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Study on (n,p) reactions of 58Ni, 99Tc, 99Ru, 131Xe, 133Cs and 186Os radioisotopes used in medicine

  • Hallo M. Abdullah (Department of Physics, College of Science, Salahaddin University-Hawler) ;
  • Ali H. Ahmed (Department of Physics, College of Science, Salahaddin University-Hawler)
  • Received : 2022.07.27
  • Accepted : 2022.09.12
  • Published : 2023.01.25

Abstract

In the last decade, nuclear medicine appears to be a good choice of medicine. 58Co, 99Mo, 99Tc, 99Re, 133Xe and 186Re are very important radionuclides for nuclear medicine. In this study, the excitation functions of 58Ni (n, p) 58Co, 99Tc (n, p) 99Mo, 99Ru (n, p) 99Tc, 131Xe (n, p) 131I, 133Cs (n, p) 133Xe and 186Os (n, p) 186Re nuclear reactions were calculated at neutron energies between 1 and 20 MeV using TALYS 1.95 and EMPIRE 3.2 nuclear codes. Furthermore, the cross sections were calculated with the empirical formula derived in our past study at 14-15 MeV. The obtained results were compared with the measured values in EXFOR library, and with the evaluated data of (JENDL-4.0/HE, JEFF-3.3, TENDL-2019, ENDF/B-VIII.0, IRDFF-II, JENDL/ImPACT-18). The results are in good agreement with those of the evaluated data libraries and experimental results and indicates that these radioisotopes can be produced by smaller cyclotrons.

Keywords

References

  1. S.S. Noori, Iskender Akkurt, N.K. Demir, Excitation functions of proton induced reactions of some radioisotopes used in medicine, Open Chem 16 (2018) 810-816. https://doi.org/10.1515/chem-2018-0085
  2. A.L. Goldenhart, S. Senthilkumaran, Nuclear medicine test, in: StatPearls, StatPearls Publishing, 2021 [Internet].
  3. M. Yi\ugit, Study of cross sections for (n,p) reactions on Hf, Ta and W isotopes, Appl. Radiat. Isot. 174 (2021), 109779.
  4. I. Radioisotopes, R.S. No, 2: production of long lived parent radionuclides for generators: 68Ge, 82Sr, 90Sr and 188W, IAEA Radioisot Radiopharm Ser 15 (2010).
  5. H.M. Abdullah, A.H. Ahmed, Empirical systematics for (n,p) reaction cross sections at 14-15 MeV neutrons, Indian J. Phys. (2022) 1-12.
  6. T.S. Reshid, Study of some structural fusion materials for (n, 2n) reactions, J. Fusion Energy 34 (2015) 746-750. https://doi.org/10.1007/s10894-015-9879-6
  7. Z. Karimi, M. Sadeghi, A. Ezati, Modeling and experimental production yield of 64Cu with natCu and natCu-NPs in Tehran Research Reactor, Nucl. Eng. Technol. 51 (2019) 269-274. https://doi.org/10.1016/j.net.2018.08.008
  8. M. Herman, M. Herman, R. Capote, M. Sin, A. Trkov, B. V Carlson, P. Oblozinsky, C.M. Mattoon, H. Wienke, S. Hoblit, et al., EMPIRE-3.2 Malta Modular System for Nuclear Reaction Calculations and Nuclear Data Evaluation Users Manual, 2013.
  9. A.J. Koning, S. Hilairey, M. Duijvestijn, TALYS-1.4: A Nuclear Reaction Program. User Manual, NRG, Petten, The Netherlands, 2009.
  10. J.J. Griffin, Statistical model of intermediate structure, Phys. Rev. Lett. 17 (1966) 478.
  11. C.K. Cline, M. Blann, The pre-equilibrium statistical model: description of the nuclear equilibration process and parameterization of the model, Nucl. Phys. A. 172 (1971) 225-259. https://doi.org/10.1016/0375-9474(71)90713-5
  12. A.J. Koning, S. Hilaire, M. Duijvestijn, TALYS-1.2 A Nuclear Reaction Program, User Manual, NRG, Netherlands, 2009, pp. 16-18.
  13. S. Ait-Tahar, The systematics of (n,p) cross sections for 14 MeV neutrons, J. Phys. G Nucl. Phys. 13 (1987) L121.
  14. Y. Kasugai, Y. Ikeda, H. Yamamoto, K. Kawade, Systematics for (n,p) excitation functions in the neutron energy between 13.3 and 15.0 MeV, Ann. Nucl. Energy 23 (1996) 1429-1444. https://doi.org/10.1016/0306-4549(95)00114-X
  15. C.H.M. Broeders, A.Y. Konobeyev, Semi-empirical systematics of (n,p) reaction cross-section at 14.5, 20, and 30 MeV, Nucl. Phys. A. 780 (2006) 130-145. https://doi.org/10.1016/j.nuclphysa.2006.09.015
  16. M. Yigit, M.E. Korkmaz, On the behavior of cross-sections of charged particle-induced reactions of 181Ta target, Mod. Phys. Lett. A. 33 (2018), 1850155.
  17. A.H. Ahmed, Systematics of (n,p) reaction cross-sections for light element target nuclei at 14.5 MeV neutrons, Int. J. Mod. Phys. E. 27 (2018), 1850079.
  18. H.A. Mahmud, A.H. Ahmad, Empirical formulae for (n,p) reaction cross-sections at 14-15 MeV neutrons, Int. J. Mod. Phys. E. 27 (2022), 1850079.
  19. C.M. Buczko, J. Csikai, S. Sud ar, A. Grallert, S.A. Jonah, B.W. Jimba, T. Chimoye, M. Wagner, Excitation functions and isomeric cross section ratio of the Ni 58 (n,p) 58 Co m, g reactions from 2 to 15 MeV, Phys. Rev. C 52 (1995) 1940.
  20. A.A. Filatenkov, Neutron Activation Cross Sections Measured at KRI in Neutron Energy Region 13.4-14.9 MeV, Rep. INDC (CCP)-0460, 2016.
  21. W. Mannhart, D. Schmidt, Measurement of Neutron Activation Cross Sections in the Energy Range from 8 MeV to 15 MeV, 2007.
  22. X. Huang, W. Yu, X. Han, W. Zhao, H. Lu, J. Chen, Z. Shi, G. Tang, G. Zhang, The effect of low-energy neutrons on activation cross-section measurement, Nucl. Sci. Eng. 131 (1999) 267-274. https://doi.org/10.13182/NSE99-A2033
  23. Y. Ikeda, C. Konno, Y. Oyama, K. Kosako, K. Oishi, H. Maekawa, Absolute measurements of activation cross sections of 27Al (n,p) 27Mg, Al27 (n,a) 24Na, 56Fe (n,p) 56Mn, 90Zr (n, 2n) 89m+ gZr and 93Nb (n, 2n) 92mNb at energy range of 13.3-14.9 MeV, J. Nucl. Sci. Technol. 30 (1993) 870-880. https://doi.org/10.1080/18811248.1993.9734561
  24. S.M. Qaim, Nuclear reaction cross-sections for 14$7 MeV neutrons on 99Tc, J. Inorg. Nucl. Chem. 35 (1973) 3669-3675. https://doi.org/10.1016/0022-1902(73)80054-5
  25. N.W. Golchert, D.G. Gardner, J. Sedlet, Cross section of some reactions of 99Tc with 14.1 MeV neutrons, Nucl. Phys. 73 (1965) 349-352. https://doi.org/10.1016/0029-5582(65)90680-2
  26. P. Reimer, A.J. Koning, A.J.M. Plompen, S.M. Qaim, S. Sud ar, Neutron induced reaction cross sections for the radioactive target nucleus 99Tc, Nucl. Phys. A. 815 (2009) 1-17. https://doi.org/10.1016/j.nuclphysa.2008.10.014
  27. D. Kielan, A. Marcinkowski, U. Garuska, Isotopic effect in (n,p) reaction on ruthenium, Nucl. Phys. A. 559 (1993) 333-346. https://doi.org/10.1016/0375-9474(93)90157-S
  28. E. Kondaiah, N. Ranakumar, R.W. Fink, Neutron activation cross sections at 14.4 MeV for Kr and Xe isotopes, Nucl. Phys. A. 120 (1968) 337-341. https://doi.org/10.1016/0375-9474(68)90770-7
  29. R.A. Sigg, P.K. Kuroda, 14.6-MeV neutron activation cross section for the xenon isotopes, Nucl. Sci. Eng. 60 (1976) 235-238. https://doi.org/10.13182/NSE76-A26880
  30. M. Bormann, H. Jeremie, G. Andersson-Lindstroem, others, Cross sections for 14 MeV neutrons in the scintillation crystals NaI (Tl), KI (Tl), CsI (Tl) and Li-6I (Eu) component nuclear reactions, Z. Naturf., Sect. A. 15 (1960) 200.
  31. A.A. Filatenkov, S. V Chuvae, Experimental Determination of Cross Sections for Several Insufficiently Known Neutron Induced Reaction on Hevy Nuclei $(Z=74-79) $, Khlopin Radiev, Inst., 2003. Leningr. Rep. No. RI-259.