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Study on (n, α) reactions for the production of 51Cr, 89Sr, 99Tc, 131I, 133Xe, 137Cs and 153Sm radioisotopes used in nuclear medicine

  • Hallo M. Abdullah (Department of Physics, College of Science, Salahaddin University-Hawler) ;
  • Ali H. Ahmed (Department of Physics, College of Science, Salahaddin University-Hawler)
  • Received : 2023.02.13
  • Accepted : 2023.05.19
  • Published : 2023.09.25

Abstract

Nuclear medicine seems to be a decent choice of medicine in the recent decade. The radioactive isotopes 51Cr, 89Sr, 99Tc, 131I, 133Xe, 137Cs and 153Sm are extremely essential in nuclear medicine. The excitation functions of the 54Fe (n, α) 51Cr, 92Zr (n, α) 89Sr, 102Rh (n, α) 99Tc, 134Cs (n, α) 131I, 136Ba (n, α) 133Xe, 140La (n, α) 137Cs and 156Gd (n, α) 153Sm reactions were calculated in this study using the EMPIRE 3.2.3 and TALYS 1.95 nuclear codes. Additionally, the cross sections at 14-15 MeV were calculated using empirical formulae and the experimental data. The computer codes were compared to the experimental data and Empirical formulas as well as the evaluated data (TENDL 2021, JENDL 3.3, JENDL 5, JEFF 3.3, EAF 2010, CENDL 3.1, CENDL 3.2, ROSFOND 2010, FENDL 3.2 b, and BROND 3.1).

Keywords

References

  1. Hallo M. Abdullah, Ali H. Ahmed, Semi-empirical formula for (n, α) reaction cross sections at 14-15 MeV neutrons, Appl. Radiat. Isot. 189 (2022), 110396, https://doi.org/10.1016/j.apradiso.2022.110396. ISSN 0969-8043.
  2. Hallo M. Abdullah, Ali H. Ahmed, Study on (n,p) reactions of 58Ni, 99Tc, 99Ru, 131Xe, 133Cs and 186Os radioisotopes used in medicine, Nucl. Eng. Technol. 55 (1) (2023) 304-309, https://doi.org/10.1016/j.net.2022.09.014. ISSN 1738-5733.
  3. Mustafa Yigit, Study on (n,p) reactions of 58,60,61,62,64Ni using new developed empirical formulas, Nucl. Eng. Technol. 52 (4) (2020) 791-796, https://doi.org/10.1016/j.net.2019.10.009. ISSN 1738-5733.
  4. Hallo M. Abdullah, AliH. Ahmed, Empirical formulae for (n,p) reaction cross sections at 14-15 MeV, Int. J. Mod. Phys. E 31 (5) (2022), https://doi.org/10.1142/S0218301322500495. ISSN 0218-3013.
  5. Mustafa Yigit, A. Kara, Model-based predictions for nuclear excitation functions of neutron-induced reactions on 64,66-68Zn targets, Nucl. Eng. Technol. 49 (5) (2017) 996-1005, https://doi.org/10.1016/j.net.2017.03.006. ISSN 1738-5733.
  6. Mustafa Yigit, Analysis of cross sections of (n,t) nuclear reaction using different empirical formulae and level density models, Appl. Radiat. Isot. 139 (2018) 151-158, https://doi.org/10.1016/j.apradiso.2018.05.008. ISSN 0969-8043.
  7. Mustafa Yigit, Cross section analysis for neutron and proton induced reactions on 55Mn material, J. Fusion Energy 34 (2015) 1392-1398, https://doi.org/10.1007/s10894-015-9978-4. ISSN 1572-9591.
  8. Mustafa Yigit, Eyyup Tel, Study on (n, 2n) and (n,p) reactions of strontium nucleus, Nucl. Eng. Des. 293 (2015) 97-104, https://doi.org/10.1016/j.nucengdes.2015.07.043. ISSN 0029-5493.
  9. Mustafa Yigit, New empirical formulae for (n,t) cross sections at 14.6 MeV, Appl. Radiat. Isot. 128 (2017) 307-310, https://doi.org/10.1016/j.apradiso.2017.07.047. ISSN 0969-8043.
  10. Experimental Nuclear Reaction Data (EXFOR), 2023. http://www.nndc.bnl.gov/exfor/.
  11. Evaluated Nuclear Data File (ENDF), 2023. https://www-nds.iaea.org/exfor/endf.htm.
  12. M. Herman, M. Herman, R. Capote, M. Sin, A. Trkov, B. V Carlson, P. Oblozinsky, C.M. Mattoon, H. Wienke, S. Hoblit, EMPIRE-3.2 Malta Modular System for Nuclear Reaction Calculations and Nuclear Data Evaluation Users Manual, others, 2013, https://www.bnl.gov/isd/documents/82108.pdf.
  13. A. Koning, S. Hilaire, M. Duijvestijn, TALYS-1.95, A Nuclear Reaction Program, NRG-1755 ZG Petten, Netherlands, 2019. https://tendl.web.psi.ch/tendl_2021/talys.html.
  14. J.J. Griffin, Statistical model of intermediate structure, Phys. Rev. Lett. 17 (1966) 478, https://doi.org/10.1103/PhysRevLett.17.478. ISSN 1079-7114.
  15. C.K. Cline, M. Blann, The pre-equilibrium statistical model: description of the nuclear equilibration process and parameterization of the model, Nucl. Phys. 172 (2) (1971) 225-259, https://doi.org/10.1016/0375-9474(71)90713-5. ISSN 0375-9474.
  16. Isao Kumabe, Katsuya Fukuda, Empirical formulas for 14-MeV (n,p) and (n, α) cross sections, J. Nucl. Sci. Technol. 24 (1987) 839-843, https://doi.org/10.1080/18811248.1987.9735887. ISSN 1881-1248.
  17. Y. Kasugai, Y. Ikeda, H. Yamamoto, K. Kawade, 3.15 Systematics of Activation Cross Sections for 13. 4-15. 0 MeV Neutrons, JAERI-Conf, 1995, p. 181. https://inis.iaea.org/collection/NCLCollectionStore/_Public/27/038/27038623.pdf?r=1.
  18. F.I. Habbani, K.T. Osman, Systematics for the cross-sections of the reactions (n,p) ,(n, α) and (n, 2n) at 14.5 MeV neutrons, Appl. Radiat. Isot. 54 (2) (2001) 283-290, https://doi.org/10.1016/S0969-8043(00)00275-X. ISSN 0969-8043.
  19. E. Tel, S. Okuducu, M.H. Bolukdemir, G. Tanir, Semi-empirical systematics of (n, 2n),(n, α) reactions cross sections at 14-15 MeV neutron energy, Int. J. Mod. Phys. E 17 (3) (2008) 567-583, https://doi.org/10.1142/S0218301308009914. ISSN 1793-6608.
  20. A.Y. Konobeyev, U. Fischer, C.H.M. Broeders, Improved systematics of (n, α) reaction cross-section at 14.5 MeV, Appl. Radiat. Isot. 67 (2) (2009) 357-361, https://doi.org/10.1016/j.apradiso.2008.07.009. ISSN 0969-8043.
  21. Zhimin Wang, Xiao Fan, Luyu Zhang, Huaiyong Bai, Jinxiang Chen, Guohui Zhang, Yu M. Gledenov, M.V. Sedysheva, L. Krupa, G. Khuukhenkhuu, Cross sections of the 56Fe (n, α) 53Cr and 54Fe (n, α) 51Cr reactions in the MeV region, Phys. Rev. C 92 (4) (2015). ISSN 2469-9985, https://journals.aps.org/prc/abstract/10.1103/PhysRevC.92.044601.
  22. W. Mannhart, D. Schmidt, Measurement of neutron activation cross sections in the energy range from 8 MeV to 15 MeV, Physikalisch-Technische Bundesanstalt, Braunschweig (Germany) Neutronenphysik, PTB Rep. PTB-N-53 (2007) 144. ISSN 0936-0492, https://www.ptb.de/cms/en.html.
  23. J.W. Meadows, D.L. Smith, L.R. Greenwood, L.P. Geraldo, W. Mannhart, G. Borker, Measurements of the neutron cross section for Fe-54 (n, alpha) Cr-51 between 5.3 and 14.6 MeV, nuclear data for science and technology, in: Conference Paper, 1992, pp. 288-290. https://link.springer.com/chapter/10.1007/978-3-642-58113-7_81.
  24. Wenrong Zhao, Hanlin Lu, Weixiang Yu, Xialin Yuan, Compilation of Measurements and Evaluations of Nuclear Activation Cross Sections for Nuclear Data Applications, International Atomic Energy Agency, 1989. https://inis.iaea.org/collection/NCLCollectionStore/_Public/21/051/21051899.pdf?r=1.
  25. Huaiyong Bai, Haoyu Jiang, Yi Lu, Zengqi Cui, Jinxiang Chen, Guohui Zhang, Yu M. Gledenov, M.V. Sedysheva, G. Khuukhenkhuu, Xichao Ruan, Hanxiong Huang, Jie ren, and qiwen fan, 56,54Fe (n, α) 53,51Cr cross sections in the MeV region, Phys. Rev. C 99 (Issue 2) (2019). ISSN 2469-9985, https://journals.aps.org/prc/abstract/10.1103/PhysRevC.99.024619.
  26. V.N. Levkovskii, Empirical behavior of the (n,p) cross-section for 14-15 MeV neutrons, Sov. Phys. - JETP 18 (1) (1964) 213-217. ISSN 1063-7761, http://jetp.ras.ru/cgi-bin/dn/e_018_01_0213.pdf.
  27. S.M. Qaim, G. Stoecklin, Measurement and Systematics of Cross Sections for Common and Low Yield 14 MeV Neutron Induced Nuclear Reactions on Structural FR-Material and Transmuted Species, EXFOR, 1974. https://wwwnds.iaea.org/exfor/servlet/X4sSearch5.
  28. V.N. Levkovskii, V. Gp, K. Ge, V.M. Stepanov, Cross sections for (n,p) and (n, alpha) reactions with 14.8-MeV neutrons 8 (1970) 1-4. https://www-nds.iaea.org/exfor/servlet/X4sSearch5.
  29. I.A. Abbasi, J.H. Zaidi, M. Arif, S. Waheed, M.S. Subhani, Measurement of fission neutron spectrum averaged cross sections of some threshold reactions on zirconium: production possibility of no-carrier-added 90Y in a nuclear reactor, Radiochim. Acta 94 (2006) 381-384, https://doi.org/10.1524/ract.2006.94.8.381. ISSN 0033-8230.
  30. B.P. Bayhurst, R.J. Prestwood, (n,p) and (n, α) excitation functions of several nuclei from 7$0 to 19.8 MeV, J. Inorg. Nucl. Chem. 23 (3-4) (December 1961) 173-185, https://doi.org/10.1016/0022-1902(61)80244-3.
  31. C.H. Reed, ABSOLUTE (n, 2n),(n, p gamma), AND (n, alpha gamma) cross sections for 14.1-mev neutrons on zirconium and the calibration of a crystal scintillation spectrometer, EXFOR (1960). https://www-nds.iaea.org/exfor/.
  32. L. Hanlin, Z. Wenrong, Y. Weixiang, Activation cross sections for element barium, Chin. J. Nucl. Phys. 14 (1992). ISSN 1674-1137, https://www.osti.gov/etdeweb/biblio/7068551.
  33. P.R. Prasad, J.R. Rao, E. Kondaiah, Cross sections for (n, 2n),(n, α) and (n,p) reactions in rare-earth isotopes at 14.2 MeV, Nucl. Phys. 125 (1969) 57-64. ISSN 0375-9474, https://www-nds.iaea.org/exfor. https://doi.org/10.1016/0375-9474(69)90828-8
  34. R.F. Coleman, B.E. Hawker, L.P. O'connor, J.L. Perkin, Cross sections for (n,p) and (n, α) reactions with 14.5 MeV neutrons, Proc. Phys. Soc. 73 (2) (1959) 215. ISSN 0370-1328, https://iopscience.iop.org/article/10.1088/0370-1328/73/2/308.
  35. S.M. Qaim, Activation cross sections of (n, α) reactions at 14.7 MeV in the region of rare earths, Radiochim. Acta 35 (1984) 5-10, https://doi.org/10.1524/ract.1984.35.1.5. ISSN 2193-3404.
  36. T. Khromyleva, I. Bondarenko, A. Gurbich, V. Ketlerov, V. Khryachkov, P. Prusachenko, Investigation of (n, $α$) reaction cross sections for a number of structural material isotopes, Nucl. Sci. Eng. 191 (3) (2018) 282-290, https://doi.org/10.1080/00295639.2018.1463746. ISSN: 0029-5639.