로졸의 농도나 입경분포에 영향을 미치는 배출량, 기온, 상대습도, 풍향, 풍속, 혼합고 등이 12~24시간 이내의 스케일로 변한다(Shen et al., 2002). 그러므로, 대기 에어로졸의 일변화 특성을 파악하기 위하여 실험실에서 사용되던 실시간 에어로졸 입경분포 측정기가 대기 에어로졸 모니터링에 활용되고 있으며(배귀남 등, 2003; Woo et at., 2001; Laitinen et al., 1996), 최근에는 대기 에어로졸을 모니터링을 목적으로 개발된 제품이 시판되고 있다.(중략)략)

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Major Factors Affecting PM2.5 Water Content in Seoul and Gosan (서울과 고산의 미세입자 수분함량에 영향을 미치는 주요 인자)

  • Choi E. K;Kim Y.P
    • Journal of Korean Society for Atmospheric Environment
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    • v.20 no.6
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    • pp.803-810
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    • 2004
  • Water contents in fine particles at Seoul and Gosan are estimated by using a gas/particle equilibrium model, SCAPE (Simulating Composition of Atmospheric Particles at Equilibrium). Also, sensitivity of particulate inorganic ionic concentrations on the total ionic species is estimated. Water content at Gosan is more sensitive to ambient relative humidity (RH) than Seoul. At both sites water content is most sensitive to sulfate concentration among sulfate, nitrate, and ammonium. Solid salts levels and compositions are also studied.