• 한국대기환경학회지
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• 제33권2호
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• pp.174-183
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• 2017

The background level and timely variation characteristics of atmospheric $^{222}Rn$ concentrations have been evaluated by the real time monitoring at Gosan site of Jeju Island, Korea, during 2008~2015. The average concentration of atmospheric radon was $2,480mBq\;m^{-3}$ for the study period. The cyclic seasonality of radon was characterized such as winter maximum and summer minimum, consistent with the reduction in terrestrial fetch going to summer. On monthly variations of radon, the mean concentration in October was the highest as $3,041mBq\;m^{-3}$, almost twice as that in July ($1,481mBq\;m^{-3}$). The diurnal radon concentrations increased throughout the nighttime approaching to the maximum ($2,819mBq\;m^{-3}$) at around 7 a.m., and then gradually decreased throughout the daytime by the minimum ($2,069mBq\;m^{-3}$) at around 3 p.m. The diurnal radon cycle in winter showed comparatively small amplitude due to little variability in atmospheric mixing depth, conversely, large amplitude was observed in summer due to relatively a big change in atmospheric mixing depth. The cluster back-trajectories of air masses showed that the high radon events occurred by the predominant continental fetch over through Asia continent, and the radon concentrations from China continent were about 1.9 times higher on the whole than those from the North Pacific Ocean. The concentrations of $PM_{10}$ also increased in proportion to the high radon concentrations, showing a good linear correlation between $PM_{10}$ and radon concentrations.

• 분석과학
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• 제29권2호
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• pp.65-72
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• 2016

액체섬광계수기(Liquid Scintillation Counter, LSC)를 이용한 토양 중 ²²⁶Ra 분석 방법에 대해 연구하였다. 용융법으로 토양에서 Ra을 추출하고, Ba(Ra)SO₄로 침전시켜 방해핵종과 Ra을 분리하였다. Ba(Ra)SO₄를 산에 녹을 수 있는 Ba(Ra)CO₃로 변환시키고, 라돈 가스를 포집할 수 있는 소수성 섬광용액과 혼합한 다음, LSC로 분석하였다. ²²⁶Ra과 ⁹⁰Sr 표준시료를 이용하여 최적의 PSA(Pulse shape analysis, 파형분석) 준위를 설정하였다. FOM(Figure of merit, 성능지수)이 최대이고 알파선 중첩정도가 최소로 나타나는 PSA 80을 최적값으로 결정하였다. Glass vial을 사용했을 때 계측 효율은 243±2% 이다. 본 연구에서 개발한 분석법은 IAEA-312, IAEA-314, IAEA-315를 이용하여 그 신뢰도를 평가를 하였다. 회수율은 60~82% 이며, 측정값과 참고값과의 상대편의가 10 % 이내였다. 최소검출농도는 토양 1 g, 바탕 계수율 0.02 cpm일 때, 회수율 70 %, 계측시간 30 분을 기준으로 2.1 Bq kg⁻¹ 이다.

• 한국대기환경학회지
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• 제29권1호
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• pp.86-96
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• 2013

The realtime monitoring of radon ($^{222}Rn$) concentrations has been carried out from Gosan site, Jeju Island for three years of 2006~2008, in order to evaluate the background level and timely variational characteristics of atmospheric radon. The mean concentration of radon measured during the studying period was $2965mBq/m^3$ with its annual mean values in the range of $2768{\sim}3124mBq/m^3$. The relative ordering of the seasonal mean concentrations was seemed to vary such as winter ($3578mBq/m^3$) > fall ($3351mBq/m^3$) > spring ($2832mBq/m^3$) > summer ($2073mBq/m^3$). The monthly mean concentrations were in the order of Jan>Feb>Oct>Nov>Dec>Mar> Sep>Apr>May>Jun>Aug>Jul, so that the highest January value ($3713mBq/m^3$) exceeded almost twice as the July minimum ($1946mBq/m^3$). The hourly concentrations in a day showed the highest level ($3356mBq/m^3$) at around 7 a.m., increasing during nighttime, while reaching the lowest ($2574mBq/m^3$) at around 3 p.m. From the backward trajectory analysis for a continental fetch of radon, the high concentrations (10%) of radon matched with the air mass moving from the Asia continent to Jeju area. In contrast, the low concentrations (10%) of radon were generally correlated with the air mass of the North Pacific Ocean. In comparison by sectional inflow pathways of air mass, the radon concentrations were relatively high from the north China and the Korean peninsula.

• 한국대기환경학회지
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• 제34권2호
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• pp.321-330
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• 2018

Concentrations of the atmospheric radon and gaseous pollutants were measured at the Gosan site on Jeju Island from 2010 to 2015, in order to observe their time-series variation characteristics and examine the concentration change related to the airflow transport pathways. Based on the realtime monitoring of the atmospheric radon and gaseous pollutants, the daily mean concentrations of radon ($^{222}Rn$) and gaseous pollutants($SO_2$, CO, $O_3$, $NO_x$) were $2,400mBq\;m^{-3}$ and 1.3, 377.6, 41.1, 3.9 ppb, respectively. On monthly variations of radon, the mean concentration in October was the highest as $3,033mBq\;m^{-3}$, almost twice as that in July ($1,452mBq\;m^{-3}$). The diurnal variation of radon concentration shows bimodal curves at early morning (around 7 a.m.) and near midnight, whereas its lowest concentration was recorded at around 3 p.m. Several gaseous pollutants($SO_2$, CO, $NO_x$) showed a similar seasonal variation with radon concentration as high in winter and low in summer, whereas the $O_3$ concentrations had a bit different seasonal trend. According to the cluster back trajectory analysis, the frequencies of airflow pathways moving from continental North China, East China, Japan and the East Sea, the Korean Peninsula, and North Pacific Ocean routes were 36, 37, 10, 13, and 4%, respectively. When the airflow were moved to Jeju Island from continental China, the concentrations of radon and gaseous pollutants were relatively high. On the other hand, when the airflows were moved from North Pacific Ocean and East Sea, their concentrations were much lower than those from continental China.

• 자원환경지질
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• 제30권1호
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• pp.51-60
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• 1997

The high radon (Rn222) potentials of soil, groundwater, hotspring and indoor environments in the Taejon city area were delineated by use of an EDA RDA-200 radon detector. The U and Th contents were also analysed using a Multi Channel Analyzer to illustrate the sources of the radon potentials. The average U concentrations in Taejon vary according to the type of granites such as $4.14{\pm}2.36ppm$ in schistose granite (SG), $3.13{\pm}1.70ppm$ in biotite granite (BG) and $3.01{\pm}1.95ppm$ in two mica granite (TG). The U contents in the granites are closely related with the amounts of uraniferous minerals. However, the U contents in the soil are found to be $5.05{\pm}4.75ppm$ in TG, $4.07{\pm}1.69ppm$ in BG and $3.87{\pm}1.91ppm$ in SG which are mainly explained by the different cation exchange capacities (CEC) of the soils from various granites. The levels of soil radon are $552{\pm}656pCi/l$ in SG, in which levels at two locations exceed the level of 1,350 pCi/l established as guideline for follow-up action by the U.S. Environmental Protection Agency (EPA), $443{\pm}284pCi/l$ in TG and $224{\pm}115pCi/l$ in the BG. The soil radon concentrations are found to be proportional to the U content and hardness of the soils. The groundwater radon concentrations in the domestic wells of - 30~-100 m depth show that $6,907{\pm}4,665pCi/l$ in TG, $5,503{\pm}6,551pCi/l$ in SG and $2,104{\pm}1,157pCi/l$ in BG which are positively related with U contents in soils. The radon levels of six groundwater wells in TG and two in SG are greater than guideline for drinking water level, 10,000 pCi/l by EPA (1986). Average radon contents of hotsprings and public bathes in the TG area are $7,071{\pm}1,942pCi/l$ and $1,638{\pm}709pCi/l$, respectively, which are below the EPA standard for remedial action value of the 10,000 pCi/l. The mean indoor radon concentrations of the TG and SG areas are $1.60{\pm}1.20pCi/l$ and $1.60{\pm}0.70pCi/l$, respectively. The elevated indoor radon levels of 5.6 pCi/l and 6.7 pCi/l are found to be particularly in TG area, which exceeds 4 pCi/i guideline, correlating positively with the U contents in the soil and radon concentration in the groundwater.