Journal of Powder Materials (한국분말재료학회지)

The Korean Powder Metallurgy & Materials Institute (한국분말재료학회 (*구 분말야금학회))
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A Review of Inorganic Solid Electrolytes for All-Solid-State Lithium Batteries: Challenges and Progress

  • Seul Ki Choi (Department of Hydrogen Energy, Dankook University) ;
  • Jaehun Han (Department of Energy Engineering, Dankook University) ;
  • Gi Jeong Kim (Department of Chemistry, Dankook University) ;
  • Yeon Hee Kim (Department of Chemistry, Dankook University) ;
  • Jaewon Choi (Department of Chemistry and Research Institute of Molecular Alchemy, Gyeongsang National University) ;
  • MinHo Yang (Department of Hydrogen Energy, Dankook University)
  • Received : 2024.07.26
  • Accepted : 2024.08.19
  • Published : 2024.08.28
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Abstract

All-solid-state lithium batteries (ASSLBs) are receiving attention as a prospective next-generation secondary battery technology that can reduce the risk of commercial lithium-ion batteries by replacing flammable organic liquid electrolytes with non-flammable solid electrolytes. The practical application of ASSLBs requires developing robust solid electrolytes that possess ionic conductivity at room temperature on a par with that of organic liquids. These solid electrolytes must also be thermally and chemically stable, as well as compatible with electrode materials. Inorganic solid electrolytes, including oxide and sulfide-based compounds, are being studied as promising future candidates for ASSLBs due to their higher ionic conductivity and thermal stability than polymer electrolytes. Here, we present the challenges currently facing the development of oxide and sulfide-based solid electrolytes, as well as the research efforts underway aiming to resolve these challenges.

Keywords

Acknowledgement

This work was supported by the National Research Foundation of Korea(NRF) grant funded by the Korea government(MSIT) (2022R1C1C1006536 and RS-2023-00221237).

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