Nuclear Engineering and Technology

  • 제54권9호
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  • Pages.3250-3259
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  • 2022
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  • 1738-5733(pISSN)
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  • 2234-358X(eISSN)
한국원자력학회 (Korean Nuclear Society)
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DOI QR코드

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A novel approach for rice straw agricultural waste utilization: Synthesis of solid aluminosilicate matrices for cesium immobilization

  • Panasenko, A.E. (Institute of Chemistry, Far Eastern Branch of Russian Academy of Sciences) ;
  • Shichalin, O.O. (Far Eastern Federal University) ;
  • Yarusova, S.B. (Institute of Chemistry, Far Eastern Branch of Russian Academy of Sciences) ;
  • Ivanets, A.I. (Institute of General and Inorganic Chemistry of National Academy of Sciences of Belarus) ;
  • Belov, A.A. (Far Eastern Federal University) ;
  • Dran'kov, A.N. (Institute of Chemistry, Far Eastern Branch of Russian Academy of Sciences) ;
  • Azon, S.A. (Far Eastern Federal University) ;
  • Fedorets, A.N. (Far Eastern Federal University) ;
  • Buravlev, I. Yu (Institute of Chemistry, Far Eastern Branch of Russian Academy of Sciences) ;
  • Mayorov, V. Yu (Institute of Chemistry, Far Eastern Branch of Russian Academy of Sciences) ;
  • Shlyk, D. Kh (Institute of Chemistry, Far Eastern Branch of Russian Academy of Sciences) ;
  • Buravleva, A.A. (Far Eastern Federal University) ;
  • Merkulov, E.B. (Institute of Chemistry, Far Eastern Branch of Russian Academy of Sciences) ;
  • Zarubina, N.V. (Far East Geological Institute, Far Eastern Branch of Russian Academy of Sciences) ;
  • Papynov, E.K. (Far Eastern Federal University)
  • 투고 : 2022.01.01
  • 심사 : 2022.04.05
  • 발행 : 2022.09.25
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초록

A new approach to the use of rice straw as a difficult-to-recycle agricultural waste was proposed. Potassium aluminosilicate was obtained by spark plasma sintering as an effective material for subsequent immobilization of 137Cs into a solid-state matrix. The sorption properties of potassium aluminosilicate to 137Cs from aqueous solutions were studied. The effect of the synthesis temperature on the phase composition, microstructure, and rate of cesium leaching from samples obtained at 800-1000 ℃ and a pressure of 25 MPa was investigated. It was shown that the positive dynamics of compaction was characteristic of glass ceramics throughout the sintering. Glass ceramics RS-(K,Cs)AlSi3O8 obtained by the SPS method at 1000 ℃ for 5 min was characterized by a high density of ~2.62 g/cm3, Vickers hardness ~ 2.1 GPa, compressive strength ~231.3 MPa and the rate of cesium ions leaching of ~1.37 × 10-7 g cm-2·day-1. The proposed approach makes it possible to safe dispose of rice straw and reduce emissions into the atmosphere of microdisperse amorphous silica, which is formed during its combustion and causes respiratory diseases, including cancer. In addition, the obtained is perspective to solve the problem of recycling long-lived 137Cs radionuclides formed during the operation of nuclear power plants into solid-state matrices.

키워드

과제정보

Synthesis of initial powders, saturation with cesium ions, AAS and XRD analyses were carried out in the Institute of Chemistry FEB RAS within the State Assignment of the Ministry of Science and Higher Education of the Russian Federation Themes № 0205-2021-0001, 0205-2021-0002. Synthesis and characterization of ceramics samples were financially supported by State Assignment of the Ministry of Science and Higher Education of the Russian Federation topic number 00657-2020-0006. The study of calculation of cesium leaching and density studies were studied by the financial support of the Russian Foundation for Basic Research, project No. 19-33-90150. The investigation was financially supported by Russian Science Foundation (project No. 21-73-00304). The work involved equipment of integrated common use center and interdisciplinary in the field of nanotechnologies and new functional materials (Far Eastern Federal University, Vladivostok, Russia), and also common use center "Far Eastern Center for Structural Research" (Institute of Chemistry, Far Eastern Branch of the Russian Academy of Sciences, Vladivostok, Russia).

참고문헌

  1. P. Szajerski, A. Bogobowicz, A. Gasiorowski, Cesium retention and release from sulfur polymer concrete matrix under normal and accidental conditions, J. Hazard Mater. 381 (2020) 121180, https://doi.org/10.1016/j.jhazmat.2019.121180.
  2. M.Z. Jacobson, Review of solutions to global warming, air pollution, and energy security, Energy Environ. Sci. 2 (2009) 148-173, https://doi.org/10.1039/b809990c.
  3. S.J. Zinkle, G.S. Was, Materials challenges in nuclear energy, Acta Mater. 61 (2013) 735-758, https://doi.org/10.1016/j.actamat.2012.11.004.
  4. M. Chino, H. Nakayama, H. Nagai, H. Terada, G. Katata, H. Yamazawa, Preliminary estimation of release amounts of 131i and 137cs accidently discharged from the fukushima daiichi nuclear power plant into the atmosphere, J. Nucl. Sci. Technol. 48 (2011) 1129-1134, https://doi.org/10.1080/18811248.2011.9711799.
  5. L.H. Ortega, M.D. Kaminski, S.M. McDeavitt, Pollucite and feldspar formation in sintered bentonite for nuclear waste immobilization, Appl. Clay Sci. 50 (2010) 594-599, https://doi.org/10.1016/j.clay.2010.10.003.
  6. O.O. Shichalin, E.K. Papynov, V.Y. Maiorov, A.A. Belov, E.B. Modin, I.Y. Buravlev, Y.A. Azarova, A.V. Golub, E.A. Gridasova, A.E. Sukhorada, I.G. Tananaev, V.A. Avramenko, Spark plasma sintering of aluminosilicate ceramic matrices for immobilization of cesium radionuclides, Radiochemistry 61 (2019) 185-191, https://doi.org/10.1134/S1066362219020097.
  7. S.B. Yarusova, O.O. Shichalin, A.A. Belov, S.A. Azon, I.Y. Buravlev, A.V. Golub, V.Y. Mayorov, A.V. Gerasimenko, E.K. Papynov, A.I. Ivanets, A.A. Buravleva, B. Merkulov, V.A. Nepomnyushchaya, O.V. Kapustina, P.S. Gordienko, Synthesis of amorphous KAlSi 3 O 8 for cesium radionuclide immobilization into solid matrices using spark plasma sintering technique, Ceram. Int. (2021), https://doi.org/10.1016/j.ceramint.2021.10.164.
  8. O.O. Shichalin, E.K. Papynov, V.A. Nepomnyushchaya, A.I. Ivanets, A.A. Belov, A.N. Dran'kov, S.B. Yarusova, I.Y. Buravlev, A.E. Tarabanova, A.N. Fedorets, S.A. Azon, Z.E. Kornakova, S.Y. Budnitskiy, I.G. Tananaev, Y. Shi, Y. Xiong, H. Wang, Hydrothermal synthesis and spark plasma sintering of NaY zeolite as solid-state matrices for cesium-137 immobilization, J. Eur. Ceram. Soc. (2022), https://doi.org/10.1016/j.jeurceramsoc.2022.02.007.
  9. I. Yanase, S. Tamai, H. Kobayashi, Sintering of pollucite using amorphous powder and its low thermal expansion property, J. Ceram. Soc. Japan. 111 (2003) 533-536, https://doi.org/10.2109/jcersj.111.533.
  10. S.K. Jesudoss, J.J. Vijaya, K. Kaviyarasu, L.J. Kennedy, R. Jothi Ramalingam, H.A. Al-Lohedan, Anti-cancer activity of hierarchical ZSM-5 zeolites synthesized from rice-based waste materials, RSC Adv. 8 (2018) 481-490, https://doi.org/10.1039/C7RA11763A.
  11. A.I. Orlova, M.I. Ojovan, Ceramic mineral waste-forms for nuclear waste immobilization, Materials (Basel) 12 (2019), https://doi.org/10.3390/ma12162638.
  12. E.K. Papynov, O.O. Shichalin, M.A. Medkov, D.N. Grishchenko, I.A. Tkachenko, A.N. Fedorets, V.S. Pechnikov, A.V. Golub, I.Y. Buravlev, I.G. Tananaev, V.A. Avramenko, Spark plasma sintering of special-purpose functional ceramics based on UO2, ZrO2, Fe3O4/a-Fe2O3, Glas, Phys. Chem. 44 (2018) 632-640, https://doi.org/10.1134/S1087659618060159.
  13. E.K. Papynov, O.O. Shichalin, A.Y. Mironenko, A.V. Ryakov, I.V. Manakov, P.V. Makhrov, I.Y. Buravlev, I.G. Tananaev, V.A. Avramenko, V.I. Sergienko, Synthesis of high-density pellets of uranium dioxide by spark plasma sintering in dies of different types, Radiochemistry 60 (2018) 362-370, https://doi.org/10.1134/S1066362218040045.
  14. E.K. Papynov, A.S. Portnyagin, E.B. Modin, V.Y. Mayorov, O.O. Shichalin, A.P. Golikov, V.S. Pechnikov, E.A. Gridasova, I.G. Tananaev, V.A. Avramenko, A complex approach to assessing porous structure of structured ceramics obtained by SPS technique, Mater. Char. 145 (2018) 294-302, https://doi.org/10.1016/j.matchar.2018.08.044.
  15. I.O. Ali, T.M. Salama, M.S. Thabet, K.S. El-Nasser, A.M. Hassan, Encapsulation of ferro- and ferricyanide complexes inside ZSM-5 zeolite synthesized from rice straw: implications for synthesis of Prussian blue pigment, Mater. Chem. Phys. 140 (2013) 81-88, https://doi.org/10.1016/j.matchemphys.2013.02.069.
  16. R.J. Lawson, M.B. Schenker, S.A. McCurdy, B. Jenkins, L.A. Lischak, W. John, D. Scales, Exposure to amorphous silica fibers and other particulate matter during pace farming operations, Appl. Occup. Environ. Hyg 10 (1995) 677-684, https://doi.org/10.1080/1047322X.1995.10387666.
  17. I. Health, A. Iron, O. Medicine, By Rice, 1995.
  18. C.R. Melo, A.C. Francisco, N.C. Kuhnen, M.R. da Rocha, A.R. Melo, H.G. Riella, E. Angioletto, Production of zeolite from rice husk ash, Mater. Sci. Forum 798-799 (2014) 617-621. https://doi.org/10.4028/www.scientific.net/MSF.798-799.617.
  19. R.M. Mohamed, I.A. Mkhalid, M.A. Barakat, Rice husk ash as a renewable source for the production of zeolite NaY and its characterization, Arab. J. Chem. 8 (2015) 48-53, https://doi.org/10.1016/j.arabjc.2012.12.013.
  20. E.-P. Ng, G.K. Lim, G.-L. Khoo, K.-H. Tan, B.S. Ooi, F. Adam, T.C. Ling, K.-L. Wong, Synthesis of colloidal stable Linde Type J (LTJ) zeolite nanocrystals from rice husk silica and their catalytic performance in Knoevenagel reaction, Mater. Chem. Phys. 155 (2015) 30-35, https://doi.org/10.1016/j.matchemphys.2015.01.061.
  21. V. Charitha, V.S. Athira, V. Jittin, A. Bahurudeen, P. Nanthagopalan, Use of different agro-waste ashes in concrete for effective upcycling of locally available resources, Construct. Build. Mater. 285 (2021), 122851, https://doi.org/10.1016/j.conbuildmat.2021.122851.
  22. H.R. Khalid, N.K. Lee, S.M. Park, N. Abbas, H.K. Lee, Synthesis of geopolymersupported zeolites via robust one-step method and their adsorption potential, J. Hazard Mater. 353 (2018) 522-533, https://doi.org/10.1016/j.jhazmat.2018.04.049.
  23. Y. Liu, C. Yan, Z. Zhang, H. Wang, S. Zhou, W. Zhou, A comparative study on fly ash, geopolymer and faujasite block for Pb removal from aqueous solution, Fuel 185 (2016) 181-189, https://doi.org/10.1016/j.fuel.2016.07.116.
  24. Q. Ge, M. Moeen, Q. Tian, J. Xu, K. Feng, Highly effective removal of Pb2+ in aqueous solution by Na-X zeolite derived from coal gangue, Environ. Sci. Pollut. Res. 27 (2020) 7398-7408, https://doi.org/10.1007/s11356-019-07412-z.
  25. C.B. Durrant, J.D. Begg, A.B. Kersting, M. Zavarin, Cesium sorption reversibility and kinetics on illite, montmorillonite, and kaolinite, Sci. Total Environ. 610-611 (2018) 511-520, https://doi.org/10.1016/j.scitotenv.2017.08.122.
  26. E.K. Papynov, O.O. Shichalin, V.Y. Mayorov, V.G. Kuryavyi, T.A. Kaidalova, L.V. Teplukhina, A.S. Portnyagin, A.B. Slobodyuk, A.A. Belov, I.G. Tananaev, V.A. Avramenko, V.I. Sergienko, SPS technique for ionizing radiation source fabrication based on dense cesium-containing core, J. Hazard Mater. 369 (2019) 25-30, https://doi.org/10.1016/j.jhazmat.2019.02.016.
  27. N.K. Lee, H.R. Khalid, H.K. Lee, Adsorption characteristics of cesium onto mesoporous geopolymers containing nano-crystalline zeolites, Microporous Mesoporous Mater. 242 (2017) 238-244, https://doi.org/10.1016/j.micromeso.2017.01.030.
  28. F.E. Titchou, R.A. Akbour, A. Assabbane, M. Hamdani, Removal of cationic dye from aqueous solution using Moroccan pozzolana as adsorbent: isotherms, kinetic studies, and application on real textile wastewater treatment, Groundw. Sustain. Dev. 11 (2020), 100405, https://doi.org/10.1016/j.gsd.2020.100405.
  29. S. Wang, Y. Boyjoo, A. Choueib, Z.H. Zhu, Removal of dyes from aqueous solution using fly ash and red mud, Water Res. 39 (2005) 129-138, https://doi.org/10.1016/j.watres.2004.09.011.
  30. H. Nsubuga, C. Basheer, M.B. Haider, R. Bakdash, Sol-gel based biogenic silica composite as green nanosorbent for chemometric optimization of microsolid-phase extraction of beta blockers, J. Chromatogr. A 1554 (2018) 16-27, https://doi.org/10.1016/j.chroma.2018.04.044.
  31. O.V. Buyko, S.I. Metelitsa, V.N. Losev, A.E. Panasenko, A.F. Shimanskii, Biosilica layer-by-layer modified with polyamines and carboxyarsenazo for REE preconcentration prior to ICP-MS determination in lignites and volcanic fumarole sediment, Anal. Methods 12 (2020) 3813-3822, https://doi.org/10.1039/D0AY00624F.
  32. P. Sazama, O. Bortnovsky, J. Dede cek, Z. Tvaruzkova, Z. Sobalik, Geopolymer based catalystsdnew group of catalytic materials, Catal. Today 164 (2011) 92-99, https://doi.org/10.1016/j.cattod.2010.09.008.
  33. N.P. Shapkin, I.G. Khal'chenko, A.A. Yudakov, V.I. Sergienko, A.E. Panasenko, V.Y. Maiorov, L.B. Leont'ev, Synthesis of a nanocomposite based on polyethylene and modified vermiculite, Inorg. Mater. 53 (2017) 1091-1096, https://doi.org/10.1134/S0020168517100120.
  34. R.A. Bakar, R. Yahya, S.N. Gan, Production of high purity amorphous silica from rice husk, Procedia Chem. 19 (2016) 189-195, https://doi.org/10.1016/j.proche.2016.03.092.
  35. A.M.N. Moudio, H.K. Tchakoute, D.L.V. Ngnintedem, F. Andreola, E. Kamseu, C.P. Nanseu-Njiki, C. Leonelli, C.H. Ruscher, Influence of the synthetic calcium aluminate hydrate and the mixture of calcium aluminate and silicate hydrates on the compressive strengths and the microstructure of metakaolin-based geopolymer cements, Mater. Chem. Phys. 264 (2021), https://doi.org/10.1016/j.matchemphys.2021.124459.
  36. W. Simanjuntak, K.D. Pandiangan, Z. Sembiring, A. Simanjuntak, S. Hadi, The effect of crystallization time on structure, microstructure, and catalytic activity of zeolite-A synthesized from rice husk silica and food-grade aluminum foil, Biomass Bioenergy 148 (2021), 106050, https://doi.org/10.1016/j.biombioe.2021.106050.
  37. E.A. Abdelrahman, Y.G. Abou El-Reash, H.M. Youssef, Y.H. Kotp, R.M. Hegazey, Utilization of rice husk and waste aluminum cans for the synthesis of some nanosized zeolite, zeolite/zeolite, and geopolymer/zeolite products for the efficient removal of Co(II), Cu(II), and Zn(II) ions from aqueous media, J. Hazard Mater. 401 (2021) 123813, https://doi.org/10.1016/j.jhazmat.2020.123813.
  38. Properties of fly ash and rice husk ash blended geopolymer with sodium aluminate as activator solution I Eng. Appl. Sci. Res., (n.d.).
  39. S.B. Yarusova, P.S. Gordienko, A.E. Panasenko, N.N. Barinov, L.A. Zemnukhova, Sorption properties of sodium and potassium aluminosilicates from alkaline hydrolyzates of rice straw, Russ. J. Phys. Chem. A 93 (2019) 333-337, https://doi.org/10.1134/S003602441902033X.
  40. D.S. Kosson, H.A. van der Sloot, T.T. Eighmy, An approach for estimation of contaminant release during utilization and disposal of municipal waste combustion residues, J. Hazard Mater. 47 (1996) 43-75, https://doi.org/10.1016/0304-3894(95)00109-3.
  41. G. de Groot, H. van der Sloot, Determination of leaching characteristics of waste materials leading to environmental product certification, in: Stab. Solidif. Hazardous, Radioact. Mix. Wastes 2nd Vol., ASTM International, 100 Barr Harbor Drive, PO Box C700, West Conshohocken, PA 19428-2959, n.d.: pp. 149-149-22. doi:10.1520/STP19548S.