• Title/Summary/Keyword: $^{137}Cs$ 방사성 핵종

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Key Parameters Analysis of Important Radionuclides in Dose Evaluation Model of Decommissioning Site (해체 부지 선량평가모텔의 주요 핵종에 대한 Key parameter 분석)

  • 임용규;김학수;손중권;박경록;강기두;김경덕;정찬우
    • Proceedings of the Korean Radioactive Waste Society Conference
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    • 2004.06a
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    • pp.52-57
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    • 2004
  • In order to analyze key parameters of important radionuclides in dose evaluation model of decommissioning site, a sensitivity analysis was performed. This analysis assumed a resident farmer for an exposure scenario and 0.037Bq/g for the concentration of radionuclides. As a result of sensitivity analysis, the key parameters of radionuclides considered were the area of contaminated zone, external gamma shielding factor and indoor time fraction for Cs-137 and Co-60. The key parameters for C-14 were the environmental parameters and hydrological parameters of unsaturated zone. Also, the key parameter for Sr-90 was the density of contaminated zone.

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A Study on the Determination of Radionuclide Concentrations in Animal Feedstuffs for Use Following a Nuclear Emergency (원자력 비상시 가축의 사료로 이용을 위한 사료내 방사성 핵종농도 결정에 대한 연구)

  • Hwang, Won-Tae;Kim, Eun-Han;Suh, Kyung-Suk;Choi, Young-Gil;Han, Moon-Hee
    • Journal of Radiation Protection and Research
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    • v.26 no.2
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    • pp.87-91
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    • 2001
  • The optimized derived intervention levels for animal products were evaluated based on cost-benefit analysis. From these results, the radionuclide concentrations in animal feedstuffs for use were derived. It was shown that radionuclide concentrations in animal feedstuffs for use depend strongly on animal products, radionuclides and feeding period (period from the starting time to be led with contaminated feedstuffs to production time of animal products). In case of feedstuffs contaminated with long-lived radionuclides ($^{l37}Cs,\;^{90}Sr$), the feedstuffs with lower contamination should be supplied to animals with increase of feeding period due to the bioaccumulation of radionuclides. While, in case of feedstuffs contaminated with short-lived radionuclides ($^{131}I$), the feeding of higher contaminated feedstuffs was possible with increase of feeding period due to radionuclide decay. It was shown that $^{137}Cs$ concentration in animal feedstuffs lot use was lower than $^{90}Sr$ concentration. It is primarily, due to the higher feed-animal product transfer factor of $^{137}Cs$.

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Distribution Characteristics of Radionuclies (60Co, 137Cs) During the Melting of Radioactive Metal Waste (방사성 금속폐기물의 용융시 방사성 핵종(60Co, 137Cs)의 분배특성)

  • Min, Byung Youn;Choi, Wang Kyu;Oh, Won Zin;Jung, Chong Hun;Kang, Yong
    • Korean Chemical Engineering Research
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    • v.45 no.6
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    • pp.627-632
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    • 2007
  • A fundamental study on the melt decontamination of metal wastes generated by dismantling the nuclear facility, the melting of metal wastes such as stainless steel and carbon steel have been carried out to investigate the distribution phenomena of the radioisotopes such as $^{60}Co$ and $^{137}Cs$ into the ingot, slag and dust phases by using the various slag types, slag concentration and basicity in an arc furnace. The $^{60}Co$ remained homogeneously in the ingot phase above 90 % and it was barely present in the slag below 10 %. The effect of the slag composition on the distribution for Co-60 was not considerable, but a basic slag former with high fluidity showed effective. $^{137}Cs$ was completely eliminated from the melt of the stainless steel as well as the carbon steel and distributed to the slag and the dust phase.

A Model for Evaluating the Radioactive Contamination in the Urban Environment (도시환경에서 방사성물질의 오염평가 모델개발)

  • Hwang, Won-Tae;Kim, Eun-Han;Jeong, Hyo-Joon;Suh, Kyung-Suk;Han, Moon-Hee
    • Journal of Radiation Protection and Research
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    • v.30 no.3
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    • pp.99-105
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    • 2005
  • A model for evaluating radioactive contamination in the urban environment, named METRO-K, was developed as a basic step for accident consequence analysis in case of an accidental release. The three kind of radionuclides $(^{137}Cs,\;^{106}Ru,\;^{131}I)$ and the different chemical forms of iodine (particulate, organic and elemental forms) are considered in the model. The radioactive concentrations are evaluated for the five types of surface (roof, paved road, wall, lawn/soil, tree) as a function of time. Using the model, the contaminative impacts of the surfaces were intensively investigated with respect to with and without precipitation during the measurement periods of radionuclides in air. In addition, a practical application study was conducted using $^{137}Cs$ concentration in air and precipitation measured in an European country at the Chernobyl accident. As a result precipitation was an influential factor in surface contamination. The degree of contamination was strongly dependent on the types of radionuclide and surface. Precipitation was more influential in contamination of $^{137}Cs$ than that of $^{131}I$ (elemental form).

A Study on the Underground Movement of Radionuclides(I) (방사성핵종의 지하이동 연구)

  • Hun Hwee Park;Kyong Won Han;Nak June Sung;Chul Soo Kim
    • Nuclear Engineering and Technology
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    • v.16 no.2
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    • pp.64-69
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    • 1984
  • With regard to the radioactive waste disposal, adsorption properties and migration rates have been evaluated for Cs-137 and Sr-90 with the domestic clay sampled from Cnyang, Sanchong and Mooan. Sorption coefficients (Ksorp) were determined by batch experiments. The measured values of Ksorp were ranged from 8000 to 17,000 ml/gr for Cs-137 of 0.1$\mu$Ci/ml, and from 10,000 to 15,000m1/gr for Sr-90 of 0.l$\mu$Ci/ml. Remarkably, Mooan clay showed lower values of Ksorp than those of the others. This could be explained by the poor soprtion capacity of the quartz found only in the Mooan clay. For the quantitative analysis, sorption isotherm equations of Freundlich type were made with the obtained values of Ksorp. $C_{R}$=18.0 $C_{A}$$^{0.74}$ : Cs-137, $C_{R}$=0.84 $C_{A}$$^{0.45}$ : Sr-90. By introducing the BOX model combined with the above relationships, simulation of underground nuclide movement was carried out. The results showed that the domestic clays could be the effective backfill material for repositories.itories.ies.

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Studies on the Sorption and Fixation of Cesium by Vermiculite (II)

  • Lee, Sang-Hoon
    • Nuclear Engineering and Technology
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    • v.6 no.2
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    • pp.97-111
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    • 1974
  • The adsorption mechanism of Cs-137 in low level radioactive solution by vermiculite treated with Na ion is studied in order to investigate its effective utilization for the radioactive effluent treatment. The beneficial role of Na-vermiculite is that Na ion can induce the wider c-axis spacing in which Cs ion can be sorbed in vermiculite. Cation exchange capacity and distribution coefficient of cesium seems to be influenced by the variation of c-axis spacing of vermiculite. Comparative identification and detection with the characteristic analyses of X-ray diffraction and electron diffraction patterns, diffrential thermal analysis and electron microscopy of Na-, K- and Cs-vermiculite are studied for the phemomena of Cs adsorption by vermiculite. This importance of the utilization in terms of adsorption and fixation of cesium involving vermiculite is discussed. It is found that the Na-vermiculite is valuable outside charging material for high level radioactive liquid waste storage tank of underground to protect the pollution of the underground water.

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고순도게르마늄(HPGe) 검출기를 이용한 방사성폐기물 드럼의 핵종농도 평가

  • 박경록;강덕원
    • Proceedings of the Korean Nuclear Society Conference
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    • 1996.11b
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    • pp.583-589
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    • 1996
  • 원자력발전소에서 발생되는 방사성폐기물들은 폐기물형태 및 방사능 농도가 다양하며 영구처분장으로 이송전까지는 발전소내의 임시 저장고에 안전하게 보관, 관리하고 있다. 생성된 폐기물드럼내에는 감마방출핵종을 비롯하여 알파 및 베타방출 핵종들이 균질 또는 비균질하게 존재하고 있으며 방사능의 세기나 폐기물의 특성에 따라 안정화시키거나 압축처리하여 드럼에 담겨져 있기 때문에 일반적인 파괴분석에 의한 화학분석법으로는 작업자의 피폭, 시료의 대표성 선정 및 장시간의 화학처리 시간소요 등으로 핵종분석이 곤란하다. 따라서 본 논문은 일반적으로 감마핵종분석시 흔히 사용하고 있는 고순도게르마늄(HPGe) 검출기를 이용하여 드럼의 감마핵종농도를 분석하는 방법과 장치의 개발에 대해 언급하였으며 알파나 베타핵종과 같이 직접 분석이 곤란한 핵종들은 각 폐기물드럼내에 존재하는 Co-60이나 Cs-137과의 상관관계를 미리 예측한 척도인자 (scaling factor)를 이용하여 간접적으로 구하는 방법을 사용하고 있으나 본 논문에서는 드럼으로부터 감마핵종만을 분석하는 방법에 대해서만 언급하였다. 또한 핵종분석시스템의 최적 운전조건을 도출하기 위해 드럼회전테이블의 속도결정 및 모의드럼을 이용한 방사능측정 등을 통해 핵종 농도 분석시의 오차를 30% 이내로 유지할 수 있었다.

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The Analytical Radioactive Waste Repository Source Term REPS Model (방사성폐기물 처분장 선원항 REPS 모델)

  • Kim, Chang-Lak;Cho, Chan-Hee;Park, Kwang-Sub;Kim, Jinwung
    • Nuclear Engineering and Technology
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    • v.22 no.4
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    • pp.315-325
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    • 1990
  • The analytical repository source term (REPS) computer code is developed for the safety assessment of radioactive waste geologic repository. For reliable prediction of the leach rates for various radionuclides, degradation of concrete structures, corrosion rate of waste container, degree of corrosion on the container surface, and the characteristics of radionuclides are considered in this REPS code. For the validation of the radionuclide leach rates predicted by the REPS model, the calculated leach rates of Cs-137, Sr-85, and Co-60 are compared with two reported leaching test results. Cesium and strontium leach congruently, and the leaching test results of these species can be reproduced by the congruent leaching model included in the REPS model. In case of cobalt, the solid diffusion model is in good agreement with the leaching test results.

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A Study on the Atmospheric Deposition of Radionuclides($^137Cs$ and $^210Pb$) on the Korean Peninsula (대기를 통하여 한반도 지표면으로 공급되는 방사성 핵종( $^137Cs$$^210Pb$)에 관한 연구)

  • 이윤구;김석현;홍기훈;이광우
    • Journal of Korean Society for Atmospheric Environment
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    • v.11 no.4
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    • pp.351-359
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    • 1995
  • In order to investigate geochemical behaviors of artificial radionuclide($^{137}$ Cs), the fallout deposition of arificial radioisotope($^{137}$ Cs) was measured from May to October in 1994 at the Korea Ocean Research & Development Institute(KORDI), Ansan, Kyunggido, Korea. And to study radioisotopic behavior and cumulative action in soil, soil samples were collected from Kwang-Leung Forest, Kyunggidom and artificial radioisotope ($^{137}$ Cs) and natural radioisotope($^{210}$ Pb) were identified. The amount of $^{137}$ Cs in atmosphere collected by wet deposition process in May was found to be 4.95 to 11.96mBq m$^{-2}$ whereas the amounts of $^{137}$ Cs by dry deposition process in May and October were found to be 4.0mBq g$^{-1}$ and 3.0mBq g$^{-1}$ , respectively. The amount of $^{137}$ Cs accumulated in soil was measured to be 311mBq cm$^{-2}$ , which contained 83% of the total inputs from atmospheric fallout (374 mBq cm$^{-2}$ ) since 1960s. In addition, the accumulation rate and the annual flux of $^{210}$ Pb into soils were 0.32cm yr$^{-1}$ and 34 mBq cm$^{-2}$ yr$^{-1}$ , respectively. Conclusively, it was found that arificial radioisotopes were mainly from the stratosphere and soil resupension of continental China through the troposphere.

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Influence of the Monitoring Interval and Intake Pattern for the Evaluation of Intake (내부피폭 감시주기 및 섭취형태가 방사성핵종 섭취량 평가에 미치는 영향)

  • Jong-Il Lee;Tae-Young Lee;Si-Young Chang;Jai-Ki Lee
    • Journal of Nuclear Fuel Cycle and Waste Technology(JNFCWT)
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    • v.2 no.1
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    • pp.53-59
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    • 2004
  • A variety of factors such as the pattern of intake (acute or chronic), monitoring interval and the characteristics of the radionuclides could have a significant influence on the estimates for the intake and internal dose. The relative differences of the assessed intakes based on the assumption of an acute intake to that of a chronic intake were evaluated by using the predicted bioassay quantity in the whole body or organs for an acute and chronic intake through the inhalation of $^{125}$ I, $^{137}$ C, $^{235}$ U with the AMAD of 1 ${\mu}{\textrm}{m}$ and 5 ${\mu}{\textrm}{m}$ for the monitoring intervals of 7, 14, 30, 60, 90, 120, 180, 360 days, respectively, The relative difference of the assessed intakes based on the intake pattern is affected by the monitoring interval, radionuclide and absorption type, but the particle size has little influence on the difference of the assessed intakes based on the intake pattern. The maximum monitoring interval, which is defined as the monitoring interval that the relative difference of the assessed intakes based on the assumption of an acute intake to that of a chronic intake is less than 10%, is 60 d for $^{125}$ I with Type F, 180 d for $^{137}$ C with Type F, 90 d for $^{235}$ U with Type M, and 360 d for $^{235}$ U with Type S. It was concluded that an intake pattern has little influence on the estimates of the assessed intake in the case where the monitoring interval is shorter than the maximum monitoring interval for each radionuclide.

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