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http://dx.doi.org/10.9713/kcer.2017.55.6.837

Recirculating Integrated System for the Treatment of Authentic Integrated-textile-dyeing Wastewater from Dyeing Industrial Complex  

Lee, Eun Ju (Department of Chemical Engineering, Daegu University and Research Institute for Industrial and Environmental Waste Air Treatment)
Lim, Kwang-Hee (Department of Chemical Engineering, Daegu University and Research Institute for Industrial and Environmental Waste Air Treatment)
Publication Information
Korean Chemical Engineering Research / v.55, no.6, 2017 , pp. 837-845 More about this Journal
Abstract
A recirculating integrated system composed of a fluidized biofilter filled with waste-tire crumb media fixed with return sludge from wastewater treatment facility of D dyeing industrial center, and a UV/photocatalytic reactor packed with calcined $TiO_2$ coated-glass beads as photocatalyst-support, was constructed and was run to treat authentic textile-dyeing wastewater from D-dyeing industrial center, which was mixed with an alkaline polyester-weight-reducing wastewater and a wastewater from sizing process. As a result, its total removal efficiency(RE(tot)) of $COD_{cr}$ and colors were ca. 81% and 55%, respectively. The synergy effect of the recirculating integrated system to enhance total removal efficiency(RE(tot)) of $COD_{cr}$ and colors were evaluated at most ca. 7% and 3%, respectively. The fluidized biofilter and the UV/photocatalytic reactor were responsible for ca. 94% and 6% of the total $COD_{cr}$ removal efficiency, respectively, and were also responsible for ca. 86% and 14% of the total color-removal efficiency, respectively. Thus, the degree of the UV/photocatalytic reactor-unit process's contribution to RE(tot) of color, was about 2.4 times of that to RE(tot) of $COD_{cr}$. Therefore, the UV/photocatalytic reactor facilitated the more effective elimination of colors by breaking down the chemical bonds oriented from colors of dyes such as azo-bond, than $COD_{cr}$. In addition, the effect of the removal efficiency of each unit process(i.e., the fluidized biofilter or the UV/photocatalytic reactor) of the recirculating integrated system on RE(tot) of $COD_{cr}$ and colors, was analysed by establishing its model equation with an analytic correlation.
Keywords
Authentic integrated-textile-dyeing Wastewater; Fluidized biofilter; Photocatalytic reactor; Recirculating integrated system; $COD_{cr}$; Color; Model equation;
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Times Cited By KSCI : 1  (Citation Analysis)
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1 Harrelkas, F., Paulo, A., Alves, M. M., El Khadir, L., Zahraa, O., Pons, M. N. and van der Zee, F. P., "Photocatalytic and Combined Anaerobic-photocatalytic Treatment of Textile Dyes," Chemosphere, 72, 1816-1822(2008).   DOI
2 Chebli, D., Fourcade, F., Brosillon, S., Nacef, S. and Amrane, A., "Integration of Photocatalysis and Biological Treatment for Azo Dye Removal-application to AR183," Environmental Technology, 32(5), 507-514(2011).   DOI
3 Shah, M. P., "Combined Application of Biological-photocatalytic Process in Degradation of Reactive Black Dye: An Excellent Outcome," American Journal of Microbiological Research, 1(4), 92-97(2013).   DOI
4 Wu, C., Kuo, C. and Chang, C., "Decolorization of C. I. Reactive Red 2 by Catalytic Ozonation Processes," J. Hazard. Mater., 153, 1052-1058(2008).   DOI
5 Fahmi, Nishihima, W. and Okada, M., "Improvement of DOC Removal by Multi-stage AOP Biodegradation Process, Enviro 2002 & IWA 3rd World Water Conference, Melbourne, Australia (2002).
6 Scheck, C. K. and Frimmel, F. H., "Degradation of Phenol and Salicylic Acid by Ultraviolet Radiation/hydrogenperoxide/oxygen," Water Res., 29(10), 2346-2352(1995).   DOI
7 Yang, S., Wang, P., Yang, X., Shan, L., Zhang, W., Shao, X. and Niu, R., "Degradation Efficiencies of Azo Dye Acid Orange 7 by the Interaction of Heat, UV and Anions with Common Oxidants: Persulfate, Peroxymonosulfate and Hydrogen Peroxide," J. Hazard. Mater., 179, 552-558(2010).   DOI
8 Chang, S.-H., Chuang, S.-H., Li, H.-C., Liang, H.-H. and Huang, L.-C., "Comparative Study on the Degradation of I. C. Remazol Brilliant Blue R and I. C. Acid Black 1 by Fenton oxidation and $Fe^0$/air Process and Toxicity Evaluation," J. Hazard. Mater., 166, 1279-1288(2009).   DOI
9 Zhang, X., Wu, Y., Xiao, G., Tang, Z., Wang, M., Liu, F. and Zhu, X., "Simultaneous Photocatalytic and Microbial Degradation of Dye-containing Wastewater by a Novel g-C3N4-P25/photosynthetic Bacteria Composite," PLoS One, 12(3), e0172747(doi: 10.1371/ journal.pone.0172747)(2017).   DOI
10 Jafari, N., Karsa-Kermanshahi, R., Soudi, M. R., Mahvi, A. H., and Gharavi, S., "Degradation of a Textile Reactive Azo Dye by a Combined Biological-photocatalytic Process: Candida tropicalis Jks2-$TiO_{2}$/UV," Iranian Journal of Environmental Health Sciences & Engineering, 9(33), 1-7(2012).   DOI
11 Ma, L. and Zhang, W. X., "Enhanced Biological Treatment of Industrial Wastewater with Bimetallic Zero-valent Iron," Environ. Sci. Technol., 42(15), 5384-9(2008).   DOI
12 Lin, Y. T., Weng, C. H. and Chen, F. Y., "Effective Removal of AB24 Dye by Nano/micro-size Zero-valent iron," Sep. Purif. Technol., 64(1), 26-30(2008).   DOI
13 Shu, H. Y., Chang, M. C. and Chang, C. C., "Integration of Nanosized Zero-valent Iron Particles Addition with $UV/H_{2}O_{2}$ Process for Purification of Azo Dye Acid Black 24 Solution," J. Hazard. Mater., 167, 1178-84(2009).   DOI
14 Paprowicz, J. and Slodczyk, S., "Application of Biologically Activated Sorptive Columns for Textile Waste Water Treatment," Environ. Technol. Lett., 9, 271-280(1988).   DOI
15 Eren, Z., "Ultrasound as a Basic and Auxiliary Process for Dye Remediation: a Review," J. Environ. Manag., 104, 127-141(2012).   DOI
16 Jin, X. C., Liu, G. Q., Xu, Z. H. and Tao, W. Y., "Decolorization of a Dye Industry Effluent by Aspergillus fumigatus XC6," Appl. Microbiol. Biotechnol., 74, 239-243(2007).   DOI
17 Kalra, S. S., Mohan, S., Sinha, A. and Singh, G., "Advance Oxidation Processes for Treatment of Textile and Dye Wastewater: a Review," 2nd International Conference on Environmental Science and Development, Singapore (2011).
18 Zhang, Y.-G., MA, L.-L., Li, J.-L. and YU, Y., "In situ Fenton Reagent Generated from $TiO_{2}/Cu_{2}O$ Composite Film: a New Way to Utilize $TiO_{2}$ Under Visible Light Irradiation," Environ. Sci. Technol., 41, 6264-6269(2007).   DOI
19 Peternel, I. T., Koprivanac, N., Bozic, A. M. L., Kusic, H. M., "Comparative Study of $UV/TiO_{2}$, UV/ZnO and Photo-Fenton Processes for the Organic Reactive Dye Degradation in Aqueous Solution," J. Hazard. Mater., 148, 477-484(2007).   DOI
20 Akyol, A. and Bayramoglu, M., "The Degradation of An Azo Dye in a Batch Slurry Photocatalytic Reactor," Chem. Eng. Process., 47, 2150-2156(2008).   DOI
21 Lim, K.-H., Park, S. W., Lee, E. J. and Hong, S. H., "Treatment of Mixed Solvent Vapors with Hybrid System Composed of Biofilter and Photo-catalytic Reactor," Korean J. Chem. Eng., 22(1), 70-79(2005).   DOI
22 Perey, J. R., Chiu, P. C., Huang, C. P., and Cha, D. K., "Zero-valent Iron Pretreatment for Enhancing the Biodegradability of Azo Dyes," Water Environ. Res., 74(3), 221-5(2002).   DOI
23 Saxe, J. P., Lubenow, B. L., Chiu, P. C., Huang, C. P. and Cha, D. K., "Enhanced Biodegradation of Azo Dyes Using an Integrated Elemental Iron-Activated Sludge System: I. Evaluation of System Performance," Water Environ. Res., 78(1), 19-25(2006).   DOI
24 Choi, Y., Park, B. and Cha, D. K. Cha, "Enhancing Biological Treatment of Dye Wastewater with Zero-valent Iron," Korean J. Chem. Eng., 32(9), 1812-1817(2015).   DOI
25 Lee, E. J. and Lim, K.-H., "Treatment of an Authentic Textiledyeing Wastewater Utilizing a Fluidized Biofilter and Hybrid Recirculating System Composed of the Fluidized Biofilter and a UV/photocatalytic Reactor," Korean Chem. Eng. Res., 53(1), 71-77(2015).   DOI
26 Lim, K.-H., Jung, Y.-J., Park, L. S. and Min, K.-S., "Preparation and Characteristics of Media from Waste Tire Powder for Wastewater Treatment," Korean Chem. Eng. Res., 39(5), 600-606(2001).
27 Lee, E. J. and Lim, K.-H., "Transient Behavior of Hybrid System Composed of a Photo-catalytic Reactor and a Biofilter to Treat Waste-air Containing Highly Concentrated-hydrogen Sulfide with High Loading," Journal of Chemical Engineering of Japan, 46(9), 636-647(2013).   DOI
28 Muruganandham, M. and Swaminathan, M., "Photocatalytic Decolourisation and Degradation of Reactive Orange 4 by $TiO_{2}$-UV Process," Dyes. Pigm., 68, 133-142(2006).   DOI